全文获取类型
收费全文 | 1233篇 |
免费 | 47篇 |
国内免费 | 137篇 |
专业分类
安全科学 | 87篇 |
废物处理 | 29篇 |
环保管理 | 174篇 |
综合类 | 501篇 |
基础理论 | 101篇 |
污染及防治 | 253篇 |
评价与监测 | 239篇 |
社会与环境 | 31篇 |
灾害及防治 | 2篇 |
出版年
2024年 | 2篇 |
2023年 | 32篇 |
2022年 | 22篇 |
2021年 | 37篇 |
2020年 | 30篇 |
2019年 | 26篇 |
2018年 | 25篇 |
2017年 | 37篇 |
2016年 | 52篇 |
2015年 | 47篇 |
2014年 | 41篇 |
2013年 | 52篇 |
2012年 | 45篇 |
2011年 | 82篇 |
2010年 | 40篇 |
2009年 | 95篇 |
2008年 | 86篇 |
2007年 | 86篇 |
2006年 | 77篇 |
2005年 | 51篇 |
2004年 | 34篇 |
2003年 | 36篇 |
2002年 | 59篇 |
2001年 | 49篇 |
2000年 | 50篇 |
1999年 | 45篇 |
1998年 | 36篇 |
1997年 | 35篇 |
1996年 | 21篇 |
1995年 | 15篇 |
1994年 | 16篇 |
1993年 | 13篇 |
1992年 | 10篇 |
1991年 | 9篇 |
1990年 | 1篇 |
1989年 | 1篇 |
1988年 | 2篇 |
1987年 | 2篇 |
1986年 | 2篇 |
1985年 | 2篇 |
1984年 | 3篇 |
1982年 | 4篇 |
1978年 | 1篇 |
1977年 | 4篇 |
1974年 | 1篇 |
1968年 | 1篇 |
排序方式: 共有1417条查询结果,搜索用时 531 毫秒
781.
We apply the entropy-based Bayesian optimizing approach of Le and Zidek to the spatial redesign of the extensive air pollution monitoring network operated by Metro Vancouver, in the Lower Fraser Valley, British Columbia. This method is chosen because of its statistical sophistication, relative to other possible approaches, and because of the very rich, two-decade long data record available from this network. The redesign analysis is applied to ozone, carbon monoxide and PM2.5 pollutants. 相似文献
782.
Paul Quincey David Butterfield David Green Mhairi Coyle J. Neil Cape 《Atmospheric environment (Oxford, England : 1994)》2009,43(32):5085-5091
The carbonaceous components of Particulate Matter samples form a substantial fraction of their total mass, but their quantification depends strongly on the instruments and methods used. United Kingdom monitoring networks have provided many relevant data sets that are already in the public domain. Specifically, hourly organic carbon (OC) and elemental carbon (EC) were determined at four sites between 2003 and 2007 using Rupprecht and Pattashnik (R & P) 5400 automatic instruments. Since 2007, daily OC/EC measurements have been made by manual thermo-optical analysis of filter samples using a Sunset Laboratory Carbon Aerosol Analysis instrument. In parallel, long term daily measurements of Black Smoke, a quantity directly linked to black carbon (measured by aethalometers) and indirectly related to elemental carbon, have been made at many sites. The measurement issues associated with these techniques are evaluated in the context of UK measurements, making use of several sets of parallel data, with the aim of aiding the interpretation of network results. From the results available, the main conclusions are that the R & P 5400 instruments greatly under-read EC and total carbon (TC = OC + EC) at kerbside sites, probably due to the fact that the smaller particles are not sampled by the instrument; the R & P 5400 instrument is inherently difficult to characterise, so that all quantitative results need to be treated with caution; both aethalometer and Black Smoke (converted to black carbon) measurements can show reasonable agreement with elemental carbon results; and manual thermo-optical OC/EC results may under-read EC (and hence over-read OC), whether either transmittance or reflectance is used for the pyrolysis correction, and this effect is significant at rural sites. 相似文献
783.
784.
Tong Cao Min Wang Yinghao Yu Shuiliang Guo Yan Liu Yang Cao 《Environmental pollution (Barking, Essex : 1987)》2009,157(4):1270-1278
In order to better understand the spatial and temporal distribution pattern of metals and sulfur present in Shanghai, moss bags with Haplocladium microphyllum (Hedw.) Broth. were suspended at 14 local monitoring stations from April through June 2006 in Shanghai, the largest city in China. The results showed that the concentrations of S, Cu, Pb, and Zn in the moss bags after exposure were higher at the sites in the industrial district and most urban districts and lower at the sites in suburban areas, and well correlated with SO2 API and PM10 API in the air both in terms of space and time. The present study provided evidence that the moss H. microphyllum is suitable for bio-monitoring air pollution with moss bags and further confirmed that the moss-bag method is a simple, inexpensive and useful technique. 相似文献
785.
G.T. Geertsema B.G.J. Wichers Schreur 《Atmospheric environment (Oxford, England : 1994)》2009,43(32):4924-4934
The predictive potential of air quality models and thus their value in emergency management and public health support are critically dependent on the quality of their meteorological inputs. The atmospheric flow is the primary cause of the dispersion of airborne substances. The scavenging of pollutants by cloud particles and precipitation is an important sink of atmospheric pollution and subsequently determines the spatial distribution of the deposition of pollutants. The long-standing problem of the spin-up of clouds and precipitation in numerical weather prediction models limits the accuracy of the prediction of short-range dispersion and deposition from local sources. The resulting errors in the atmospheric concentration of pollutants also affect the initial conditions for the calculation of the long-range transport of these pollutants. Customary the spin-up problem is avoided by only using NWP (Numerical Weather Prediction) forecasts with a lead time greater than the spin-up time of the model. Due to the increase of uncertainty with forecast range this reduces the quality of the associated forecasts of the atmospheric flow.In this article recent improvements through diabatic initialization in the spin-up of large-scale precipitation in the Hirlam NWP model are discussed. In a synthetic example using a puff dispersion model the effect is demonstrated of these improvements on the deposition and dispersion of pollutants with a high scavenging coefficient, such as sulphur, and a low scavenging coefficient, such as cesium-137. The analysis presented in this article leads to the conclusion that, at least for situations where large-scale precipitation dominates, the improved model has a limited spin-up so that its full forecast range can be used. The implication for dispersion modeling is that the improved model is particularly useful for short-range forecasts and the calculation of local deposition. The sensitivity of the hydrological processes to proper initialization implies that the spin-up problem may reoccur with changes in the model and increased model resolution. Spin-up should be an ongoing concern for atmospheric modelers. 相似文献
786.
The sensitivity of modeled ozone to the temporal distribution of point, area, and mobile source emissions in the eastern United States 总被引:1,自引:0,他引:1
Patricia Castellanos Jeffrey W. Stehr Russell R. Dickerson Sheryl H. Ehrman 《Atmospheric environment (Oxford, England : 1994)》2009,43(30):4603-4611
Ozone remains one of the most recalcitrant air pollution problems in the US. Hourly emissions fields used in air quality models (AQMs) generally show less temporal variability than corresponding measurements from continuous emissions monitors (CEM) and field campaigns would imply. If emissions control scenarios to reduce emissions at peak ozone forming hours are to be assessed with AQMs, the effect of emissions' daily variability on modeled ozone must be understood. We analyzed the effects of altering all anthropogenic emissions' temporal distributions by source group on 2002 summer-long simulations of ozone using the Community Multiscale Air Quality Model (CMAQ) v4.5 and the Carbon Bond IV (CBIV) chemical mechanism with 12 km resolution. We find that when mobile source emissions were made constant over the course of a day, 8-h maximum ozone predictions changed by ±7 parts per billion by volume (ppbv) in many urban areas on days when ozone concentrations greater than 80 ppbv were simulated in the base case. Increasing the temporal variation of point sources resulted in ozone changes of +6 and −6 ppbv, but only for small areas near sources. Changing the daily cycle of mobile source emissions produces substantial changes in simulated ozone, especially in urban areas at night; results suggest that shifting the emissions of NOx from day to night, for example in electric powered vehicles recharged at night, could have beneficial impacts on air quality. 相似文献
787.
Evaluating the air quality impacts of the 2008 Beijing Olympic Games: On-road emission factors and black carbon profiles 总被引:3,自引:0,他引:3
Xing Wang Dane Westerdahl Lung Chi Chen Ye Wu Jiming Hao Xiaochuan Pan Xinbiao Guo K. Max Zhang 《Atmospheric environment (Oxford, England : 1994)》2009,43(30):4535-4543
The aggressive traffic interventions and emission control measures implemented to improve air quality during the 2008 Beijing Olympic Games created a valuable case study to evaluate the effectiveness of these measures on mitigating air pollution and protecting public health. In this paper, we report the results from our field campaign in summer 2008 on the on-road emission factors of carbon monoxide, black carbon (BC) and ultrafine particles (UFP) as well as the ambient BC concentrations. The fleet average emission factors for light-duty gasoline vehicles (LDGV) showed considerable reduction in the Olympic year (2008) compared to the pre-Olympic year (2007). Our measurement of Black Carbon (BC), a primary pollutant, at different elevations at the ambient site suggests consistent decrease in BC concentrations as the height increased near the ground level, which indicates that the nearby ground level sources, probably dominated by traffic, contributed to a large portion of BC concentrations in the lower atmospheric layer in Beijing during summertime. These observations indicate that people living in near ground levels experience higher exposures than those living in higher floors in Beijing. The BC diurnal patterns on days when traffic control were in place during the Olympic Games were compared to those on non-traffic-control days in both 2007 and in 2008. These patterns strongly suggest that diesel trucks are a major source of summertime BC in Beijing. The median BC concentration on Olympic days was 3.7 μg m−3, which was dramatically lower than the value on non-traffic-control days, indicating the effectiveness of traffic control regulations in BC reduction in Beijing. 相似文献
788.
Megan V. Brachtl Carlos Paez Perez Jorge Oviedo 《Environmental pollution (Barking, Essex : 1987)》2009,157(2):528-536
Motor vehicles are a major source of air pollution in Quito, Ecuador; however, little work has been done to characterize spatial and temporal variations in traffic-related pollutants, or to measure pollutants in vehicle emissions. We measured PAH continuously for one year at two residential sites in Quito, and PAH and traffic patterns for one week near a busy roadway. Morning rush-hour traffic and temperature inversions caused daily PAH maxima between 06:00 and 08:00. SO2, NOx, CO, and PM2.5 behaved similarly. At the residential sites PAH levels during inversions were 2-3-fold higher than during the afternoon, and 10-16-fold higher than 02:00-03:00 when levels were lowest. In contrast, at the near-roadway site, PAH concentrations were 3-6-fold higher than at the residential sites, and the effects of inversions were less pronounced. Cars and buses accounted for >95% of PAH at the near-roadway site. Near-roadway PAH concentrations were comparable to other polluted cities. 相似文献
789.
Ozone and urban forests in Italy 总被引:2,自引:0,他引:2
Paoletti E 《Environmental pollution (Barking, Essex : 1987)》2009,157(5):1506-1512
Ozone levels along urban-to-rural gradients in three Italian cities (Milan, Florence, Bari) showed that average AOT40 values at rural and suburban sites were 2.6 times higher than those determined at urban sites. However, O3 also exceeded the European criteria to protect forest health at urban sites, even when the standards for human health protection were met. For protecting street trees in Mediterranean cities, the objectives of measurement at urban sites should extend from the protection of human health to the protection of vegetation as well. A review of forest effects on O3 pollution and of O3 pollution on forest conditions in Italian cities showed that it was not possible to distinguish the effect of O3 in the complex mixture of urban pollutants and stressors. A preliminary list of tree species for urban planning in the Mediterranean area shows the average tree capacity of O3 removal and VOC emission. 相似文献
790.
Junxia Wang Maud Mercury Maurice Millet Michel Montury 《Environmental pollution (Barking, Essex : 1987)》2009,157(2):365-370
To estimate the atmospheric exposure of the greenhouse workers to pesticides, solid phase microextraction (SPME) was used under non-equilibrium conditions. Using Fick's law of diffusion, the concentrations of pesticides in the greenhouse can be calculated using pre-determined sampling rates (SRs). Thus the sampling rates (SRs) of two modes of SPME in the lab and in the field were determined and compared. The SRs for six pesticides in the lab were 20.4-48.3 mL min−1 for the exposed fiber and 0.166-0.929 mL min−1 for the retracted fiber. In field sampling, two pesticides, dichlorvos and cyprodinil were detected with exposed SPME. SR with exposed SPME for dichlorvos in the field (32.4 mL min-1) was consistent with that in the lab (34.5 mL min-1). SR for dichlorvos in the field (32.4 mL min−1) was consistent with that in the lab (34.5 mL min−1). The trends of temporal concentration and the inhalation exposure were also obtained. 相似文献