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991.
准确判断臭氧(O3)生成敏感性对O3污染成因分析和防控对策的制定至关重要.首次利用响应曲面方法设计最优试验方案,基于盒子模式模拟结果,快速量化O3对其前体物变化的响应.结果表明,CO对O3有正贡献,NOx和VOCs与O3呈现显著非线性关系,当φ(VOCs)与[φ(NOx)-13.75]比值大于4.17时,为NOx控制区,小于4.17时,为VOCs控制区;烯烃为影响O3生成的关键VOCs组分,当φ(烯烃)与[φ(NOx)-15]比值小于1.10且φ(烯烃)<35×10-9时,烯烃有利于O3的生成.响应曲面法在多因素和其交互作用对O3生成影响的研究中取得了良好效果,为高效判断O3敏感性提供了新的思路和方法. 相似文献
992.
目前基于排放清单估算的区域和城市尺度上的人为CO2排放不确定性较大.为了我国实现碳达峰和碳中和的目标,亟需对我国的区域尺度,特别是大城市群的人为CO2排放进行准确估算.分别利用两种先验人为CO2排放数据(EDGAR v6.0清单和EDGAR v6.0联合GCG v1.0的改进清单)作为输入数据,采用WRF-STILT大气传输模型模拟长三角地区2017年12月至2018年2月大气CO2摩尔分数,再以安徽全椒高塔观测的大气CO2摩尔分数作为参考值,通过贝叶斯反演方法得到的比例因子改进了模拟结果,并实现了长三角人为CO2排放通量的估算.结果表明:(1)在冬季,相对于基于EDGAR v6.0模拟的大气CO2摩尔分数值而言,基于改进清单模拟的大气CO2摩尔分数与观测值更为一致;(2)模拟的大气CO2摩尔分数在夜间高于观测值,白天则相反,主要因为排放清单的CO2排放数据不能表征人为... 相似文献
993.
In this paper, the dynamic relationship between global surface temperature (global warming) and global carbon dioxide emission (CO2) is modelled and analyzed by causality and spectral analysis in the time domain and frequency domain, respectively. Historical data of global CO2emission and global surface temperature anomalies over 129 years from 1860–1988 are used in this study. The causal relationship between the two phenomena is first examined using the Sim and Granger causality test in the time domain after the data series are filtered by ARIMA models. The Granger causal relationship is further scrutinized and confirmed by cross-spectral and multichannel spectral analysis in the frequency domain. The evidence found from both analyses proves that there is a positive causal relationship between the two variables. The time domain analysis suggests that Granger causality exists between global surface temperature and global CO2emission. Further, CO2emission causes the change in temperature. The conclusions are further confirmed by the frequency domain analysis, which indicates that the increase in CO2emission causes climate warming because a high coherence exists between the two variables. Furthermore, it is proved that climate changes happen after an increase in CO2emission, which confirms that the increase in CO2emission does cause global warming. 相似文献
994.
995.
EDTA直接滴定测定镍 总被引:1,自引:0,他引:1
参考磷酸在345~356℃时有强腐蚀性的特点,采有硫磷混合酸消解矿样,能使样品消解完全。本方法经加标校核证明,检测结果重现性好,准确度高。 相似文献
996.
997.
998.
E. Pipiras C. Dupont S. Chantot-Bastaraud J. P. Siffroi M. Bucourt A. Batallan C. Largillière M. Uzan J. P. Wolf B. Benzacken 《黑龙江环境通报》2004,24(2):101-103
True structural chromosomal mosaicism are rare events in prenatal cytogenetics practice and may lead to diagnostic and prognostic problems. Here is described the case of a fetus carrying an abnormal chromosome 15 made of a whole chromosome 2p translocated on its short arm in 10% of the cells, in association with a normal cell line. The fetal karyotype was 46,XX,add(15)(p10).ish t(2;15)(p10;q10)(WCP2+)[3]/46,XX[27]. Pregnancy was terminated and fetus examination revealed a growth retardation associated with a dysmorphism including dolichocephaly, hypertelorism, high forehead, low-set ears with prominent anthelix and a small nose, which were characteristic of partial trisomy 2p. Possible aetiologies for prenatal mosaicism involving a chromosomal structural abnormality are discussed. Copyright © 2004 John Wiley & Sons, Ltd. 相似文献
999.
Brian L. Altland Danielle Cox Robert M. Enick Eric J. Beckman 《Resources, Conservation and Recycling》1995,15(3-4)
High-pressure, near-critical liquids were used as float-sink separation media for the microsortation of polyolefin mixtures and PET/PVC mixtures. Near-critical carbon dioxide was used for the refinement of the polyolefins, and sulfur hexafluoride was used to separate post-consumer PVC from PET. Preliminary experiments indicated that there was no overlap in the density ranges of post-consumer HDPE, LDPE and PP containers. There was no overlap in the PET and PVC densities, with the exception of a single PVC packaging material with a density in the PET range. These initial results indicated that a float-sink separation was a viable means of microsortation. Separations of 91% LDPE (1/8′ beads)/9% PP (1/8′ chopped strands) resin mixtures and mixed post-consumer polyolefin flakes were then conducted in a laboratory-scale, 1-I batch apparatus. This apparatus not only permitted the observation of the separation, but also enabled the separated fractions to be removed from the high-pressure environment. The results indicated that LDPE purity of greater than 98.9% was obtained in 3 min or less if (a) the fluid density was 0.018 g/cm3 greater than the PP density and only 0.002 g/cm3 less than the LDPE density, thereby providing the greatest buoyancy force for the removal of the PP, (b) the fluid was recirculated upward through the bed of mixed plastics, facilitating the upward movement of the PP, and (c) the loading was kept at levels below 40% by volume. HDPE purity of 99% was also attained with clean, dry, post-consumer mixed plastic flakes. The loadings for these separations were very low, however, due to the difficulty in agitating the mixed bed of plastics using fluid recirculation. An economic analysis of these microsortation processes indicated that the value of the sorted plastics relative to the mixed feed must increase by approx. $0.08/lb for the CO2-based separation and approx. $0.27/lb for the SF6-based separation to justify the implementation of these high-pressure processes. 相似文献
1000.
Michael M. Reddy Kotra V. Krishnamurty Eugene Shpirt G. Anders Carlson Leo Hetling 《Environment international》1982,7(5):315-323
Total and particulate metal concentrations, measured during intensive synoptic studies of the Genesee River, NY, correlated with suspended-sediment concentration and river discharge. Dissolved metal concentrations, on the other hand, showed little systematic variation over the length of the river. Metal and sediment fluxes for two elevated-discharged periods peaked at a midbasin sampling site. For most metals at most sampling sties particulate materials comprised over one-half of the total material. Comparison of particulate material metal concentrations, normalized to the measured suspended-sediment concentrations had with basinwide average values shows that sites having low suspended-sediment concentrations had high particulate material metal contents relative to the basin averages, while sites with high suspended-sediment concentration had low metal contents. These results are consistent with a metal transport mechanism in the Genesee River involving (1) a nearly constant dissolved component, (2) a fine acid-soluble component, and (3) a coarse component that is effectively a neutral diluent in the sediment. Chemical factors, such as sediment organic content, also appear to affect metal transport in the Genesee River. 相似文献