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1.
Influence of environmental factors on arsenic accumulation and biotransformation using the aquatic plant species Hydrilla verticillata 总被引:1,自引:0,他引:1
Hydrilla verticillata(waterthyme) has been successfully used for phytoremediation in arsenic(As) contaminated water.To evaluate the effects of environmental factors on phytoremediation,this study conducted a series of orthogonal design experiments to determine optimal conditions,including phosphorus(P),nitrogen(N),and arsenate(As(Ⅴ))concentrations and initial pH levels,for As accumulation and biotransformation using this aquatic plant species,while also analyzing As species transformation in culture media after 96-hr exposure.Analysis of variance and the signal-to-noise ratio were used to identify both the effects of these environmental factors and their optimal conditions for this purpose.Results indicated that both N and P significantly impacted accumulation,and N was essential in As species transformation.High N and intermediate P levels were critical to As accumulation and biotransformation by H.verticillata,while high N and low P levels were beneficial to As species transformation in culture media.The highest total arsenic accumulation was(197.2±17.4) μg/g dry weight when As(V) was at level 3(375μg/L),N at level 2(4 mg/L),P at level 1(0.02 mg/L),and pH at level 2(7).Although H.verticillata is highly efficient in removing As(Ⅴ) from aquatic environments,its use could be potentially harmful to both humans and the natural environment due to its release of highly toxic arsenite.For cost-effective and ecofriendly phytoremediation of As-contaminated water,both N and P are helpful in regulating As accumulation and transformation in plants. 相似文献
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Juan Huang Jun Xiao Yang Guo Wenzu Guan Chong Cao Chunni Yan Mingyu Wang 《环境科学学报(英文版)》2020,32(1):319-330
Silver nanoparticles(AgNPs) have been widely used in many fields,which raised concerns about potential threats to biological sewage treatment systems.In this study,the phosphorus removal performance,enzymatic activity and microbial population dynamics in constructed wetlands(CWs) were evaluated under a long-term exposure to Ag NPs(0,50,and 200 μg/L) for 450 days.Results have shown that Ag NPs inhibited the phosphorus removal efficiency in a short-term exposure,whereas caused no obviously negative effects from a long-term perspective.Moreover,in the coexisting CW system of Ag NPs and phosphorus,competition exhibited in the initial exposure phase,however,cooperation between them was observed in later phase.Enzymatic activity of acid-phosphatase at the moderate temperature(10–20°C) was visibly higher than that at the high temperature(20–30℃) and CWs with Ag NPs addition had no appreciable differences compared with the control.High-throughput sequencing results indicated that the microbial richness,diversity and composition of CWs were distinctly affected with the extension of exposure time at different Ag NPs levels.However,the phosphorus removal performance of CWs did not decline with the decrease of polyphosphate accumulating organisms(PAOs),which also confirmed that adsorption precipitation was the main way of phosphorus removal in CWs.The study suggested that Ag NPs and phosphorus could be removed synergistically in the coexistence system.This work has some reference for evaluating the influences of Ag NPs on the phosphorus removal and the interrelation between them in CWs. 相似文献
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水量衡算条件下人工湿地对有机物的去除研究 总被引:1,自引:0,他引:1
构建了芦苇和无植物2种人工湿地,在系统水量衡算的基础上比较了2种湿地对生活污水中有机物的去除效果。结果证明,在植物收割后的冬季,芦苇湿地对有机物的去除率低于无植物湿地系统约2%;在其他季节,芦苇湿地对污水CODcr的去除率比无植物湿地高出3.3%-5%。但对BOD5的去除率却比无植物湿地低了1.9%-2.7%。因此,芦苇湿地对有机物的去除效果比无植物湿地高,但提高不多。比较了2种系统的氧化还原电位,芦苇湿地比无植物湿地的高(P〈0.05),这种提高主要集中在湿地水面以下约10cm的深度;从整个湿地床体来看。2块连续运行的潜流水平湿地内部氧化还原状态大部分相同。主要是厌氧状态。比较了2种人工湿地基质中降解有机物的细菌,放线菌和真菌的数量,二者没有明显的差别。考察了湿地进水有机负荷与去除量的关系,二者呈现显著的线性相关性(R^2〉0.99)。 相似文献
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本试验以HAc作为厌氧释磷的碳源有机物,以SBR系统外循环污泥作为研究对象,探索外循环活性污泥的厌氧释磷能力和获取高浓度富磷污水的途径,试验表明:厌氧过程中聚磷菌吸收HAc和释放PO4^3 的分子比为1:1。即吸收2.06mgHAc-COD将诱导1mgP释放,单位时段比污泥的平均释磷速率Vp=6.54.t^0.76,理想的厌氧时间为60-180min,减少循环污泥释磷系统的反应容积可以提高富磷污水磷酸盐的浓度。 相似文献
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反硝化聚磷一体化设备生产性实验研究 总被引:4,自引:0,他引:4
反硝化聚磷一体化设备主要特点是在利用含反硝化聚磷菌的活性污泥在缺氧状态过量聚磷,在完成磷去除的同时进行反硝化。通过实验得出缺氧释磷在前30min内大量释放,60min以后甚微;反硝化吸磷在最初10几分钟内速率极大;吸磷与反硝化紧密相关;聚磷菌在释、聚磷时利用一定量的有机物。 相似文献
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Yongfeng Ji Zidan Yuan Guoqing Zhang Xing Wu Xu M Jinru Lin Shaofeng Wang 《环境科学学报(英文版)》2023,35(2):31-41
An advanced cost-saving method of removal of high-As(Ⅲ) from SO4(-Ⅱ)-rich metallurgi cal wastewater has been developed by diluting the SO4(-Ⅱ) content with As(Ⅲ)-Cl(-Ⅰ)-rich metallurgical wastewater and then by the direct precipitation of As(Ⅲ) with Fe(Ⅲ) at pH2.3.As(Ⅲ) removal at various SO4(-Ⅱ)/Cl(-Ⅰ) molar ratios and temperatures was investigated The results showed that 65.2–98.2%of As(III) immobilization into solids occurred at the SO4(Ⅱ)/Cl(-Ⅰ) mo... 相似文献