全文获取类型
收费全文 | 516篇 |
免费 | 4篇 |
国内免费 | 82篇 |
专业分类
安全科学 | 7篇 |
废物处理 | 7篇 |
环保管理 | 79篇 |
综合类 | 288篇 |
基础理论 | 65篇 |
污染及防治 | 124篇 |
评价与监测 | 28篇 |
社会与环境 | 4篇 |
出版年
2024年 | 1篇 |
2023年 | 13篇 |
2022年 | 11篇 |
2021年 | 17篇 |
2020年 | 16篇 |
2019年 | 11篇 |
2018年 | 12篇 |
2017年 | 15篇 |
2016年 | 18篇 |
2015年 | 25篇 |
2014年 | 27篇 |
2013年 | 31篇 |
2012年 | 22篇 |
2011年 | 58篇 |
2010年 | 27篇 |
2009年 | 35篇 |
2008年 | 39篇 |
2007年 | 33篇 |
2006年 | 33篇 |
2005年 | 15篇 |
2004年 | 13篇 |
2003年 | 23篇 |
2002年 | 21篇 |
2001年 | 15篇 |
2000年 | 8篇 |
1999年 | 12篇 |
1998年 | 5篇 |
1997年 | 8篇 |
1996年 | 4篇 |
1995年 | 6篇 |
1994年 | 5篇 |
1993年 | 4篇 |
1992年 | 7篇 |
1991年 | 3篇 |
1989年 | 2篇 |
1988年 | 1篇 |
1985年 | 1篇 |
1984年 | 2篇 |
1982年 | 1篇 |
1979年 | 1篇 |
1974年 | 1篇 |
排序方式: 共有602条查询结果,搜索用时 15 毫秒
61.
Shujuan Zhang Li Wang Fang M Xue Zhang Zhe Li Shiyang Li Xiaofeng Jiang 《环境科学学报(英文版)》2015,27(7):211-218
Our study sought to assess how much phosphorus (P) runoff from paddy fields could be cut down by fertilizer management and inoculation with arbuscular mycorrhizal fungi. A field experiment was conducted in Lalin River basin, in the northeast China: six nitrogen–phosphorus–potassium fertilizer levels were provided (0, 20%, 40%, 60%, 80%, and 100% of the recommended fertilizer supply), with or without inoculation with Glomus mosseae. The volume and concentrations of particle P (PP) and dissolved P (DP) were measured for each runoff during the rice growing season. It was found that the seasonal P runoff, including DP and PP, under the local fertilization was 3.7 kg/ha, with PP, rather than DP, being the main form of P in runoff water. Additionally, the seasonal P runoff dropped only by 8.9% when fertilization decreased by 20%; rice yields decreased with declining fertilization. We also found that inoculation increased rice yields and decreased P runoff at each fertilizer level and these effects were lower under higher fertilization. Conclusively, while rice yields were guaranteed arbuscular mycorrhizal inoculation and fertilizer management would play a key role in reducing P runoff from paddy fields. 相似文献
62.
In order to find effective measures to control diatom blooms, a better understanding of the physiological characteristics of nutrient uptake in diatoms is needed. A study of P and Si-uptake kinetics for diatom species from two light regimes was conducted at low (LL), moderate (ML) and high light intensities (HL) (2, 25 and 80 μmol photons/(m2·sec)), respectively. The results showed that P uptake of diatoms was heavily influenced by historic light regimes. P affinity changed with growth and photosynthetic activity. The lowest half saturation constant for P uptake (Km(P)) was under HL for high-light adapted diatoms while the lowest half-saturation constant for low-light adapted diatoms was observed under LL. The Si half-saturation constant (Km(Si)) increased with increasing light intensities for pennate diatoms but decreased for centric diatoms. Diatom volumes were correlated with the maximum Si uptake rates (Vm(Si)) at HL and Km(Si) at ML and HL for six diatom species. Our results imply that when we assess the development of diatom blooms we should consider light intensity and cell volume in addition to ambient Si or P concentration. The relationship between light intensity and P-uptake suggests that we can find suitable methods to control diatom blooms on the basis of reducing phytoplankton activity of P-uptake and photosynthesis simultaneously. 相似文献
63.
Nanoparticles in wastewater from a science-based industrial park - coagulation using polyaluminum chloride 总被引:1,自引:0,他引:1
The Hsinchu Science-based Industrial Park (HSIP) is the hi-tech manufacturing hub of Taiwan. Wastewater from the HSIP contains numerous nano-sized silicate particles whose size distributions peak at 2 and 90 nm. A 3-5 mg l(-1) as Al dose of polyaluminum chloride (PACl) was used in the field to coagulate these particles, but the removal efficiency was low. Laboratory scale tests indicated that although PACl coagulation removed 52% of the turbidity and 48% of the chemical oxygen demand (COD) from water, its effect on nano-particle removal was minimal. About 58% of the soluble COD was associated with colloidal Si particles. A light scattering test and transmission electron microscopy (TEM) demonstrated that the nano-particles agglomerated in approximately linear aggregates of sizes 100-300 nm. Prolonged contact between residual PACl and the nano-particles generated large aggregates with sizes of up to 10 microm and a fractal dimension of 2.24-2.63. The results presented herein should be of interest in the processing of "high-tech" wastewater that contains nanosized silica particles. 相似文献
64.
The rapid increase of phosphorus (P) use in farming has raised concerns regarding its conservation and environmental impact. Increasing the P use efficiency (PUE) is an approach to mitigating these adverse impacts. In this study, we applied substance flow analysis (SFA) to establish a life-cycle P use efficiency model to determine the life-cycle PUE of the farming system used in Anhui Province in 2011, which is typical of the agriculture practiced in central China. Based on this model, the P flows and PUEs of five subsystems were identified and quantified: crop farming, crop processing, livestock breeding, rural living, and urban living. The three largest P flows were found in the crop farming and livestock breeding subsystems; it can therefore be concluded that these subsystems have substantial impacts on the entire farming system. In contrast, the PUEs of crop farming, rural consumption, and livestock breeding subsystems presented the three lowest PUEs (58.79%, 71.75%, and 76.65%, respectively). These results were also consistent with the finding that the greatest P losses occurred in crop farming and livestock breeding. Consequently, the study proposes that great potential exists for increasing PUEs in the farming system of Anhui, and several of the most promising measures could be combined for improving PUEs. Finally, the study assesses data quality and presents a sensitivity analysis for use in interpreting the results. The study also shows that improving PUE and decreasing P losses in farming systems through improved nutrient management must be considered an important issue, and this study represents valuable experience in resource conservation and agricultural development in China. 相似文献
65.
Jose Oliva Paula Payá Miguel Ángel Cámara Alberto Barba 《Journal of environmental science and health. Part. B》2013,48(7):775-781
The effects of six clarification agents [egg albumin, blood albumin, bentonite + gelatine, charcoal, polyvinylpolypyrrolidine (PVPP) and silica gel] on the removal of residues of three fungicides (famoxadone, fluquinconazole and trifloxystrobin) applied directly to a racked red wine, elaborated from Monastrell variety grapes from the D.O. Region of Jumilla (Murcia, Spain) were studied. The clarified wines were filtered with 0.45 μ m nylon filters to determine the influence of this winemaking process in the disappearance of fungicide residues. Analytical determination of fluquinconazole and trifloxystrobin was performed by gas chromatography with electron captor detector (ECD), while that of famoxadone using an HPLC equipped with a diode array detector (DAD). Generally, trifloxystrobin is the fungicide that is the lowest persistent one in wines, except in the egg albumin study whereas, the most persistent one is fluquinconazole. The elimination depends on the nature of the active ingredient, though the water stability in the presence of light within it has more influence than the solubility and polarity of the product itself. The most effective clarifying agents were the charcoal and PVPP. The silica gel and bentonite plus gelatine were not enough to reduce considerably the residual contents in the wine clarified with them. In general terms, filtration is not an effective step in the elimination of wine residues. The greatest removal after filtration is obtained in wines clarified with egg albumine and bentonite plus gelatine, and the lowest in those clarified with PVPP. 相似文献
66.
The potential of commonly available green alga Ulva lactuca was investigated as viable biomaterials for removal of synthetic azo dye (Direct Yellow 12, DY-12) from aqueous solution. The results obtained from the batch experiments revealed that the ability of the U. lactuca to remove DY-12 from its aqueous solution was dependent on the dye concentration, pH, and algal biomass but less dependent on the particle size of the U. lactuca. The equilibrium conditions and kinetics of adsorption were investigated, and the adsorption kinetic was consistent with the pseudo-second-order model (R2=1). The adsorption isotherm followed only the Freundlich model with a correlation coefficient R2=0.99. This study demonstrated that the U. lactuca could be used as an effective biosorbent for the removal of DY-12 from its aqueous solution. 相似文献
67.
Xiaoya Liu Yu Hong Peirui Liu Jingjing Zhan Ran Yan 《Frontiers of Environmental Science & Engineering》2019,13(5):78
68.
69.
M. A. C. Veer 《Journal of Coastal Conservation》1997,3(1):41-48
The encroachment of some tall grass species in open dune vegetation, as observed in a Dutch dry dune area, is considered unfavourable
from a conservation viewpoint. This paper investigates differences in vegetation and soil properties between grass-dominated
and still existing open dune grassland plots at four locations along the coast. Soil properties studied include nitrogen and
phosphorus pools and nitrogen availability by mineralization. Vegetation properties included are above and below-ground biomass
and nitrogen and phosphorus concentrations in above-ground biomass.
Systematic differences in N-pools between grass-dominated and open dune grassland plots were not observed. However, N-availability
by mineralization and its turnover rates are higher in grass-dominated plots than in open dune grassland plots, as well as
above and below-ground biomass. In open dune grassland plots, atmospheric N-input is an important source of N, whereas in
grass-dominated plots mineralization largely exceeds atmospheric N-input. However, these observations do not explain the mosaic-like
vegetation pattern. Grazing intensity is most likely the determinant factor in the dry dune system. It is concluded, that
grass encroachment is probably triggered by atmospheric deposition and is enhanced by positive feedbacks in the N-cycle. The
relevance of these results for restoration management is briefly discussed. 相似文献
70.
Effect of low-molecular weight organic acids on phosphorus release and phytoavailabilty of phosphorus in phosphate rocks added to soils 总被引:2,自引:0,他引:2
Phosphorus (P) is critically needed to improve soil fertility in many parts of the world. The use of water-soluble P fertilizers, e.g., single super-phosphate and triple super-phosphate in developing countries to improve crop production has been limited primarily by their high cost. The presence of indigenous phosphate deposits in some countries provides an incentive for direct application or local chemical treatment at low cost to improve the solubility of low reactive phosphate rocks (PRs). The use of naturally occurring low-molecular weight organic acids (LMWOAs) that are produced in soil as microbial metabolites or plant exudates from dead or living cells represents a new perspective in PR research. The LMWOAs contain various functional groups that may play a significant role in PR dissolution. Little information is available, however, about the potential of LMWOAs in releasing P from PRs. This study reports P release from 12 PRs, four each of low, medium, and high reactivity, obtained from various deposits (Kodjari, Tahoua, North Carolina, Gafsa, Khouribga, Tilemsi Valley, Central Florida, Sechura, Minjingu, North Florida, Hahotoe, and Parc W) using nine LMWOAs containing mono-, di-, and tri-carboxylic groups and a mineral acid (H2SO4). Laboratory studies showed that the organic acids are effective in releasing P from low and medium reactive PRs, but very ineffective in releasing P from high reactive PRs. The average amounts of P released by all the organic acids from the three types of PRs were 65.5 mmol kg−1 PR from the low reactive PRs, 55.1 mmol kg−1 from the medium, and 11.1 mmol kg−1 from the high; those released from across all the PRs were 21.9 by the mono-carboxylic acid group, 54.2 by the di-carboxylic acid group, and 57.0 mmol P kg−1 by the tri-carboxylic acid group. The P released was negatively correlated with the equilibrium pH, but positively correlated with Ca released from the PRs. Laboratory incubation studies on the release of P from PRs added to soils with or without organic acids and incubated at 25 °C for 15, 30, and 45 days showed that the percentage of plant-available P released varied considerably from 0.95 in the Kodjari PR to 40.1% in the North Carolina PR and was related to PR reactivity. A greenhouse study with corn (Zea mays L.) grown for 60 days on soils treated with PRs or with PRs mixed with organic acids showed that corn response to addition of oxalic or citric acid varied with P rates and PR sources, suggesting that organic acids have potential as amendments for increasing plant-available P in PR-treated soils. 相似文献