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291.
中三角区域已经是我国第四个国家级城市群,也将成为我国经济增长的"第四极"。在经济发展的同时,更需要以节能减排、资源环境等为重点,以实现经济建设与生态文明"双可持续"的协同发展。本文以二氧化硫、氮氧化物、烟(粉)尘为主要大气污染物,对我国中三角区域大气污染物排放进行了详细的分析,并与京津冀、长三角、珠三角、"三区十群"等进行了多方位比较。结果表明,2013年中三角区域二氧化硫排放量为151.7万t,其中工业二氧化硫排放量为140.1万t;氮氧化物排放量为147.2万t,其中工业氮氧化物排放量为93.6万t;烟(粉)尘排放量为81.8万t,其中工业烟(粉)尘排放量为71.4万t。中三角区域二氧化硫、氮氧化物、烟(粉)尘排放量均位于"四极"的第三。中三角区域二氧化硫、氮氧化物、烟(粉)尘单位GDP排放强度分别为25.03t/亿元、24.29 t/亿元、13.50 t/亿元,分别位于"四极"的第一、第二、第二。同时,本文还从经济发展模式、产业结构调整、煤炭消费方式等方面对我国中三角等经济"四极"提出了相关建议。 相似文献
292.
Jussi Kosonen Leif Kronberg 《Environmental science and pollution research international》2009,16(5):555-564
Background, aim and scope Each year, large quantities of pharmaceuticals are consumed worldwide for the treatment and prevention of human and animal
diseases. Although the drugs and the metabolites observed in the wastewaters and in the environment are present at concentrations
several orders of magnitude lower than the concentrations required to exert their effects in humans or animals, their long-term
impact on the environment is commonly not known. In this study, the occurrence of six antihistamines, which are used for the
relief of allergic reactions such as hay fever, was determined in sewage treatment plants wastewaters and in recipient river
waters.
Materials and methods The occurrence of the antihistamines cetirizine, acrivastine, fexofenadine, loratadine, desloratadine and ebastine in sewage
treatment plants wastewaters and in recipient river waters was studied. The analytical procedure consisted of solid-phase
extraction of the water samples followed by liquid chromatography separation and detection by a triple-quadrupole mass spectrometer
in the multiple reaction mode.
Results Cetirizine, acrivastine and fexofenadine were detected in both influent and effluent wastewater samples at concentration levels
ranging from about 80 to 220 ng/L, while loratadine, desloratadine and ebastine could not be detected in any samples. During
sewage treatment, the concentration of the antihistamines dropped by an average of 16–36%. Furthermore, elevated concentrations
of antihistamines were observed in samples collected during the season of most intensive plant pollen production, i.e. in
May. In the river water samples, the relative pattern of occurrence of cetirizine, acrivastine and fexofenadine was similar
to that in the wastewater samples; although the concentration of the compounds was substantially lower (4–11 ng/L). The highest
concentrations of the studied drugs were observed near the discharging point of the sewage treatment plant.
Discussion The highest concentrations of antihistamines in STP wastewaters correlate with the outbreak of allergic reaction caused by
high amounts of plant pollens in the air. The analysis results of the river water samples show that the antihistamines are
carried far away from the effluent discharge points. They may account for a part of the mix of pharmaceuticals and of pharmaceutical
metabolites that occur downstream of STPs.
Conclusions Antihistamines are poorly degraded/eliminated under the biological treatment processes applied in the wastewater treatment
plants and, consequently, they are continuously being discharged along with other drugs to the aquatic environment.
Recommendations and perspectives As a huge quantity and variety of drugs and their metabolites are continuously discharged to rivers and the sea, the compounds
should be considered as contaminants that may possess risks to the aquatic ecosystem. Further studies are urgently needed
on the environmental fate of the antihistamines and other pharmaceuticals in the aquatic environment. These studies should
be concerned with the stability of the compounds, their transformation reactions and the identity of the transformation products,
the distribution of drugs and their uptake and effects in organisms. On the basis of these studies, the possible environmental
hazards of pharmaceuticals may be assessed. 相似文献
293.
A decision framework for possible remediation of contaminated sediments in the River Kymijoki, Finland 总被引:1,自引:1,他引:0
Verta M Kiviranta H Salo S Malve O Korhonen M Verkasalo PK Ruokojärvi P Rossi E Hanski A Päätalo K Vartiainen T 《Environmental science and pollution research international》2009,16(1):95-105
Background, aim, and scope The paper describes the spatial contamination of the River Kymijoki, South-Eastern Finland, and the coastal region of the
Gulf of Finland with PCDD/Fs and mercury. The findings of ecotoxicologial and human health studies are also reported, including
environmental and human risk assessments. Sediments from the River Kymijoki, draining into the Gulf of Finland, have been
heavily polluted by the pulp and paper industry and by chemical industries. A wood preservative, known as Ky-5, was manufactured
in the upper reaches of the river between 1940 and 1984 causing severe pollution of river sediments with polychlorinated dibenzo-p-dioxins (PCDD) and dibenzofurans (PCDF). Moreover, the sediments have been polluted with mercury (Hg) from chlor-alkali production
and the use of Hg as a slimicide in pulp and paper manufacturing.
Materials and methods An extensive sediment survey was conducted as well as sediment transport modeling, toxicity screening of sediment invertebrates,
and a survey of contaminant bioaccumulation in invertebrates and fish. Studies on human exposure to PCDD/Fs and the possible
effects on hypermineralization of teeth as well as an epidemiological study to reveal increased cancer risk were also conducted.
An assessment of the ecological and human health risks with a null hypothesis (no remediation) was undertaken.
Results The sediment survey revealed severe contamination of river and coastal sediments with PCDD/Fs and Hg. The total volume of
contaminated sediments was estimated to reach 5 × 106 m3 and hot spots with extremely high concentrations (max 292,000 ng g−1 or 1,060 ng I-TEQ g−1 d.w.) were located immediately downstream from the pollution source (approximately 90,000 m3). Sediment contamination was accompanied by changes in benthic assemblages, but direct effects were masked by many factors.
The fish showed only slightly elevated PCDD/F levels in muscle, but orders of magnitude higher in the liver compared with
reference freshwater sites and the Baltic Sea. The concentrations in human fat did not reveal high human exposure in the Kymijoki
area in general and was lower than in sea fishermen. The relative risk for total cancer among farmers was marginally higher
(RR = 1.13) among those living close to the river, compared with farmers living further away, and the possibility of increased
cancer risk cannot be ruled out. A conservative risk assessment revealed that the present probability of exceeding the WHO
upper exposure limit of 4 pg WHO-TEQ kg−1 d−1 for PCDD/Fs and DL-PCBs was 6%. The probability of exceeding the WHO limit value of 0.23 μg kg−1 d−1 for methyl mercury was estimated to be notably higher at 62%. Based on these studies and the estimated risks connected with
different remediation techniques a general remediation plan with cost benefit analysis was generated for several sub-regions
in the river. Dredging, on-site treatment, and a close disposal of the most contaminated sediments (90,000 m3) was suggested as the first phase of the remediation. The decision regarding the start of remediation will be made during
autumn 2008.
Conclusions The sediments in the River Kymijoki are heavily polluted with PCDD/Fs and mercury from earlier chlorophenol, chlor-alkali,
and pulp and paper manufacturing. A continuous transport of contaminants is taking place to the Gulf of Finland in the Baltic
Sea. The highly increased PCDD/F and Hg levels in river sediments pose an ecotoxicological risk to benthic fauna, to fish-eating
predators and probably to human health. The risks posed by mercury exceed those from PCDD/Fs and need to be evaluated for
(former) chlor-alkali sites and other mercury releasing industries as one basis for remediation decision making.
Recommendations and perspectives The studies form the basis of a risk management strategy and a plan for possible remediation of contaminated sediments currently
under consideration in the Southeast Finland Regional Environment Centre. It is recommended that a detailed restoration plan
for the most seriously contaminated areas should be undertaken. Based on current knowledge, the restoration of the whole river
is not feasible, considering the current risk caused by the contaminated sediment in the river and the costs of an extensive
restoration project. The experiences gained in the present case should be utilized in the evaluation of PCDD/F- and mercury-contaminated
sites in other countries. The case demonstrates that the historic reservoirs are of contemporary relevance and should be addressed,
e.g., in the national implementation plans of the Stockholm Convention.
Electronic supplementary material The online version of this article (doi:) contains supplementary material, which is available to authorized users. 相似文献
294.
Ying Guo Huan-Yun Yu Eddy Y. Zeng 《Environmental pollution (Barking, Essex : 1987)》2009,157(6):1753-1763
This review summarizes and analyzes available data in the literature (mostly after 2000) on the occurrence of dichlorodiphenyltrichloroethane (DDT) and its main metabolites, dichlorodiphenyldichloroethane (DDD) and chlorodiphenyldichloroethylene (DDE), in the environment of the Pearl River Delta (PRD), South China. Generally, the concentration levels of the sum of DDT, DDD, and DDE, designated as DDTs thereafter, have not significantly declined since 1983. However, the composition of DDTs residues has changed with time. DDTs in soil, freshwater sediment and freshwater fish species were mainly residues from chronological use. There is evidence that new point sources, such as dicofol and anti-fouling paint, may have contributed DDTs to various environmental compartments. Risk assessment against existing criteria indicated that the levels of DDTs in water and some fish species may pose adverse effects to humans or wildlife, and those in sediment/soil may also cause negative impacts to the eco-environment of the PRD. 相似文献
295.
River channel network design for drought and flood control: A case study of Xiaoqinghe River basin, Jinan City, China 总被引:2,自引:0,他引:2
Baoshan Cui Chongfang Wang Wendong Tao Zheyuan You 《Journal of environmental management》2009,90(11):3675-3686
Vulnerability of river channels to urbanization has been lessened by the extensive construction of artificial water control improvements. The challenge, however, is that traditional engineering practices on isolated parts of a river may disturb the hydrologic continuity and interrupt the natural state of ecosystems. Taking the Xiaoqinghe River basin as a whole, we developed a river channel network design to mitigate river risks while sustaining the river in a state as natural as possible. The river channel risk from drought during low-flow periods and flood during high-flow periods as well as the potential for water diversion were articulated in detail. On the basis of the above investigation, a network with “nodes” and “edges” could be designed to relieve drought hazard and flood risk respectively. Subsequently, the shortest path algorithm in the graph theory was applied to optimize the low-flow network by searching for the shortest path. The effectiveness assessment was then performed for the low-flow and high-flow networks, respectively. For the former, the network connectedness was evaluated by calculating the “gamma index of connectivity” and “alpha index of circuitry”; for the latter, the ratio of flood-control capacity to projected flood level was devised and calculated. Results show that the design boosted network connectivity and circuitry during the low-flow periods, indicating a more fluent flow pathway, and reduced the flood risk during the high-flow periods. 相似文献
296.
Three geomorphic considerations that underpin the design and implementation of realistic and strategic river conservation
and rehabilitation programs that work with the nature are outlined. First, the importance of appreciating the inherent diversity
of river forms and processes is discussed. Second, river dynamics are appraised, framing the contemporary behavioral regime
of a reach in relation to system evolution to explain changes to river character and behavior over time. Third, the trajectory
of a reach is framed in relation to downstream patterns of river types, analyzing landscape connectivity at the catchment
scale to interpret geomorphic river recovery potential. The application of these principles is demonstrated using extensive
catchment-scale analyses of geomorphic river responses to human disturbance in the Bega and Upper Hunter catchments in southeastern
Australia. Differing implications for reach- and catchment-scale rehabilitation planning prompt the imperative that management
practices work with nature rather than strive to ‘fight the site.’ 相似文献
297.
298.
Spatial distribution of 238U and 226Ra activities in sediment columns along the Krka River and estuary, were studied using gamma spectrometry. Markedly different 238U and 226Ra activities between riverine, estuarine and marine sediments were observed. Distribution of these radionuclides, as well as their anthropogenic and natural origin, was evaluated by activity measurements, taking into account sedimentation rates estimated by 137Cs distribution in sediment columns. 相似文献
299.
江苏省沿江开发区空间分工、制造业集聚与转移 总被引:3,自引:0,他引:3
基于新经济地理学相关理论,针对江苏省沿江开发战略实施以后,制造业空间可能存在的变动,在整理和分析调查问卷资料的基础上,选择专业化指数和基尼系数2种方法来定量分析江苏省21个沿江省级以上开发区空间分工、制造业集聚和转移态势。结果表明:(1)2002~2006年江南沿江开发区通过向江北沿江开发区转移部分传统产业,逐渐形成了江南沿江技术/资本密集型制造业“中心”和江北沿江劳动密集型制造业“外围”的空间分工格局;(2)江南沿江开发区内部、江北沿江开发区内部尚未形成良好的分工关系;(3)受开发区发展阶段、区域产业政策、本地化资源供给和市场需求等因素影响,并未发现理论预期的普遍存在的产业集聚现象,仅纺织服装、石化、电力、塑料橡胶等产业呈现集中趋势. 相似文献
300.
汉江堵河流域地表水质时空变化特征 总被引:4,自引:0,他引:4
对汉江堵河流域9个点位为期1年的地表水水质理化特性进行时空特征分析,应用〖WTBX〗t〖WTBZ〗检验进行水质季节性变化分析,聚类分析进行空间相似性分析以确定空间尺度的分类情况,判别分析识别显著性指标,并以此反映上述空间聚类分析结果的差异性。结果表明:①Cl-、总溶解性固体(TDS)及浊度(Turbidity) 3项指标没有表现出显著的时间差异性;②温度、pH、NO-3、TP表现为丰水季显著大于枯水季,而SO2-4、HCO-3、NH+4、 DO则表现出相反的变化趋势,即枯水季显著大于丰水季;③空间聚类分析将采样点分为4类;④判别分析体现出良好的指标降维能力,仅需4个指标(NO-3、TDS、SO2-4、HCO-3)即可反映整体水质的空间差异性。 相似文献