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311.
• PM2.5-related deaths were estimated to be 227 thousand in BTH & surrounding regions. • Local emissions contribute more to PM2.5-related deaths than PM2.5 concentration. • Local controls are underestimated if only considering its impacts on concentrations. • Rural residents suffer larger impacts of regional transport than urban residents. • Reducing regional transport benefits in mitigating environmental inequality. The source-receptor matrix of PM2.5 concentration from local and regional sources in the Beijing-Tianjin-Hebei (BTH) and surrounding provinces has been created in previous studies. However, because the spatial distribution of concentration does not necessarily match with that of the population, such concentration-based source-receptor matrix may not fully reflect the importance of pollutant control effectiveness in reducing the PM2.5-related health impacts. To demonstrate that, we study the source-receptor matrix of the PM2.5-related deaths instead, with inclusion of the spatial correlations between the concentrations and the population. The advanced source apportionment numerical model combined with the integrated exposure–response functions is used for BTH and surrounding regions in 2017. We observed that the relative contribution to PM2.5-related deaths of local emissions was 0.75% to 20.77% larger than that of PM2.5 concentrations. Such results address the importance of local emissions control for reducing health impacts of PM2.5 particularly for local residents. Contribution of regional transport to PM2.5-related deaths in rural area was 22% larger than that in urban area due to the spatial pattern of regional transport which was more related to the rural population. This resulted in an environmental inequality in the sense that people staying in rural area with access to less educational resources are subjected to higher impacts from regional transport as compared with their more resourceful and knowledgeable urban compatriots. An unexpected benefit from the multi-regional joint controls is suggested for its effectiveness in reducing the regional transport of PM2.5 pollution thus mitigating the associated environmental inequality.  相似文献   
312.
Fluorescence excitation-emission matrix spectroscopy (EEMs) combined with fluorescence regional integration (FRI) analysis was used to investigate the composition and transformation of humic acid (HA) and fulvic acid (FA) from landfill. The EEMs of HAs at different landfill ages were characterized by two typical fluorescence chromophores with Ex/Em pairs at Ex = 420-470 nm/Em = 490-530 nm and Ex = 345-375 nm/Em = 450-465 nm. EEMs of FA were featured by other two distinctly different fluorophores with Ex/Em pairs at Ex = 315-335 nm/Em = 420-440 nm and Ex = 255-275 nm/Em = 425-455 nm. The results show that HA extracted from the refuse disposed in the year of 1989 was formed by connecting small-condensed aromatic structures with protein-like chains. Compared with HA extracted from the refuse disposed in the year of 1992, HA extracted from the refuse of 1996 had a higher fluorescence intensity and lower r(B,A) (the ratio of the fluorescence intensities of peak B and peak A) value. It contained low molar mass components, low aromatic condensation degree, and more easily oxidized substituents. This indicates that the landfill time strongly affects the EEMs characteristics of HA, and that the humification degree of HA increases with the landfill time. A red shift to a longer wavelength region and an increase of fluorescence intensity were observed when the concentration of HA was increased, suggesting that concentration had a great influence on the fluorescence characteristics of HAs. pH (2-12) also had significant effects on the fluorescence intensity, although it exerted no effect on the peak position of fluorescence of HA and FA. The results of FRI show that increasing concentration lead to more interactions among various structure components and that small molecular weight units tend to aggregate or be masked into more complicated and larger structures. The pH influence on the fluorescence intensity of HA seems mainly through molecular configuration, while the fluorescence intensity change with pH may be due to various substituents of FA.  相似文献   
313.
在研究易燃、易爆、有毒的重大危险源和泄漏物扩散模型的基础上,建立了易燃、易爆、有毒物三维数值模拟程序,得到了复杂地形条件下关键点的有害物浓度历史和有害物的时空分布  相似文献   
314.
区域农业生态环境质量综合评价方法与模型研究   总被引:24,自引:0,他引:24  
为了客观准确的评价区域农业生态环境质量,引入灰色系统理论中的关联度分析法,提出了区域生态环境质量的多级模糊综合评价——灰色关联优势分析复合模型,并以安徽省芜湖市区域农业生态环境质量的综合评价为例,根据芜湖市区域农业生态环境调查与监测资料,进行了实例研究。结果表明:安徽省芜湖市区域农业生态环境已经受到了明显的污染,并且各区域污染水平具有一定的差异;芜湖市区域农业生态环境质量优劣的关联序依次为:南陵县、芜湖县、繁昌县和城市郊区。   相似文献   
315.
基于2015—2020年近地面NO2质量浓度数据和2019年哨兵-5P TROPOMI卫星探测的对流层NO2柱浓度数据,采用相关性分析、趋势分析等方法探究新疆天山北坡经济带6个城市NO2污染的时空分布特征。结果表明:(1)从年均值来看,天山北坡经济带NO2质量浓度总体呈下降趋势,尤其2018—2020年下降明显。其中乌鲁木齐NO2质量浓度值最高、博乐最低。(2)从季度均值和月均值来看,各城市NO2质量浓度季节变化明显,其中夏季最低、冬季最高;月均值呈“中间低、两头高”的变化特征。(3)从日均值来看,各城市NO2质量浓度大多呈现双峰型分布,分别出现在早上10:00和晚上23:00。(4)从空间分布来看,NO2柱浓度高值区多分布在人口密集和工业发达的城市地区,尤其是乌鲁木齐、昌吉、五家渠、石河子污染最为严重。  相似文献   
316.
应用统计分析方法,对湖南省湘潭市2001年城区环境噪声网格布点及其监测结果总体进行了区域环境噪声监测点的最优集合,并通过网格布点法与优化布点法对该市2002年和2003年环境噪声监测结果进行了对比检验,结果表明,两种方法监测的等效声级和标准差平均值均<1dB(A),监测结果之间无显著性差异。  相似文献   
317.
为探究沈阳地区重污染天气成因,文章利用地面、高空气象观测资料、风廓线雷达资料、NECP再分析资料以及大气污染物监测资料,对2019年3月1~6日沈阳地区出现的一次持续性重污染天气过程,探讨了大气污染物质量浓度、地面气象要素变化特征、大气环流配置与外来输送等特征.结果表明,均压场、地面风场弱及辐合、高温高湿是本次重污染天...  相似文献   
318.
王艳 《环境与发展》2020,(2):146-147
随着各地雾霾等大气污染问题反复出现,各种复杂的大气环境质量问题开始在全球集中呈现。大气污染物在环流扰动之下已经开始了长距离传输,不再是过去单纯的点源污染,而是表现出了蔓延速度更加迅速、污染更加复杂的情况,加强大气环境监测工作刻不容缓。因此本文以大气环境质量现状为出发点,对目前我国大气环境质量监测中存在的问题进行了分析,并就此提出了完善我国大气环境质量监测工作的对策,希望能推动我国大气环境质量的进一步改善。  相似文献   
319.
上海市浦东新区作为承接国家自由贸易区的先行试点地区,近年来吸引大批国内外企业入驻,同时经济发展与环境友好型社会矛盾依然突出。本文以2014年-2018年来浦东新区区域噪音与交通噪数据为依据,分析本地区声环境状况,结果表明声环境质量有所下降,一类功能区及交通噪音需进一步加强治理。通过源头屏蔽,大力发展张江、周浦、滴水湖等科技园区建设,阻断企业对居民区的噪声影响等措施,进而提升和改善浦东新区声环境质量状况。  相似文献   
320.
Soil inventories of anthropogenic radionuclides were investigated in altitudinal transects in 2 French regions, Savoie and Montagne Noire. Rain was negligible in these 2 areas the days after the Chernobyl accident. Thus anthropogenic radionuclides are coming hypothetically only from Global Fallout following Atmospheric Nuclear Weapon Tests. This is confirmed by the isotopic signatures (238Pu/239+240Pu; 137Cs/239+240Pu; and 241Am/239+240Pu) close to Global Fallout value. In Savoie, a peat core age-dated by 210Pbex confirmed that the main part of deposition of anthropogenic radionuclides occurred during the late sixties and the early seventies. In agreement with previous studies, the anthropogenic radionuclide inventories are well correlated with the annual precipitations. However, this is the first time that a study investigates such a large panel of annual precipitation and therefore of anthropogenic radionuclide deposition. It seems that at high-altitude sites, deposition of artificial radionuclides was higher possibly due to orographic precipitations.  相似文献   
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