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281.
To evaluate the quantities of 137Cs from past nuclear tests being transported to and deposited in Japan by naturally-occurring phenomena, the authors developed long-range transport models for 137Cs considering Asian dust. The simulation using these models backed the observed recent increase of 137Cs deposition along the coast of the Sea of Japan in early spring. For the sake of public safety, it is vital to ascertain whether an increase of radioactive deposition is caused by natural phenomena or a nuclear accident. The observations in recent years have suggested that dust and soil containing 137Cs is transported from the regions around Inner Mongolia to Japan by the wind. In this paper, using observation data from the early spring of 2002 and 2006, the authors have found good agreement between the simulations and the measurements. The simulations reproduced the entrainment of 137Cs and subsequent transport to Japan caused by strong winds associated with low pressure areas around the Inner Mongolian grasslands. The most likely cause of high-level 137Cs deposition over northern Japan during March 2002 was 137Cs associated with particles transported at low-altitude (1 km) and subjected to precipitation on the 22nd to 24th. 相似文献
282.
Sanders CJ Smoak JM Cable PH Patchineelam SR Sanders LM 《Journal of environmental radioactivity》2011,102(12):1122-1125
Total 210Pb and 7Be fallout rates were measured on the coastal region of Niteroi, Brazil. The monthly depositional flux of 210Pb and 7Be varied by a factor of 26, from 1.7 to 43.3 mBq cm−2 year−1 and ∼27, from 7.5 to 203.5 mBq cm−2 year−1, respectively. The relatively large oscillations in the depositional flux of 210Pb at this study site were likely due to variations in air mass sources, while the 7Be fluctuations may be driven by a combination of weather conditions. Local geology could support the periodic high fluxes of 210Pb from continental air masses, as shifting oceanic wind sources were affirmed by the uncorrelated 210Pb and 7Be fallout activities and 7Be/210Pb ratios. The 210Pb atmospheric deposition was found to be in agreement with local sediment inventories, an important consideration in geochemical studies that estimate sedimentation processes. 相似文献
283.
Akata N Kakiuchi H Shima N Iyogi T Momoshima N Hisamatsu S 《Journal of environmental radioactivity》2011,102(9):837-842
This study aimed at obtaining background tritium concentrations in precipitation and air at Rokkasho where the first commercial spent nuclear fuel reprocessing plant in Japan has been under construction. Tritium concentration in monthly precipitation during fiscal years 2001-2005 had a seasonal variation pattern which was high in spring and low in summer. The tritium concentration was higher than that observed at Chiba City as a whole. The seasonal peak concentration at Rokkasho was generally higher than that at Chiba City, while the baseline concentrations of both were similar. The reason for the difference may be the effect of air mass from the Asian continent which is considered to have high tritium concentration. Atmospheric tritium was operationally separated into HTO, HT and hydrocarbon (CH3T) fractions, and the samples collected every 3 d-14 d during fiscal year 2005 were analyzed for these fractions. The HTO concentration as radioactivity in water correlated well with that in the precipitation samples. The HT concentration was the highest among the chemical forms analyzed, followed by the HTO and CH3T concentrations. The HT and CH3T concentrations did not have clear seasonal variation patterns. The HT concentration followed the decline previously reported by Mason and Östlund with an apparent half-life of 4.8 y. The apparent and environmental half-lives of CH3T were estimated as 9.2 y and 36.5 y, respectively, by combining the present data with literature data. The Intergovernmental Panel on Climate Change used the atmospheric lifetime of 12 y for CH4 to estimate global warming in its 2007 report. The longer environmental half-life of CH3T suggested its supply from other sources than past nuclear weapon testing in the atmosphere. 相似文献
284.
The Geological Survey of Sweden (SGU) has been conducting airborne gamma spectrometry measurements of natural radioactivity in Sweden for more than 40 years. Today, the database covers about 80% of the country’s land surface. This article explores the first step of putting this data into use in radioactive source search at ground level. However, in order to be able to use the airborne background measurements at ground level, SGU data must be validated against terrestrial data. In this work, we compare the SGU data with data measured by a portable backpack system. This is done for three different areas in southern Sweden. The statistical analysis shows that a linear relationship and a positive correlation exist between the air and ground data. However, this linear relationship could be revealed only when the region possessed large enough variations in areal activity. Furthermore, the activity distributions measured show good agreement to those of SGU. We conclude that the SGU database could be used for terrestrial background assessment, given that a linear transfer function is established. 相似文献
285.
Górka M Sauer PE Lewicka-Szczebak D Jędrysek MO 《Environmental pollution (Barking, Essex : 1987)》2011,159(1):294-301
This paper describes results of chemical and isotopic analysis of inorganic carbon species in the atmosphere and precipitation for the calendar year 2008 in Wroc?aw (SW Poland). Atmospheric air samples (collected weekly) and rainwater samples (collected after rain episodes) were analysed for CO2 and dissolved inorganic carbon (DIC) concentrations and for δ13C composition. The values obtained varied in the ranges: atmospheric CO2: 337-448 ppm; δ13CCO2 from −14.4 to −8.4‰; DIC in precipitation: 0.6-5.5 mg dm−3; δ13CDIC from −22.2 to +0.2‰. No statistical correlation was observed between the concentration and δ13C value of atmospheric CO2 and DIC in precipitation. These observations contradict the commonly held assumption that atmospheric CO2 controls the DIC in precipitation. We infer that DIC is generated in ambient air temperatures, but from other sources than the measured atmospheric CO2. The calculated isotopic composition of a hypothetical CO2 source for DIC forming ranges from −31.4 to −11.0‰, showing significant seasonal variations accordingly to changing anthropogenic impact and atmospheric mixing processes. 相似文献
286.
PCDD/Fs atmospheric deposition fluxes and soil contamination close to a municipal solid waste incinerator 总被引:1,自引:0,他引:1
Bulk depositions and surface soil were collected in a suburban area, near the Adriatic Sea, in order to assess the contribution of a municipal solid waste incinerator to the area’s total contamination with polychlorinated dibenzodioxins and polychlorinated dibenzofurans (PCDDs and PCDFs). Samples were collected at two sites, situated in the area most affected by plant emissions (according to the results of the Calpuff air dispersion model), and at an external site, considered as a reference. Results show that the studied area is subject to low contamination, as far as these compounds are concerned. Deposition fluxes range from 14.3 pg m−2 d−1 to 89.9 pg m−2 d−1 (0.75 pg-TEQ m−2 d−1 to 3.73 pg-TEQ m−2 d−1) and no significant flow differences are observed among the three monitored sites. Total soil concentration amounts to 93.8 ng kg−1 d.w. and 1.35 ng-TEQ kg−1 d.w, on average, and confirms a strong homogeneity in the studied area. Furthermore, from 2006 to 2009, no PCDD/Fs enrichment in the soil was noticed. Comparing the relative congener distributions in environmental samples with those found in stack emissions from the incineration plant, significant differences are observed in the PCDD:PCDF ratio and in the contribution of the most chlorinated congeners. From this study we can conclude that the incineration plant is not the main source of PCDD/Fs in the studied area, which is apparently characterized by a homogeneous and widespread contamination situation, typical of an urban area. 相似文献
287.
Evaluation of surface runoff and road dust as sources of nitrogen using nitrate isotopic composition 总被引:1,自引:0,他引:1
Stable nitrogen and oxygen isotope ratios of nitrate (δ15N-NO3 and δ18O-NO3) have recently been used to identify nitrogen sources in water environments. However, there have been no investigations designed to determine nitrate isotopes in non-point sources in urban areas for evaluating the impact of surface deposits on nitrogen in surface runoff. In this study, we collected rainwater, surface runoff and surface deposits (road dust, roof dust and soil) to evaluate the nitrogen sources in surface runoff using nitrate isotopes. There were no large differences in δ15N-NO3 among rainwater (−0.3‰ to 1.5‰), surface runoff (−2.7‰ to 0.4‰), leachates from road dust (−5.8‰ to 6.2‰) and soil (−11.5‰ to 0.6‰). In contrast, the δ18O-NO3 in surface runoff (28.5-47.9‰) was lower than that in rainwater (62.7-78.6‰), and higher than that in leachates from road dust (6.1-27.6‰) and soil (−1.1‰ to 6.6‰). δ18O-NO3 is a useful indicator for evaluating the NO3-N sources in surface runoff. Using this indicator, NO3-N from road dust was estimated to account for more than half of the NO3-N in surface runoff. This is consistent with a result based on a comparison of their loads per unit surface between rainwater and surface runoff, which also showed that most of the nitrogen in surface runoff was derived from surface deposits. 相似文献
288.
E. Tipping J.J. Rothwell A.J. Lawlor 《Environmental pollution (Barking, Essex : 1987)》2010,158(5):1521-1529
Simulation modelling with CHUM-AM was carried out to investigate the accumulation and release of atmospherically-deposited heavy metals (Ni, Cu, Zn, Cd and Pb) in six moorland catchments, five with organic-rich soils, one with calcareous brown earths, in the Pennine chain of northern England. The model considers two soil layers and a third layer of weathering mineral matter, and operates on a yearly timestep, driven by deposition scenarios covering the period 1400-2010. The principal processes controlling heavy metals are competitive solid-solution partitioning of solutes, chemical interactions in solution, and chemical weathering. Agreement between observed and simulated soil metal pools and surface water concentrations for recent years was generally satisfactory, the results confirming that most contemporary soil metal is from atmospheric pollution. Metals in catchments with organic-rich soils show some mobility, especially under more acid conditions, but the calcareous mineral soils have retained nearly all anthropogenic metal inputs. Complexation by dissolved organic matter and co-transport accounts for up to 80% of the Cu in surface waters. 相似文献
289.
One century sedimentary records of polycyclic aromatic hydrocarbons, mercury and trace elements in the Qinghai Lake, Tibetan Plateau 总被引:2,自引:0,他引:2
Xiaoping Wang Handong Yang Xin Zhao Simon Turner 《Environmental pollution (Barking, Essex : 1987)》2010,158(10):3065-3070
Sediments from a remote lake of northeastern Tibetan Plateau were analyzed for polycyclic aromatic hydrocarbons (PAHs) and trace metals. USEPA priority PAHs, ranged from 11 in 1860 to 279 ng g−1 in 2002, while, the deposition fluxes were in the range of 0.2-11.4 ng cm−2 yr−1. Similarly, from 1860 to 2002, an increased trend of Hg flux was observed (0.5-3.2 ng cm−2 yr−1). Remarkable increase of PAHs and Hg concentration began from 1970, nearly the same period of the “Reform and Open” Policy had been embarked (1978) in China. Good correlations were found between concentrations of Pb, Zn, Cd, As, Hg, and PAHs, which suggested the sources of these chemicals in the sediment is analogous, likely from anthroprogenic sources. Based on isomer ratios, PAHs in core were dominantly from the incomplete combustion of coal. Owing to the proximity to dust source area (Qaidam Basin) and the close association between PAHs, Hg, Pb, and particle matters, atmospheric dust-transport and deposition might be the main pathways that pollutants enter into Qinghai Lake. 相似文献
290.
Tipping E Thacker SA Wilson D Hall JR 《Environmental pollution (Barking, Essex : 1987)》2008,152(1):41-49
During the last 50 years nitrate concentrations in Buttermere and Wastwater (Cumbria, UK) have risen significantly, by 70 and 100%, respectively. By estimating contemporary nitrate fluxes in the lakes' catchments and in sub-catchments and comparing them with the fractional areas of different soil types, it is deduced that the surface water nitrate is derived almost entirely from organic-rich ranker soils that have a limited ability to retain atmospherically-deposited nitrogen. Little or no nitrate leaches from the other major soil type, a brown podzol, despite it having a lower C:N ratio (12.0 g g(-1)) than the ranker (17.0 g g(-1)), nor is there much contribution from the small areas of improved (chemically fertilised) grassland within the catchments. Although some nitrate leaching is occurring, total N losses are appreciably smaller than atmospheric inputs, so the catchment soils are currently accumulating between 3 and 4 g N m(-2) a(-1). 相似文献