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11.
Fractionation of Cu, Pb and Zn in certified reference soils SRM 2710 and SRM 2711 using the optimized BCR sequential extraction procedure 总被引:4,自引:0,他引:4
Sequential extraction of metals from solid media is a common analytical tool used in environmental and exploration geochemistry. A number of procedures exist, but without harmonization and standardization, meaningful comparisons are tenuous without baseline data. A newly developed, standardized sequential extraction procedure (optimized BCR) was applied to two contaminated certified reference soils from Montana, US (SRM 2710 and SRM 2711) for Cu, Pb and Zn. Four operationally defined fractions were isolated, acid extractable, reducible, oxidizable, and residual (by aqua regia). Fraction-specific concentrations, percentages and recoveries for Cu, Pb and Zn were used to explore differences between the optimized BCR procedure and three other sequential extraction schemes with published data for SRM 2710 and 2711 (i.e. Tessier scheme, Geological Survey of Canada scheme and the original BCR scheme). Results indicate significant differences between the four schemes, even for schemes that are closely associated (i.e. the original and optimized BCR schemes). Order-of-magnitude fraction-specific concentration differences were observed, especially for Pb in the reducible fraction. Differences between schemes are worrisome because trends varied between metals, between fractions and between reference soils. These data reinforce the need for increased adoption of standardized sequential extraction procedures and further examination of different solid media. 相似文献
12.
Developing Canada's National Forest Carbon Monitoring, Accounting and Reporting System to Meet the Reporting Requirements of the Kyoto Protocol 总被引:2,自引:0,他引:2
The rate of carbon accumulation in the atmosphere can be reduced by decreasing emissions from the burning of fossil fuels
and by increasing the net uptake (or reducing the net loss) of carbon in terrestrial (and aquatic) ecosystems. The Kyoto Protocol
addresses both the release and uptake of carbon. Canada is developing a National Forest Carbon Monitoring, Accounting and
Reporting System in support of its international obligations to report greenhouse gas sources and sinks. This system employs
forest-inventory data, growth and yield information, and statistics on natural disturbances, management actions and land-use
change to estimate forest carbon stocks, changes in carbon stocks, and emissions of non-CO2 greenhouse gases. A key component of the system is the Carbon Budget Model of the Canadian Forest Sector (CBM-CFS). The model
is undergoing extensive revisions to enable analyses at four spatial scales (national, provincial, forest management unit
and stand) and in annual time steps. The model and the supporting databases can be used to assess carbon-stock changes between
1990 and the present, and to predict future carbon-stock changes based on scenarios of future disturbance rates and management
actions. 相似文献
13.
14.
Ten out of the 12 new EU members, used to belong to the so-called “former eastern block”, with a post WWII environmental policy radically different from the tendencies followed in Western Europe. The lack of conservation regulations has resulted in a rather harmful industrialization, regarding natural resources and environmental quality. While air pollution transfer is a phenomenon of transboundary level, there is a particular interest in examining the contribution of the new EU member states to the environmental pressure faced by the older member states and vice versa. The current study utilises the official data for almost 20 years published by the European Monitoring and Evaluation Program concerning the transboundary transfer of NOx and SO2 in order to analyse the situation and discuss the present and future environmental policy regarding air pollution. 相似文献
15.
Bernard Barraqué 《Natural resources forum》2003,27(3):200-211
The article contributes to a discussion on two global issues on water: water resources management, and water supply and sanitation. Focusing on Europe, it traces the legal roots of current systems in history: as a resource, water is considered as a common property, rather than a market good; while as a public service it is usually a commodity. Public water supply and sanitation technologies and engineering have developed under three main paradigms: quantitative and civil engineering; qualitative and chemical/sanitary engineering (both on the supply side); and the most recent one, environmental engineering and integrated management (on the demand side). The cost of public drinking water is due to rise sharply in view of the two‐fold financial challenge of replacing an ageing infrastructure and keeping up with ever‐rising environmental and sanitary quality standards. Who will pay? Government subsidies, or water users? The author suggests that apparent successes with privatisation may have relied heavily on hidden government subsidies and/or the healthy state of previously installed water infrastructure: past government subsidies are still felt for as long as the lifetime of the infrastructure. The article stresses the importance of public participation and decentralized local management of water and sanitation services. Informing and involving users in water management decisions is seen as an integral part of the ‘ethics’ side of the crucial three E's (economics, environment, ethics). The article strongly argues for municipal provision of water services, and hopes that lessons learnt and solutions found in the European experience may serve water services management efforts in other regions of the world. 相似文献
16.
Black liquor gasification–combined cycle (BLGCC) is a new technology that has the potential to increase electricity production of a chemical pulping mill. Increased electricity generation in combination with the potential to use biomass (e.g. bark, hog fuel) more efficiently can result in increased power output compared to the conventional Tomlinson-boiler. Because the BLGCC enables an integrated pulp and paper mill to produce excess power, it can offset electricity produced by power plants. This may lead to reduction of the net-CO2 emissions. The impact of BLGCC to offset CO2 emissions from the pulp and paper industry is studied. We focus on two different plant designs and compare the situation in Sweden and the US. The CO2 emissions are studied as function of the share of recycled fibre used to make the paper. The study shows that under specific conditions the production of “CO2-free paper” is possible. First, energy efficiency in pulp and paper mills needs to be improved to allow the export of sufficient power to offset emissions from fossil fuels used in boilers and other equipment. Secondly, the net-CO2 emission per ton of paper depends strongly on the emission reduction credits for electricity export, and hence on the country or grid to which the paper mill is connected. Thirdly, supplemental use of biomass to replace fossil fuel inputs is important to reduce the overall emissions of the pulp and paper industry. 相似文献
17.
Summary The balance of evidence suggests a perceptible human influence on global ecosystems. Human activities are affecting the global
ecosystem, some directly and some indirectly. If researchers could clarify the extent to which specific human activities affect
global ecosystems, they would be in a much better position to suggest strategies for mitigating against the worst disturbances.
Sophisticated statistical analysis can help in interpreting the influence of specific human activities on global ecosystems
more carefully. This study aims at identifying significant or influential human activities (i.e. factors) on CO2 emissions using statistical analyses. The study was conducted for two cases: (i) developed countries and (ii) developing
countries. In developed countries, this study identified three influential human activities for CO2 emissions: (i) combustion of fossil fuels, (ii) population pressure on natural and terrestrial ecosystems, and (iii) land
use change. In developing countries, the significant human activities causing an upsurge of CO2 emissions are: (i) combustion of fossil fuels, (ii) terrestrial ecosystem strength and (iii) land use change. Among these
factors, combustion of fossil fuels is the most influential human activity for CO2 emissions both in developed and developing countries. Regression analysis based on the factor scores indicated that combustion
of fossil fuels has significant positive influence on CO2 emissions in both developed and developing countries. Terrestrial ecosystem strength has a significant negative influence
on CO2 emissions. Land use change and CO2 emissions are positively related, although regression analysis showed that the influence of land use change on CO2 emissions was still insignificant. It is anticipated, from the findings of this study, that CO2 emissions can be reduced by reducing fossil-fuel consumption and switching to alternative energy sources, preserving exiting
forests, planting trees on abandoned and degraded forest lands, or by planting trees by social/agroforestry on agricultural
lands. 相似文献
18.
19.
Shuxiao Wang Lei Zhang Long Wang Qingru Wu Fengyang Wang Jiming Hao 《Frontiers of Environmental Science & Engineering》2014,8(5):631-649
Mercury, as a global pollutant, has significant impacts on the environment and human health. The current state of atmospheric mercury emissions, pollution and control in China is comprehensively reviewed in this paper. With about 500-800 t of anthropogenic mercury emissions, China contributes 25%-40% to the global mercury emissions. The dominant mercury emission sources in China are coal combustion, non-ferrous metal smelting, cement production and iron and steel production. The mercury emissions from natural sources in China are equivalent to the anthropogenic mercury emissions. The atmospheric mercury concentration in China is about 2-10 times the background level of North Hemisphere. The mercury deposition fluxes in remote areas in China are usually in the range of 10-50μg·m^-2·yr^-1. To reduce mercury emissions, legislations have been enacted for power plants, non-ferrous metal smelters and waste incinerators. Currently mercury contented in the flue gas is mainly removed through existing air pollution control devices for sulfur dioxide, nitrogen oxides, and particles. Dedicated mercury control technologies are required in the future to further mitigate the mercury emissions in China. 相似文献
20.
Identification of magnetic particulates in road dust accumulated on roadside snow using magnetic, geochemical and micro-morphological analyses 总被引:2,自引:0,他引:2
Bućko MS Magiera T Johanson B Petrovský E Pesonen LJ 《Environmental pollution (Barking, Essex : 1987)》2011,159(5):1266-1276
The aim of this study is to test the applicability of snow surveying in the collection and detailed characterization of vehicle-derived magnetic particles. Road dust extracted from snow, collected near a busy urban highway and a low traffic road in a rural environment (southern Finland), was studied using magnetic, geochemical and micro-morphological analyses. Significant differences in horizontal distribution of mass specific magnetic susceptibility (χ) were noticed for both roads. Multi-domain (MD) magnetite was identified as the primary magnetic mineral. Scanning electron microscope (SEM) analyses of road dust from both roads revealed: (1) angular-shaped particles (diameter ∼1-300 μm) mostly composed of Fe, Cr and Ni, derived from circulation of motor vehicles and (2) iron-rich spherules (d ∼ 2-70 μm). Tungsten-rich particles (d < 2 μm), derived from tyre stud abrasion were also identified. Additionally, a decreasing trend in χ and selected trace elements was observed with increasing distance from the road edge. 相似文献