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91.
92.
Yongjie Yang Rui Zhou Yue Yu Yan Yan Yan Liu Yi''an Di Dan Wu Weiqi Zhang 《环境科学学报(英文版)》2017,29(5):146-156
The characteristics of water-soluble ions in size-resolved particulate matter were investigated usingion chromatography at Shangdianzi,a regional background station of Beijing,Tianjin,and Hebei.Seasonal total concentrations of ions(Na~+,Mg~(2+),K~+,Ca~(2+),NH_4~+,Cl~-,SO_4~(2-) and NO_3~-) were75.5±52.9 μg/m~3 in spring,26.5±12.3μg/m~3 in summer,22.7±20.4μg/m~3 in autumn,and31.1±23.9 μg/m~3 in winter,respectively.The secondary ions(NO_3~-,SO_4~(2-) and NH_4~+),mainly associated with fine particles,accounted for 84.2%in spring,82.1%in summer,81.5%in autumn and 76.3%in winter of all ions.Strong correlations were found between NH_4~+ and SO_4~(2-)(r=0.95,p0.01) as well as NH_4~+ and NO_3~-(r=0.90,p0.01) in fine particles;while in coarse particles,correlations between Mg~(2+) and NO_3~-(r=0.80,p0.01),and Ca~(2+) and NO_3~-(r=0.85,p0.01) were found.The concentrations of Na~+,K~+,Mg~(2+),Ca~(2+),NH_4~+,Cl~-,NO_3~-,and SO_4~(2-) were 2.02,0.81,0.36,1.65,9.58,4.01,18.9,and 18.4 μg/m~3 in particulate matter from southeast-derived air masses,which were typically 1.58-3.37 times higher than in northwest trajectories.Thus,concentrations of water-soluble ions at this background station were heavily influenced by regional transport of serious pollution derived from biomass burning,coal combustion,industrial and vehicle exhaust emissions from Beijing,Tianjin,and Hebei. 相似文献
93.
Kang Sun Xingang Liu Jianwei Gu Yunpeng Li Yu Qu Junling An Jingli Wang Yuanhang Zhang Min Hu Fang Zhang 《环境科学学报(英文版)》2015
Size-resolved aerosol samples were collected by MOUDI in four seasons in 2007 in Beijing. The PM10 and PM1.8 mass concentrations were 166.0 ± 120.5 and 91.6 ± 69.7 μg/m3, respectively, throughout the measurement, with seasonal variation: nearly two times higher in autumn than in summer and spring. Serious fine particle pollution occurred in winter with the PM1.8/PM10 ratio of 0.63, which was higher than other seasons. The size distribution of PM showed obvious seasonal and diurnal variation, with a smaller fine mode peak in spring and in the daytime. OM (organic matter = 1.6 × OC (organic carbon)) and SIA (secondary inorganic aerosol) were major components of fine particles, while OM, SIA and Ca2 + were major components in coarse particles. Moreover, secondary components, mainly SOA (secondary organic aerosol) and SIA, accounted for 46%–96% of each size bin in fine particles, which meant that secondary pollution existed all year. Sulfates and nitrates, primarily in the form of (NH4)2SO4, NH4NO3, CaSO4, Na2SO4 and K2SO4, calculated by the model ISORROPIA II, were major components of the solid phase in fine particles. The PM concentration and size distribution were similar in the four seasons on non-haze days, while large differences occurred on haze days, which indicated seasonal variation of PM concentration and size distribution were dominated by haze days. The SIA concentrations and fractions of nearly all size bins were higher on haze days than on non-haze days, which was attributed to heterogeneous aqueous reactions on haze days in the four seasons. 相似文献
94.
三沙湾海水中磷的分布和富营养化研究 总被引:1,自引:0,他引:1
根据2010、2011年三沙湾水质监测资料,评价了活性磷酸盐的分布及时空变化特征,根据N/P和Si/N比判断三沙湾浮游植物生长的限制因子,用营养状态指数评价该湾水体的富营养化状态.结果表明,霍童溪为三沙湾海水中磷的主要陆源输入来源,磷为三沙湾植物生长繁殖限制因子,磷含量季节周期变化特征明显,5月植物生长繁殖旺盛,由于磷的匮乏,生长受到限制,磷含量降至最低水平,8月由于植物腐败分解释放磷和海水水温较高抑制植物生长,使磷含量升高,11月至次年1月,磷含量持续升高.三沙湾内富营养化指数大于1,存在发生赤潮的风险. 相似文献
95.
《环境科学学报(英文版)》2023,35(3):524-532
The study of atmospheric polycyclic aromatic hydrocarbons (PAHs) in northeastern Tibetan Plateau with fragile ecological environment and complex atmospheric circulation system is blank. To understand the characteristics and sources of persistent organic pollutants in the atmosphere of the northeastern Tibetan Plateau, we monitored levels in the central Qilian Mountain. From 2016 to 2017, we collected 45-pair (particle + gas) samples using active air samplers to investigate the sources, transport paths, and their influencing factors. Sources of PAHs were analysed with a source diagnostic model, and atmospheric transport paths were calculated. The concentration range for ∑15PAHs was 439–4666 pg/m3, and the average was 2015 pg/m3. The PAHs in central Qilian Mountain are mainly low molecular weight (LMW) PAHs. Winter concentrations of PAHs were higher than those in summer. The transport of PAHs is mainly affected by westerlies, and there are seasonal differences. Source analysis showed that PAHs mainly came from coal and biomass combustion and vehicle emissions, with seasonal differences. This study clarifies the concentration and seasonal variation of PAHs in the northern Tibetan Plateau, which is conducive to understanding the atmospheric transport process and fate of pollutants. The background site of Qilian Mountains located in the Silk Road economic belt has the value and significance of long-term observation of pollutants. 相似文献
96.
The inorganic anion pollution of the New Calabar River surface water was investigated. Results showed seasonal variations
in the inorganic anion levels. Water parameters such as sulfite, nitrate, phosphate, and alkalinity showed significantly higher
values in the rainy season than in the dry season. Dissolved oxygen, pH, sulfide, sulfate, ammonia, and nitrite showed no
significant differences between their rainy and dry season levels. Upstream-downstream changes were shown by conductivity,
total dissolved solids, chloride, salinity, and temperature. Exceptions occurred in the nitrite levels, where the effect was
minimal. Although the concentrations of some anions analyzed fell within internationally acceptable limits, the New Calabar
River water is, in the main, polluted with inorganic anions and may be unacceptable for potable and industrial uses without
treatment. 相似文献
97.
Zhihua Li Zhenyu Hang Qian Zhang Shuangshuang Zhang Tianyu Zhang Hanqing Yu 《环境科学学报(英文版)》2019,31(5):330-338
Respirograms of activated sludge OUR_ x~Tand OUR_x~(20)were measured under site(T) and standard(20°C) temperatures, respectively, and the predicted standard temperature respirogram OUR_( x,cal)~(20)was also calculated using the Arrhenius equation. These respirogram profiles reveal more information than effluent quality. A decrease of OUR_ x ~(20)is a critical alarm signal for the loss of pollutant removal capacity, and a sudden increase of the predicted value OUR_( x,cal)~(20)is an alarm signal for the unrecoverable deterioration of biomass. The sign of OUR_x~(20)–OUR_(x,cal)~(20)can be used for selection of tuning strategies. For example, a negative value of OUR_x~(20)–OUR_( x,cal)~(20)indicates that doubling biomass is difficult,thus strategies such as extending the reaction time with limited available biomass is preferred. The findings in this study elucidated the respiration profile of activated sludge under changes of temperature and can be effectively used for the stable operation of Wastewater Treatment Plants under cold temperatures and seasonal variations. 相似文献
98.
Zhen-Chao Zhou Ze-Jun Lin Xin-Yi Shuai Ji Zheng Ling-Xuan Meng Lin Zhu Yu-Jie Sun Wei-Chun Shang Hong Chen 《环境科学学报(英文版)》2021,33(5):12-19
Antibiotic resistance genes (ARGs) as emergence contaminations have spread widely in the water environment. Wild fish may be recipients and communicators of ARGs in the water environment, however, the distribution and transmission of ARGs in the wild fish and relevant water environment were rarely reported. Here, we have profiled ARGs and bacterial communities in wild freshwater fish and relevant water in a peri-urban river using high-throughput qPCR and 16S rRNA gene sequence. A total of 80 and 220 unique ARG subtypes were identified in fish and water samples. Fish and water both showed significant ARG seasonal variations (P < 0.05). The highest absolute abundance of ARGs in fish and water occurred in summer (1.32 × 109 copies per g, on average) and autumn (9.04 × 106 copies per mL), respectively. In addition, the bipartite network analysis showed that 9 ARGs and 1 mobile genetic element continuously shared in fish and water. Furthermore, bacteria shared in fish and water were found to significantly correlate with shard ARGs. The findings demonstrate that bacteria and ARGs in fish and water could interconnect and ARGs might transfer between fish and water using bacteria as a spreading medium. 相似文献
99.
Monitoring of Seasonal Variation in the Water Quality of Ubu River in Ekwusigo and Nnewi Local Government Areas of Anambra State,Nigeria 总被引:1,自引:0,他引:1
Investigation of the water quality of the Ubu river has been carried out. The upstream course of the river is slightly acidic (pH 5.45 ± 0.23), and the acidity decreases along the lower courses of the river. Turbidity, surfactant, and iron content parameters of the river increased during the wet season, and these changes have been attributed to inputs from flood, leachates of soil erosion, and storm water runoff discharged into the river in increased quantities during the season. Concentrations of some metals were found to increase during the dry season because of absence of dilution of the river by storm water runoff. Most water quality parameters are within World Health Organization acceptable limits set for potable water, and they include most of the cationic and anionic constituents. Although there is no hydrocarbon or metal ion pollution, potability is reduced along the mid to downstream courses of the river by unacceptable levels of turbidity, surfactant concentration, and iron content, particularly during the wet season. 相似文献
100.
Christopher C. Estes John F. Orsborn 《Journal of the American Water Resources Association》1986,22(3):389-398
ABSTRACT: Present guidelines for selecting a method to determine instream flow requirements and evaluating the validity of the results from a particular method are insufficient. This paper contributes to the efforts of researchers to develop a guide and critique for instream flow methods. A review of instreani flow methods and recommendations for their application is supplemented by a summary of a comparison of four independent analyses. The four analyses: the Physical Habitat Simulation System approach of the Instream Flow Incremental Methodology by the U.S. Fish and Wildlife Service, the Montana Method by Tennant, and two methods by Orsborn (Maximum Spawning Area Flow and Maximum Spawning Area) represent resource intensive and simplistic data collection and analysis methods. Each analysis was used to independently determine flows to support spawning by chinook salmon (Oncorhynchus tshawytscha) in Willow Creek, Alaska. Results of these analyses indicate that each method can be used independently or collectively to generate instream flow recommendations, if calibrated to the site or area studied. Once adjusted to the species and basin of interest, methods similar to the Montana and two Orsborn methods should be used to determine flow recommendations for areas where competition for water is minimal. The Instream Flow Incremental Methodology or similar methods should be applied when competition for water is keen or when detailed evaluations of the responses of species/life phases to flow variations are required. 相似文献