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Fraser M Barker JF Butler B Blaine F Joseph S Cooke C 《Journal of contaminant hydrology》2008,100(3-4):101-115
An emplaced source of coal tar creosote within the sandy Borden research aquifer has documented the long-term (5140 days) natural attenuation for this complex mixture. Plumes of dissolved chemicals were produced by the essentially horizontal groundwater flowing at about 9 cm/day. Eleven chemicals have been extensively sampled seven times using a monitoring network of approximately 280, 14-point multilevel samplers. A model of source dissolution using Raoult's Law adequately predicted the dissolution of 9 of 11 compounds. Mass transformation has limited the extent of the plumes as groundwater has flowed more than 500 m, yet the plumes are no longer than 50 m. Phenol and xylenes have been removed and naphthalene has attenuated from its maximum extent on day 1357. Some compound plumes have reached an apparent steady state and the plumes of other compounds (dibenzofuran and phenanthrene) are expected to continue to expand due to an increasing mass flux and limited degradation potential. Biotransformation is the major process controlling natural attenuation at the site. The greatest organic mass lost is associated with the high solubility compounds. However, the majority of the mass loss for most compounds has occurred in the source zone. Oxygen is the main electron acceptor, yet the amount of organics lost cannot be accounted for by aerobic mineralization or partial mineralization alone. The complex evolution of these plumes has been well documented but understanding the controlling biotransformation processes is still elusive. This study has shown that anticipating bioattenuation patterns should only be considered at the broadest scale. Generally, the greatest mass loss is associated with those compounds that have a high solubility and low partitioning coefficients. 相似文献
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煤焦油加氢制燃料油的试验研究 总被引:2,自引:0,他引:2
实验室研究利用煤焦油研制汽柴油替代品燃料油.以高温煤焦油为原料,选择加氢保护剂、脱金属剂及加氢精制催化剂,采用加氢工艺,脱除煤焦油中硫、氮、氧和金属等有害杂质,使煤焦油中烯烃饱和,从而改善煤焦油质量,制得合格的汽油、柴油替代品燃料油. 相似文献
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有害固体废物热解焦油特性研究 总被引:6,自引:0,他引:6
通过对几种有害固体废物(皮橡胶,废电路板,医疗废物,废油漆,污泥)的热解实验,考察了不同工况下有害固体废弃物热解焦油的特性。研究了不同工况下焦油产率的影响因素。物料特性、热解终温及加热方式,对有害固体废物热解焦油的产率有着重要的影响。在实验温度范围内,不同工况条件下,对热解焦油密度和热值进行了测定,热解焦油密度在0.75—0.95g/m1范围内,焦油热值在6.306—9.112kal/g之间,高于原始物料的热值。对不同工况下的热解焦油进行了族分分析,焦油中一般饱和烃和极性物的含量较高。 相似文献
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Occurrence and attenuation of specific organic compounds in the groundwater plume at a former gasworks site 总被引:1,自引:0,他引:1
The changing contaminant pattern with travelled distance was investigated in the anaerobic groundwater plume downstream from an extended zone containing residual NAPL at a former gas manufacturing plant. With increasing distance, O- and N-heterocyclic aromatic compounds are enriched in the plume relative to the usually assessed coal tar constituents (poly- and monocyclic aromatic compounds). In a first approximation, the overall concentration decrease of the investigated compounds follows a first order overall decay. The half life distance in the plume downgradient from the source varied between 20 m for benzene and up to 167-303 m for alkyl-naphthalenes. Acenaphthene is degraded only within about 50 m downstream from the source area, then its concentration remains constant (ca. 180 microg/l) and far above the legal limit. Dimethyl-benzofurans were the most recalcitrant among all compounds which could be quantified with the analytical method available. The overall groundwater contamination in the plume is seriously underestimated if only BTEX and 16-EPA-PAHs are monitored. 相似文献