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181.
Soonchul Kwon Maohong Fan Herbert F. M. DaCost Armistead G. Russell 《环境科学学报(英文版)》2011,23(8):1233-1239
Olivine, one of the most abundant minerals existing in nature, is explored as a CO2 carbonation agent for direct carbonation of
CO2 in flue gas. Olivine based CO2 capture is thermodynamically favorable and can form a stable carbonate for long-term storage.
Experimental results have shown that water vapor plays an important role in improving CO2 carbonation rate and capacities. Other
operation conditions including reaction temperature, initial CO2 concentration, residence time corresponding to the flow rate of CO2
gas stream, and water vapor concentration also considerably affect the performance of the technology. 相似文献
182.
Pretreatment of thickened waste activated sludge (TWAS) by combined microwave and alkaline pretreatment (MAP) was studied to
improve thermophilic anaerobic digestion efficiency. Uniform design was applied to determine the combination of target temperature
(110–210°C), microwave holding time (1–51 min), and NaOH dose (0–2.5 g NaOH/g suspended solids (SS)) in terms of their effect
on volatile suspended solids (VSS) solubilization. Maximum solubilization ratio (85.1%) of VSS was observed at 210°C with 0.2
g-NaOH/g-SS and 35 min holding time. The effects of 12 different pretreatment methods were investigated in 28 thermophilic batch
reactors by monitoring cumulative methane production (CMP). Improvements in methane production in the TWAS were directly related
to the microwave and alkaline pretreatment of the sludge. The highest CMP was a 27% improvement over the control. In spite of the
increase in soluble chemical oxygen demand concentration and the decrease in dewaterability of digested sludge, a semi-continuous
thermophilic reactor fed with pretreated TWAS without neutralization (at 170°C with 1 min holding time and 0.05 g NaOH/g SS)
was stable and functioned well, with volatile solid (VS) and total chemical oxygen demand (TCOD) reductions of 28% and 18%,
respectively, which were higher than those of the control system. Additionally, methane yields (L@STP/g-CODadded, at standard
temperature and pressure (STP) conditions of 0°C and 101.325 kPa) and (L@STP/g VSadded) increased by 17% and 13%, respectively,
compared to the control reactor. 相似文献
183.
The Hg0 vapor adsorption experimental results on a novel sorbent obtained by impregnating a commercially available activated
carbon (Darco G60 from BDH) with silver nitrate were reported. The study was performed by using a fundamental approach, in an
apparatus at laboratory scale in which a synthetic flue gas, formed by Hg0 vapors in a nitrogen gas stream, at a given temperature
and mercury concentration, was flowed through a fixed bed of adsorbent material. Breakthrough curves and adsorption isotherms were
obtained for bed temperatures of 90, 120 and 150°C and for Hg0 concentrations in the gas varying in the range of 0.8–5.0 mg/m3. The
experimental gas-solid equilibrium data were used to evaluate the Langmuir parameters and the heat of adsorption. The experimental
results showed that silver impregnated carbon was very effective to capture elemental mercury and the amount of mercury adsorbed by
the carbon decreased as the bed temperature increased. In addition, to evaluate the possibility of adsorbent recovery, desorption was
also studied. Desorption runs showed that both the adsorbing material and the mercury could be easily recovered, since at the end of
desorption the residue on solid was almost negligible. The material balance on mercury and the constitutive equations of the adsorption
phenomenon were integrated, leading to the evaluation of only one kinetic parameter which fits well both the experimentally determined
breakthrough and desorption curves. 相似文献
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188.
淀山湖沉积物碳-氮垂直分布特征 总被引:1,自引:0,他引:1
近年来,经过一系列污染治理措施,淀山湖的营养水平持续下降,但每年仍有不同程度的蓝藻水华暴发,严重影响其作为水源地的安全性。为了进一步探讨淀山湖水质改善策略,本研究对淀山湖沉积物营养状况进行了调查研究,分析了淀山湖沉积物碳、氮分布特征及垂直变化规律,并用沉积物肥力评价了淀山湖沉积物营养程度。结果表明,淀山湖沉积物营养盐存在明显的富集作用,二十多年来沉积物碳、氮含量大幅上升,表层沉积物均属于重污染状态。空间分布上,沉积物营养盐北部高,南部低,北部样点大部分属于重污染状态,南部样点基本属于中污染状态。垂直分布上,受航道回淤与北部围网养殖影响,部分样点营养盐垂直分布规律不显著,其他样点均表现出随深度增加营养盐显著降低的趋势。除出水口D1样点外,淀山湖有机质与TN表现出显著的同源相关性,表明有机质是淀山湖内源负荷的主要来源。 相似文献
189.
苯酚对活性污泥活性及微型动物群落结构的影响 总被引:1,自引:1,他引:0
为了探究苯酚对污泥活性及微型动物群落结构的影响,以SBR工艺的活性污泥为研究对象,分析苯酚对污泥TTC-ETS活性、INT-ETS活性和微型动物群落结构及其动态变化的影响.结果表明,污泥TTC-ETS活性较之INT-ETS活性能够更有效表征有机毒害物质苯酚对污泥活性的影响,且随着进水苯酚浓度的增大,苯酚对污泥活性的抑制越明显:进水浓度在50mg·L-1时,苯酚对污泥活性的抑制率为(20.75±10.43)%.进水苯酚浓度为100 mg·L-1时,抑制率为(39.73±26.92)%,且波动较大.在300 mg·L-1进水运行后期,苯酚对污泥活性的抑制率稳定在40%左右;苯酚对活性污泥微型动物群落结构的影响随浓度的增大而增大,且对不同微型动物类群影响不同:在低浓度苯酚进水条件下,只有单个微型动物类群(有壳变形虫)受到明显的抑制,而当浓度增大至100 mg·L-1和300 mg·L-1时,对多个微型动物类群(固着型纤毛虫、有壳变形虫、匍匐型纤毛虫、肉食性纤毛虫等)产生抑制,对少数类群(鞭毛虫、线虫等)产生促进作用;苯酚影响下的污泥活性与微型动物之间存在一定的关联性,针棘匣壳虫(Centropyxis aculeata)、多变斜板虫(Plagiocampa mutabilis)等可作为含酚废水处理过程中污泥活性低的指示生物,湖累枝虫(Epistylis lacustris)、软波豆虫(Bodo lens)、跳侧滴虫(Pleuromonas jaculans)等可作为污泥活性高的指示生物. 相似文献
190.
Multi-walled carbon nanotube(MWCNT) sheet was fabricated from a drawable MWCNT forest and then deposited on poly(methyl methacrylate) film. The film was further coated with a natural antimicrobial peptide nisin. We studied the effects of nisin coating on the attachment of Bacillus anthracis spores, the germination of attached spores, and the subsequent biofilm formation from attached spores. It was found that the strong adsorptivity and the super hydrophobicity of MWCNTs provided an ideal platform for nisin coating. Nisin coating on MWCNT sheets decreased surface hydrophobicity, reduced spore attachment, and reduced the germination of attached spores by 3.5 fold, and further inhibited the subsequent biofilm formation by 94.6% compared to that on uncoated MWCNT sheet. Nisin also changed the morphology of vegetative cells in the formed biofilm.The results of this study demonstrated that the anti-adhesion and antimicrobial effect of nisin in combination with the physical properties of carbon nanotubes had the potential in producing effective anti-biofilm formation surfaces. 相似文献