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171.
Xihua Zhang Yongbing Xie Hongbin Cao Faheem Nawaz Yi Zhang 《Waste management (New York, N.Y.)》2014,34(9):1715-1724
To solve the recycling challenge for aqueous binder based lithium-ion batteries (LIBs), a novel process for recycling and resynthesizing LiNi1/3Co1/3Mn1/3O2 from the cathode scraps generated during manufacturing process is proposed in this study. Trifluoroacetic acid (TFA) is employed to separate the cathode material from the aluminum foil. The effects of TFA concentration, liquid/solid (L/S) ratio, reaction temperature and time on the separation efficiencies of the cathode material and aluminum foil are investigated systematically. The cathode material can be separated completely under the optimal experimental condition of 15 vol.% TFA solution, L/S ratio of 8.0 mL g?1, reacting at 40 °C for 180 min along with appropriate agitation. LiNi1/3Co1/3Mn1/3O2 is successfully resynthesized from the separated cathode material by solid state reaction method. Several kinds of characterizations are performed to verify the typical properties of the resynthesized LiNi1/3Co1/3Mn1/3O2 powder. Electrochemical tests show that the initial charge and discharge capacities of the resynthesized LiNi1/3Co1/3Mn1/3O2 are 201 mAh g?1 and 155.4 mAh g?1 (2.8–4.5 V, 0.1 C), respectively. The discharge capacity remains at 129 mAh g?1 even after 30 cycles with a capacity retention ratio of 83.01%. 相似文献
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Zinc is one of the most widely applied nonferrous metals in China. Study on the applications and recurrent situation of zinc resources is of great strategic importance for the sustainable development of China's economy. In this paper, a dynamic material flow analysis (MFA) method has been adopted to analyze quantificationally zinc resources in China, as well as to analyze and predict the quantity of zinc product scrap and their recycling situation. The weighted average method was applied to calculate average lifetimes of six major zinc products in China. The average lifetimes of battery, zinc oxide, zinc die-casting alloys, zinc material products, galvanized zinc and brass are 0.17, 5.3, 11.1, 12, 21 and 30 years, respectively. Assuming the lifetime of zinc product group obeys the Weibull distribution and the consumption of zinc products varies linearly with time, the future consumption and scrap generation of zinc products will increase continuously. It is expected that they would increase from 49% to 76% during 2004–2020, respectively. Assuming the recycling rate remains unchanged with time, the zinc old scrap index, both the theoretical and actual values, would continue increasing in China. The values are expected to reach 0.402 and 0.076 by 2020, respectively. Therefore, the regeneration resource of depreciated zinc is actually insufficient in China. According to the scenario analysis, the actual value of old scrap indexes is positively correlated with the recycling rate of zinc products. Because galvanized products are the largest consumption area of zinc products in China, the influence of their recycling rate on old scrap index is obviously larger than other zinc products. Through the analysis, this paper suggests that the increase of the recycling rate of zinc products could not only improve to a certain degree China's relative shortage of zinc resources, but greatly relive the supply pressure of zinc in the world. 相似文献
174.
Primary steelmaking involves CO2-intensive processes, but the expansion of secondary steel production is limited by the global availability of steel scrap. The present work examines global scrap consumption in the past (1870–2012) and future scrap availability (2013–2050) based on the historical trend. The results reveal that (i) historically, the consumption of old scrap has been insufficient compared with the amounts of discarded steel, and (ii) based on historical scrap consumption, the future availability of scrap will not be sufficient to satisfy the two assumed cases of steel demand. Primary steelmaking is expected to remain the dominant process, at least up until 2050. Under the reference-demand case of 2.19 billion tons in crude steel production by 2050, the total production of pig iron and direct reduced iron could reach 1.35 billion tons. Consumption of old scrap could reach 0.76 billion tons. Because the availability of scrap will be limited in the context of the global total, it is important to research and develop innovative low-carbon technologies for primary steelmaking and to explore their economic viability if we are to aim for achieving large reductions in CO2 emissions from the iron and steel industry. 相似文献
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介绍了不同加工方式对铬靶烧结密度的影响。在机压过程中,采用双向压制,不添任何成型剂和脱氧剂。机压+真空烧结铬环靶材密度为78%~80%;冷等静压+真空烧结铬板靶材密度大于82%;而经轧制后,铬板靶材密度提高到90%~95%;铬合金靶材采用热压方式,其密度大于98%。通过优化烧结时间和烧结温度等工艺参数,铬环靶材的烧结成本大大降低。 相似文献
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The scrap vehicle recycling program was formally initiated in 1995 when the illegal dumping issues of scrap tires and cars turn out to be intolerable in the society of Taiwan. The inherent complexity of such a recycling program, however, by integrating many public and private sectors that functions as a whole from the collection, storage, transport, treatment, and the disposal of scrape vehicles, makes the entire managerial efficiency hard to be maintained. Therefore, the state-of-the-art information technology via the use of the Internet platform becomes an indispensable tool to present a good communication mechanism, to provide the essential information sharing between all users and agencies, and to end up with improving the overall managerial efficiency. The idea using advanced web database along with geographical information system to help general public to dump their scrap vehicles smoothly and to make governmental agency control the disposal procedure easily could be one of the best solutions from the long-term environmental management perspective. This paper, representing contemporary progress of environmental management skill performed by the Foundation for Reduction, Reuse and Recovery, sponsored by the Environmental Protection Administration (EPA) in Taiwan, is designed to illustrate how to build up such a system, as named by the Scrap Vehicles Recycling Program Information System (SVRPIMS) in order to meet the requirement from both supply and demand sides of scrap vehicles disposal. Experience gained in this study indicates that the SVRPIMS successfully integrates the Coldfusion® and Mapguide® software engineering technologies on the World Wide Web (WWW) platform. After actual implementation in 1999, it proved that communication between users and agencies at various levels in the recycling program became much easier through instant information retrieval and analysis via such a system. Besides, SVRPIMS also provides two decision-support functionalities to assist in automatic search for the most appropriate dumping site for the users and to perform possible trading of spare parts for the recyclers through a logistic optimization analysis. 相似文献