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851.
McKenzie C.H. Lim Godwin A. Ayoko Lidia Morawska Zoran D. Ristovski E. Rohan Jayaratne 《Atmospheric environment (Oxford, England : 1994)》2005,39(40):7836-7848
Emissions from 12 in-service heavy-duty buses powered by low- (LSD) and ultra low-sulfur (ULSD) diesel fuels were measured with the aim to characterize the profile of polycyclic aromatic hydrocarbons (PAHs) in the exhaust and to identify the effect of different types of fuels on the emissions. To mimic on-road conditions as much as possible, sampling was conducted on a chassis dynamometer at four driving modes, namely: mode 7 or idle (0% power), mode 11 (25% power), mode 10 (50% power) and mode 8 (100% power). Irrespective of the type of fuel used, naphthalene, acenaphthene, acenaphthylene, anthracene, phenanthrene, fluorene, fluoranthene and pyrene were found to be the dominant PAHs in the exhaust emissions of the buses. However, the PAH composition in the exhausts of ULSD buses were up to 91±6% less than those in the LSD buses. In particular, three- and four-ringed PAHs were more abundant in the later than in the former. Lowering of fuel sulfur content not only reduced PAH emission, but also decreased the benzo(a)pyrene equivalent (BAPeq) and hence the toxicity of the exhaust. Result from multicriteria decision-making and multivariate data analysis techniques showed that the use of ULSD afforded cleaner exhaust compositions and emissions with characteristics that are distinct from those obtained by the use of LSD. 相似文献
852.
This paper considers two alternative feedstocks for bioethanol production, both derived from household waste—Refuse Derived Fuel (RDF) and Biodegradable Municipal Waste (BMW). Life Cycle Assessment (LCA) has been carried out to estimate the GHG emissions from bioethanol using these two feedstocks. An integrated waste management system has been considered, taking into account recycling of materials and production of bioethanol in a combined gasification/bio-catalytic process. For the functional unit defined as the ‘total amount of waste treated in the integrated waste management system’, the best option is to produce bioethanol from RDF—this saves up to 196 kg CO2 equiv. per tonne of MSW, compared to the current waste management practice in the UK.However, if the functional unit is defined as ‘MJ of fuel equiv.’ and bioethanol is compared with petrol on an equivalent energy basis, the results show that bioethanol from RDF offers no saving of GHG emissions compared to petrol. For example, for a typical biogenic carbon content in RDF of around 60%, the life cycle GHG emissions from bioethanol are 87 g CO2 equiv./MJ while for petrol they are 85 g CO2 equiv./MJ. On the other hand, bioethanol from BMW offers a significant GHG saving potential over petrol. For a biogenic carbon content of 95%, the life cycle GHG emissions from bioethanol are 6.1 g CO2 equiv./MJ which represents a saving of 92.5% compared to petrol. In comparison, bioethanol from UK wheat saves 28% of GHG while that from Brazilian sugar cane – the best performing bioethanol with respect to GHG emissions – saves 70%. If the biogenic carbon of the BMW feedstock exceeds 97%, the bioethanol system becomes a carbon sequester. For instance, if waste paper with the biogenic carbon content of almost 100% and a calorific value of 18 MJ/kg is converted into bioethanol, a saving of 107% compared to petrol could be achieved. Compared to paper recycling, converting waste paper into bioethanol saves 460 kg CO2 equiv./t waste paper or eight times more than recycling. 相似文献
853.
Environmental evaluation of transfer and treatment of excess pig slurry by life cycle assessment 总被引:1,自引:0,他引:1
Lopez-Ridaura S Werf Hv Paillat JM Le Bris B 《Journal of environmental management》2009,90(2):1296-1304
Slurry management is a central topic in the agronomic and environmental analysis of intensive livestock production systems. The objective of this study is to compare the environmental performance of two scenarios of collective slurry management for the disposal of excess nitrogen from animal manure. The scenarios are the transfer of slurry and its injection to crop land, and the treatment of slurry in a collective biological treatment station. The study is based on a real case in the West of France, where a group of farmers is developing a collective plan for the disposal of almost 7000 m(3) of excess pig slurry. The evaluation is carried out by Life Cycle Assessment, where emissions and resource consumption are quantified and aggregated into four environmental impact categories: eutrophication, acidification, climate change, and non-renewable energy use. Ammonia emitted is the most important contributor to acidification and eutrophication, while methane contributes most to climate change. Both ammonia and methane are mostly emitted during the storage of slurry and, in the case of the treatment scenario, also during composting the solid fraction of the slurry. The two management strategies are similar with respect to climate change, whereas eutrophication and acidification are twice as large for treatment relative to transfer. Electricity needed for the treatment process is the main contributor to non-renewable energy use for the treatment scenario, while the transfer scenario represents a net energy saving, as energy saved by the reduction of mineral fertiliser use more than compensates for the energy needed for transport and injection of slurry. The overall environmental performance of transfer is better than that of treatment, as it involves less acidification, eutrophication and non-renewable energy use. The method employed and the results obtained in this study can provide elements for a transparent discussion of the advantages and disadvantages of contrasting excess slurry management scenarios as well as the identification of the main aspects determining their environmental performance. 相似文献
854.
Nutrient-Balance Modeling as a Tool for Environmental Management in Aquaculture: The Case of Trout Farming in France 总被引:1,自引:0,他引:1
Papatryphon E Petit J Van Der Werf HM Sadasivam KJ Claver K 《Environmental management》2005,35(2):161-174
The control and prevention of nutrient pollution from fish farming plays an essential role in the French regulatory framework. Assessing nutrient emissions from fish farms is important in terms of farm authorization, taxation, and monitoring. Currently employed strategies involve both water sampling and empirical modeling. This article reports the work and outcomes of an expert panel that evaluated existing methodologies and their possible alternatives. The development and evaluation of a nutrient-balance approach was assessed as a potential alternative to currently used methodologies. A previously described nutrient-balance model was suggested and parameterized using expert choice, and its validity and applicability were assessed. The results stress that the nutrient-balance model provides more robust and relatively conservative waste estimates compared to the currently used methodologies. Sensitivity of the approach to the uneven data quality available at farm level, difficulties of on-farm measurements, as well as model requirements and limitations are discussed. 相似文献
855.
Li Lin Hao Jiming Hu Jingnan 《Frontiers of Environmental Science & Engineering in China》2007,1(3):339-344
This work evaluates the influence of energy consumption on the future air quality in Beijing, using 2000 as the base year
and 2008 as the target year. It establishes the emission inventory of primary PM10, SO2 and NOx related to energy utilization in eight areas of Beijing. The air quality model was adopted to simulate the temporal and spatial
distribution of each pollutant concentration in the eight urban areas. Their emission, concentration distribution, and sectoral
share responsibility rate were analyzed, and air quality in 2008 was predicted. The industrial sector contributed above 40%
of primary PM10 and SO2 resulting from energy consumption, while vehicles accounted for about 65% of NOx. According to the current policy and development trend, air quality in the eight urban areas could become better in 2008
when the average concentrations of primary PM10, SO2 and NO2 related to energy utilization at each monitored site are predicted to be about 25, 50 and 51 μg/m3, respectively.
Translated from China Environmental Science, 2005, 25(6): 746–750 [译自: 中国环境科学] 相似文献
856.
John G. Farmer Lorna J. Eades Margaret C. Graham 《Environmental geochemistry and health》1999,21(3):257-272
More than 60 coal samples, predominantly from the principal coalfields of England and Wales (25) and Scotland (30), were analysed for lead by AAS and for stable lead isotopes by ICPMS. While the average lead content of Scottish coal, 23.9mg kg–1, was more than double that of coal from England and Wales, 11.0mg kg–1, the corresponding mean 206Pb/207Pb ratios (± 1 s.d.) were nearly identical, at 1.181±0.011 and 1.184±0.006, respectively. In the light of the lead isotopic signatures of British coals and of both indigenous (206Pb/207Pb 1.17) and imported Australian (206Pb/207Pb 1.04) lead ores, an approach based on estimated lead emissions from these sources and the deconvolution of the historical lead and 206Pb/207Pb records preserved in lake sediments, peat bogs and archival herbage material indicates that coal combustion became an increasingly significant contributor to atmospheric lead deposition in the UK during the period 1830–1930, especially after the onset of Englands decline as a major location of lead mining and smelting in the late19th Century. Since 1930 and the introduction of leaded petrol, the atmospheric 206Pb/207Pb ratio in the UK has been strongly influenced by carexhaust emissions of comparatively 206Pbdepleted lead of predominantly Australian origin, counterbalanced to some extent by coalcombustion emissions of lead, although these have fallen dramatically since the mid1950s. Nevertheless, with the introduction and substantial uptake of unleaded petrol in the UK during the last decade, even the declining releases from coal, along with contributions from other sources, are continuing to affect the atmospheric lead content and 206Pb/207Pb ratio. 相似文献
857.
M. -L. Quinn 《Environmental management》1991,15(2):179-194
The Copper Basin is located within the southern Appalachian Mountains primarily in extreme southeastern Tennessee, USA. It
has long been known for its copper mining/smelting and associated chemical industry, as well as its severely injured environment.
Virtually all previous commentary on the environmental degradation at this location have focused on human activities and their
destructive impact. This article approaches the subject from a different angle, one that emphasizes the interaction between
man and nature.
The site's physical setting, industrial history, and environmental history are briefly reviewed. The theory then presented
here is that certain of the Copper Basin's natural features made its environment unusually vulnerable to the negative impact
of copper mining and smelting, especially as practiced around the turn of the century. These features are identified. This
reasoning provides the basis for the concept of environmental susceptibility, which is defined and discussed. A few of its
applications are mentioned. This study offers a new perspective on the Copper Basin, as well as insights for those whose work
involves investigating the man/nature relationship—both past and present. 相似文献
858.
This paper assesses the distribution of ammonium (NH4+) and nitrate (NO3-) nitrogen deposition in native bushland soil adjacent to an open ventilated poultry farm. The farm is located in Thirlmere 150 km south west of Sydney, Australia. A total of 104 geographically referenced soil cores were obtained from the study area. Soil pH, electrical conductivity (EC), NH4(+) - and NO3(-)-nitrogen concentrations were analysed for variable trends at three depths, i.e. 0-30, 30-60, and 60-90 cm. Significantly higher concentrations of the two nitrogen forms and EC were observed nearer to the farm in the surface soil samples (0-30 cm). The distribution of NH4+, NO3- and EC were all correlated in surface samples throughout the study area. There was no indication of NH4+ and NO3- leaching within soil profile sampled and it appears that weeds and native vegetation had utilised the accumulated nitrogen. The level of N deposition adjacent to the poultry farm decreased downwind due to dispersion of plume and to the buffering effects from the bushland. 相似文献
859.
Source characterization and identification by real-time single particle mass spectrometry 总被引:1,自引:0,他引:1
Melissa S. Reinard Kouame Adou Joseph M. Martini Murray V. Johnston 《Atmospheric environment (Oxford, England : 1994)》2007,41(40):9397-9409
A Real-Time Single Particle Mass Spectrometer, RSMS-3, was deployed to Wilmington, Delaware to study regional and local contributions to fine and ultra-fine urban particulate matter (PM). Approximately two-thirds of PM1 consisted of internally mixed secondary aerosol. The remaining one-third was externally mixed including biomass burning (13%), fossil fuel combustion (7%) and various industrial sources (13%). In this last group, particle classes containing specific combinations of transition and/or heavy metals gave wind-rose plots consistent with specific point sources. For example, particles containing V and Ni were detected from different wind directions than those containing V and Fe. Samples from two industrial emission stacks, a steel manufacturing facility 10 km away and a coal-fired electrical power generation facility 5 km away, were analyzed and compared to the ambient data set. In each case, a direct correlation was found: a Pb–Zn–K–Na class for the steel manufacturing facility and an Fe–La/Ce class for the power generation facility. The ambient particle classes showed additional small signals from secondary components indicating atmospheric processing. Ambient particle classes containing only a subset of these elements, such as Zn only, Fe only and Pb–K only, were nonspecific, that is, the wind-rose plots were more diffuse and the particles could not be mapped to individual sources. The merits of stack sampling as an aid to interpreting single particle data sets are discussed. 相似文献
860.
Various approaches have been proposed for allocating commitments to countries regarding the mitigation of greenhouse gas emissions. One of these methods is the ‘contraction and convergence’ approach, which defines emission permits on the basis of converging per capita emissions under a contracting global emission profile. The approach is unique in its simplicity. Only two major issues need to be negotiated and agreed upon: the target atmospheric concentration of CO2 and the date when the entitlements are to converge at equal per capita allocations. According to the contraction and convergence approach, developing countries can continue their current emission trends, whereas industrialized countries should reduce their emissions quite dramatically. This regime represents a shift away from the current approach towards defining commitments for all parties and their evolution over the long term. This article analyses how allocation schemes determined by the contraction and convergence approach might affect certain OECD and non‐OECD countries. Results for eleven countries selected for analysis (United States, United Kingdom, Germany, France, Japan, China, Venezuela, Thailand, Brazil, India and Indonesia) reveal that trends observed in the past few decades in most industrialized countries will lead to the contraction and convergence target. 相似文献