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51.
Yang Zhang Tianyi Zhao Yu Yan Bian Zhou Xuezhen Zhong Xiaoyu Hu Lijia Zhang Peng Huo Kang Xiao Yuanxun Zhang 《环境科学学报(英文版)》2023,35(2):835-845
Ambient particulate matter (PM) can cause adverse health effects via their ability to produce Reactive Oxygen Species (ROS). Water-Soluble Organic Compounds (WSOCs), a complex mixture of organic compounds which usually coexist with Transition Metals (TMs) in PM, have been found to contribute to ROS formation. However, the interaction between WSOCs and TMs and its effect on ROS generation are still unknown. In this study, we examined the ROS concentrations of V, Zn, Suwannee River Fulvic Acid (SRFA), Suwannee River Humic Acid (SRHA) and the mixtures of V/Zn and SRFA/SRHA by using a cell-free 2′,7′-Dichlorodihydrofluorescein (DCFH) assay. The results showed that V or Zn synergistically promoted ROS generated by SRFA, but had an antagonistic effect on ROS generated by SRHA. Fluorescence quenching experiments indicated that V and Zn were more prone to form stable complexes with aromatic humic acid-like component (C1) and fulvic acid-like component (C3) in SRFA and SRHA. Results suggested that the underlying mechanism involving the fulvic acid-like component in SRFA more tending to complex with TMs to facilitate ROS generation through π electron transfer. Our work showed that the complexing ability and complexing stability of atmospheric PM organics with metals could significantly affect ROS generation. It is recommended that the research deploying multiple analytical methods to quantify the impact of PM components on public health and environment is needed in the future. 相似文献
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Recovery of heavy metals from electroplating sludge and stainless steel pickle waste liquid by ammonia leaching method 总被引:2,自引:0,他引:2
1 IntroductionElectroplatingsludge,containingCu,Ni,Zn,Cr,Fe,etc.,isharmfulwastematerialproducedbygalvanizationindustry.Thereisstillnoeffectivemethodtorecoverresourceandcontrolpollutionbothathomeandabroad.Themetalsdiscardedbygalvanizationindustryamoun… 相似文献
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This paper deals with the release of base cations and Al3+ at the treatment with simulated acid rain (SAR) in main soil types collected from South China. Results showed that the amounts of base cations increased obviously when the pH value of simulated acid rain was lower than 3.0 or 3.5. Compared with the leaching of K+ and Na+, the leaching of Ca2+ and Mg2+ was affected by the pH value of SAR. Only when the amounts of base cations leached from soils exceeded the cation exchange capacity, the pH value of leaching solutions decreased sharply and the amounts of released Al3+ increased. The H+ buffering mechanisms, which were affected notonly by the pH values of SAR, but also by the types and solid components of soils, were proposed for the main soils studied. 相似文献
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利用空气质量资料、常规观测资料、NCEP1.0°×1.0°再分析资料,应用数理统计、天气学等方法对宿迁市3次突发性重污染天气进行对比分析.结果表明:①宿迁"突发"空气重污染时,AQI级别由前一日的一、二级至第2日转为五级以上,AQI值迅速上升.②3次空气重污染过程天气背景相似,高层为宽广平直的偏西气流,地面受高压控制,中低层风向和温度平流突然转变,且都有深厚的逆温层结;持续变化较小的气压梯度、较低风速、温度日较差及相对湿度的增大(150328过程(即2015年3月28日—4月1日污染过程)除外)为颗粒物浓度迅速增长提供了条件.③大气稳定度级别迅速变高和混合层高度迅速降低并维持,对污染物快速聚集有显著影响.④物理量诊断表明,污染发生前期上空为弱上升运动,随后迅速转为下沉运动,或气流下沉运动区域迅速扩大、升高,是空气质量迅速转差的重要动力因素.⑤内蒙古地区的沙尘远距离输送形成的污染,是造成150328过程与另外两次过程明显不同的主要原因. 相似文献
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几种重金属对紫背萍过氧化氢酶活性的影响 总被引:12,自引:0,他引:12
通过测定被暴露植物分解过氧化氢后放出氧气的体积,确定紫背萍过氧化氢酶(CAT)的活性。结果表明,紫背萍暴露在Hg、Pb、Cr、Ni、Fe的溶液中,其CAT活性除在Pb作用下明显降低外,在其它4种重金属的作用下都有不同程度的升高。这表明Pb对紫背萍 CAT活性有抑制作用,而其它4种重金属对紫背萍CAT均有刺激作用。紫背萍对5种重金属所表现出来的这种生态效应,是重金属水污染的植物潜在效应,植物的CAT 相似文献
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In this paper it was reported that PbCl2 , CdCl2 , HgCl2, and aquatic environmental samples containing Al, Cd, Cu, Pb, Sr, Zn and other heavy metal ions as well as organic chemicals suppressed thegrowth of E. coli only at higher exposed concentrations. The stimulative effects of PbCl2 and HgCl2 on thegrowth of E. coli were clearly showed at lower concentrations and longer time. It suggested that the toxic effects of heavy metal ions and other pollutants on the growth of E. coli are variable according to the differentexposed levels. 相似文献
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IntroductionFertilizationisessentialforagriculturalproduction ,butunreasonablyapplyingfertilizerscouldresultinseriesofproblemssuchascropqualitydecline,fertilizeruseefficiencydecrease,residualfertilizerspollution groundwaterandriversandnitrogencontented … 相似文献