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It has been shown that starch can effectively stabilize nanoscale magnetite particles, and starch-stabilized magnetite nanoparticles (SMNP) are promising for in situ remediation of arsenic-contaminated soils. However, a molecular level understanding has been lacking. Here, we carried out XAFS studies to bridge this knowledge gap. Fe K-edge XAFS spectra indicated that the Fe-O and Fe-Fe coordination numbers of SMNP were lower than those for bare magnetite particles, and these coordination numbers decreased with increasing starch concentration. The decrease in the average coordination number at elevated stabilizer concentration was attributed to the increase in the surface-to-volume ratio. Arsenic K-edge XAFS spectra indicated that adsorbed arsenate on SMNP consisted primarily of binuclear bidentate (BB) complexes and monodentate mononuclear (MM) complexes. More BB complexes (energetically more favorable) were observed at higher starch concentrations, indicating that SMNP not only offered greater adsorption surface area, but also stronger adsorption affinity toward arsenate. 相似文献
43.
Rachnarin Nitisoravut Cao N. D. Thanh Roshan Regmi 《International Journal of Green Energy》2017,14(8):712-723
There is an increasing trend to conduct the researches related to Microbial Fuel Cells (MFCs) in the recent years. Limited power output has been the major obstacle for the practical application and upscaling of MFCs. Attempts have been made on electrode modifications such as anode treatments, cathode modifications with catalysts and bio cathodes developments to produce varying degrees of improved output current depending upon the types of modifications. Power density and Coulombic efficiency have been considered as the important parameters to analyze the system performances. This paper overviews on the advances made in MFCs’ researches focusing on different types of electrodes modifications along with the involved methodology. Furthermore, the system performances of different modified MFCs are compared in terms of the power density and the Coulombic efficiency. 相似文献
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双区电除尘器降低锅炉烟尘排放浓度 总被引:1,自引:0,他引:1
粉尘在传统结构的荷电区荷电之后,一部分尘粒被阳极板捕集,大部分带有正、负电荷的尘粒再分别被收尘区的管式辅助电极和阳极板捕集.模拟试验数据表明,收尘区具有高电压、低电流和板电流密度分布均匀的特性.工业性试验结果显示,应用双区电除尘技术设计或改造电除尘器,不仅可以较好地防止发生反电晕,而且能够将锅炉烟尘排放质量浓度降低到50 mg/m3以下.与传统的卧式电除尘器相比,还可节省10%左右的占地面积和钢材用量. 相似文献
46.
Toropov AA Toropova AP Benfenati E Gini G Puzyn T Leszczynska D Leszczynski J 《Chemosphere》2012,89(9):1098-1102
Convenient to apply and available on the Internet software CORAL (http://www.insilico.eu/CORAL) has been used to build up quantitative structure-activity relationships (QSAR) for prediction of cytotoxicity of metal oxide nanoparticles to bacteria Escherichia coli (minus logarithm of concentration for 50% effect pEC50). In this study six random splits of the data into the training and test set were examined. It has been shown that the CORAL provides a reliable tool that could be used to build up a QSAR of the pEC50. 相似文献
47.
Dariusz Guziejewski Mariola Brycht Agnieszka Nosal-Wiercińska Sylwia Smarzewska Witold Ciesielski Sławomira Skrzypek 《Journal of environmental science and health. Part. B》2013,48(8):550-556
The electrochemical behavior of new generation fungicide acibenzolar-s-methyl (S-methyl 1,2,3-benzothiadiazole-7-carbothioate, ASM) on the hanging mercury drop electrode (HMDE) was investigated using square wave adsorptive stripping voltammetry. This method of determination is based on the irreversible reduction of ASM at the HMDE. The well-defined ASM peak was observed at ?0.4 V (vs. Ag/AgCl) in BR buffer at pH 2.2. The reduction peak current was proportional to concentration of ASM from 1.0 × 10?8 to 6.0 × 10?8 mol L?1 with detection and quantification limit 3.0 × 10?9 and 1.0 × 10?8 mol L?1, respectively. The applicability of the developed method for analysis of spiked samples of tap water, river water, and soil is illustrated. The effect of adsorption on the mercury electrode was studied in detail using the AC impedance method. Possible interferences with other common pesticides and heavy metal ions were examined. Clarification of the electrode mechanism was made using cyclic voltammetry (CV) technique. 相似文献
48.
介绍了阜康冶炼厂无污染新工艺和环境治理的有关情况 ,从理论上阐述了无污染工艺和污水治理的技术原理 ,对有色金属冶炼工业逐步采用湿法精炼清洁工艺有一定的指导作用 相似文献
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为解决传统电化学方法在含聚污水处理时电极板消耗严重、絮渣量大的问题,通过改进电极板材料、组合数及结构等,研究适度降解-除油一体化电化学技术,在降低渣泥量的同时保证处理效果。实验结果表明:最佳电极板组合为"网状惰性金属复合物极板(阳)-网状铝极板(阴)-网状铝极板(阴)-网状惰性金属复合物极板(阳)";在电解电流为4.0 A、极板间距为8.0 cm、面体比(电极板面积与处理污水量的比值)为2/17 cm~2/mL、电解时间为30 min的最佳处理条件下,几乎无絮渣产出,含聚污水的浊度去除率为93.3%、聚合物降解率为92.0%、除油率为95.0%,展现了优良的处理效果。 相似文献