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1.
Bunge Michael Khknen Mika A. Rmisch Winfried Opel Matthias Vogler Susanne Walkow Fred Salkinoja-Salonen Mirja Lechner Ute 《Environmental science and pollution research international》2007,14(1):3-10
Background, Aims and Scope Sediments of the Spittelwasser creek are highly polluted with organic compounds and heavy metals due to the discharge of untreated
waste waters from the industrial region of Bitterfeld-Wolfen, Germany over the course of more than one century. However, relatively
few data have been published about the chloroorganic contamination of the sediment. This paper reports on the content of different
(chloro)organic compounds with special emphasis on polychlorinated dibenzo-p-dioxins and dibenzofurans (PCDD/F), and chlorobenzenes. Existing concepts for the remediation of Spittelwasser sediment include
the investigation of natural attenuation processes, which largely depend on the presence of an intact microbial food web.
In order to gain more insight in terms of biological activity, we analyzed the capacity of sediment microflora to degrade
organic matter by measuring the activities of extracellular hydrolytic enzymes involved in the biogeochemical cycling of carbon,
nitrogen, phosphorus and sulfur. Furthermore, the detection of physiologically active bacteria in the sediment, particularly
of those known for their capability to reductively dehalogenate organochlorine compounds, illustrates the potential for intrinsic
bioremediation processes.
Methods PCDD/F and chlorobenzenes were analyzed by gas chromatography(GC)/mass spectrometry and GC/flame ionization detection, respectively.
The activities of hydrolytic enzymes were determined from freshly sampled sediment layers using 4-methylumbelliferyl (MUF)
or 7-amino-4-methylcoumarin-conjugated model compounds and kinetic fluorescence measurements. Physiologically active bacteria
from different sediment layers were microscopically visualized by fluorescence in situ hybridization (FISH). Specific bacteria were identified by 16S rRNA gene amplification and sequencing.
Results and Discussion The PCDD/F congener profile was dominated by dibenzofurans. In addition, the presence of specific tetra and pentachlorinated
dibenzofurans supported the assumption that extensive magnesium production was one possible source for the high contamination.
A range of other chloroorganic compounds, including several isomers of chlorobenzenes, hexachlorocyclohexane and 1,1,1-trichloro-2,2-bis
(p-chloro-phenyl)ethane (DDT), was present in the sediment. Activities of extracellular hydrolytic enzymes showed a strong
decrease in those sediment layers that were characterized by high contents of absorbable organic halogen (AOX), indicating
disturbed organic matter decay. Interestingly, an abnormal increase of cellulolytic enzyme activities below the organochlorine-rich
layers was observed, possibly caused by residual cellulose from discharges of sulfite pulping wastes. FISH revealed physiologically
active bacteria in most sediment layers from the surface down to the depth of about 60 cm, including members of Desulfitobacterium (D.) and Sulfurospirillum. The presence of D. dehalogenans was confirmed by its partial 16S rRNA gene sequence.
Conclusions Results of chemical sediment analyses demonstrated high loads of organochlorine compounds, particularly of PCDD/F. Several
years after stopping the waste water discharge to Spittelwasser creek, this sediment remains a main source for pollution of
the downstream river system by way of the ongoing mobilization of sediment during high floods. As indicated by our enzyme
activity measurements, the decomposition potential for organic matter is low in organochlorine-rich sediment layers. In contrast,
the comparably higher enzyme activities in less organochlorine-polluted sediment layers as well as the presence of physiologically
active bacteria suggest a considerable potential for natural attenuation.
Recommendations and Perspectives From our data we strongly recommend to explore the degradative capacity of sediment microorganisms and the limits for in situ activity towards specific sediment pollutants in more detail. This will give a sound basis for the integration of bioremediation
approaches into general concepts to reduce the risk that permanently radiates from this highly contaminated sediment.
Submission Editor: Dr. Henner Hollert (Henner.Hollert@urz.uniheidelberg.de) 相似文献
2.
国际海事组织目前正在对《MARPOL73/78公约》附则Ⅱ-控制散装液体有毒物质污染规则作重大修改,内容包手胡毒液体物质和化学品,这很可能对主管机关、船公司和化工界造成严重的冲击。 相似文献
3.
4.
单级与两级序批式反应器用于牛场污水处理的比较研究 总被引:1,自引:0,他引:1
对序批式反应器 (SBR)的特点进行了简要的介绍。研究了水力停留时间和有机负荷率对单级和两级SBR用于牛场污水处理时污染物去除率和出水水质的影响 ,并对单级和两级SBR的污水处理性能进行了比较。研究结果表明 ,当用单级SBR处理 10 0 0 0mg LCODCr的污水时 ,1d水力停留时间即可获得较好的处理效果 ,但出水中仍含有一定量的氨。两级SBR可使用较短的水力停留时间而获得较高的污染物去除率和较好的出水水质 ,并可通过硝化过程实现氨的完全的去除 相似文献
5.
介绍了采用中和混凝 水解酸化 生物接触氧化 化学除磷工艺对可发性聚苯乙烯 (EPS)废水的处理工艺。在废水中的CODCr、TP、SS、NH3 N分别为 194 0mg L、112mg L、5 92mg L、2 3 6mg L的条件下 ,废水经过处理后 ,出水CODCr、TP、SS、NH3 N分别为 70mg L、0 38mg L、2 6mg L、0 32mg L ,均可达到《污水综合排放标准》中的一级标准 ,废水中CODCr、TP、SS、NH3 N的平均去除率分别为 96 4 %、99 3%、95 6 %、98 6 %。 相似文献
6.
爆炸法处理废旧轮胎制造橡胶粉末技术及关键机理研究 总被引:6,自引:0,他引:6
主要介绍了利用爆炸法处理废旧轮胎制造橡胶粉末的技术 ;探讨了橡胶在爆炸作用下破坏的机理 ,爆炸法中橡胶变形速率与它的剪切模量和断裂韧性的关系 ;分析了利用直接爆炸法处理废旧轮胎的 3种实验结果 ,验证了对轮胎进行预处理的必要性 ,探讨了炸药用量的选择原则 相似文献
7.
水解酸化+两级生物接触氧化处理高盐度水产品加工废水 总被引:1,自引:0,他引:1
介绍了“水解酸化+两级生物接触氧化”处理水产品加工废水的运行效果和工程实例,结果表明:对C1^-浓度平均6000mg/L的高盐度水产品加工废水,系统对COD、SS、氨氮的去除率分别超过了88%、90%、85%,出水COD、SS、氨氮分别低于100mg/L、70mg/L、15mg/L,出水完全可以达到《污水综合排放标准》(GB8978—1996)一级排放标准。 相似文献
8.
随着新型工业化的发展,污染治理已实现了从单纯的末端治理向在生产过程中治理转变的跨越式发展。但新的环境问题如消费废弃物污染的面更广,内容更多和高新技术污染等相继出现。这些污染应引起人们的广泛关注。 相似文献
9.
涡凹气浮机在炼油污水处理中的应用 总被引:3,自引:0,他引:3
陈长顺 《石油化工环境保护》2004,27(4):21-22,49
对涡凹气浮机在炼油污水气浮工艺的改造的应用进行了总结,改造后该气浮机具有投资省、运行费用低、操作维护简单、工作效率高等优点,且运行稳定,效果比较理想,应用前景十分广阔。 相似文献
10.