全文获取类型
收费全文 | 1384篇 |
免费 | 144篇 |
国内免费 | 472篇 |
专业分类
安全科学 | 69篇 |
废物处理 | 57篇 |
环保管理 | 297篇 |
综合类 | 1004篇 |
基础理论 | 303篇 |
污染及防治 | 141篇 |
评价与监测 | 60篇 |
社会与环境 | 58篇 |
灾害及防治 | 11篇 |
出版年
2024年 | 5篇 |
2023年 | 15篇 |
2022年 | 35篇 |
2021年 | 43篇 |
2020年 | 42篇 |
2019年 | 43篇 |
2018年 | 35篇 |
2017年 | 52篇 |
2016年 | 57篇 |
2015年 | 74篇 |
2014年 | 86篇 |
2013年 | 121篇 |
2012年 | 115篇 |
2011年 | 104篇 |
2010年 | 106篇 |
2009年 | 89篇 |
2008年 | 56篇 |
2007年 | 121篇 |
2006年 | 102篇 |
2005年 | 65篇 |
2004年 | 86篇 |
2003年 | 70篇 |
2002年 | 67篇 |
2001年 | 56篇 |
2000年 | 60篇 |
1999年 | 53篇 |
1998年 | 46篇 |
1997年 | 39篇 |
1996年 | 33篇 |
1995年 | 20篇 |
1994年 | 16篇 |
1993年 | 13篇 |
1992年 | 8篇 |
1991年 | 4篇 |
1990年 | 6篇 |
1989年 | 5篇 |
1988年 | 3篇 |
1987年 | 2篇 |
1986年 | 2篇 |
1985年 | 4篇 |
1984年 | 4篇 |
1983年 | 5篇 |
1982年 | 10篇 |
1981年 | 3篇 |
1980年 | 2篇 |
1979年 | 3篇 |
1978年 | 3篇 |
1975年 | 2篇 |
1972年 | 2篇 |
1969年 | 1篇 |
排序方式: 共有2000条查询结果,搜索用时 31 毫秒
141.
142.
Charles D. Ikenberry William G. Crumpton Jeffrey G. Arnold Michelle L. Soupir Philip W. Gassman 《Journal of the American Water Resources Association》2017,53(6):1267-1280
The ability to accurately simulate flow and nutrient removal in treatment wetlands within an agricultural, watershed‐scale model is needed to develop effective plans for meeting nutrient reduction goals associated with protection of drinking water supplies and reduction of the Gulf of Mexico hypoxic zone. The objectives of this study were to incorporate new equations for wetland hydrology and nutrient removal in Soil and Water Assessment Tool (SWAT), compare model performance using original and improved equations, and evaluate the ramifications of errors in watershed and tile drain simulation on prediction of NO3‐N dynamics in wetlands. The modified equations produced Nash‐Sutcliffe Efficiency values of 0.88 to 0.99 for daily NO3‐N load predictions, and percent bias values generally less than 6%. However, statistical improvement over the original equations was marginal and both old and new equations provided accurate simulations. The new equations reduce the model's dependence on detailed monitoring data and hydrologic calibration. Additionally, the modified equations increase SWAT's versatility by incorporating a weir equation and an irreducible nutrient concentration and temperature coefficient. Model improvements enhance the utility of SWAT for simulating flow and nutrients in wetlands and other impoundments, although performance is limited by the accuracy of inflow and NO3‐N predictions from the contributing watershed. Editor's note : This paper is part of the featured series on SWAT Applications for Emerging Hydrologic and Water Quality Challenges. See the February 2017 issue for the introduction and background to the series. 相似文献
143.
144.
对自然恢复下4类不同年代样地的灰渣养分含量及重金属含量进行研究,通过对比分析发现,有机质、全氮、全钾、全磷含量随着自然恢复时间的增加呈现递增的趋势,全磷含量在各恢复阶段与对照样地之间并不存在显著差异(P0.05)。pH随着恢复时间的增加呈现递减的趋势。对灰渣综合质量指数进行研究发现,自然恢复长期、中期、短期与自然恢复初期对比均有显著提高(P0.05),且随着自然恢复时间的增加灰渣综合质量指数逐渐提高。对灰渣场锌、铅、铜3种重金属研究后发现,在自然恢复下随着时间的增加,灰渣中重金属含量均呈现递减的趋势。 相似文献
145.
为了提高传统污水处理工艺的脱氮除磷效率、实现污泥资源化,本实验通过超声破解污泥获取碳源,采用耗氧呼吸速率分析上清液作为碳源的可行性,并将上清液回用于生活污水,考察其对A2O工艺长期运行的脱氮除磷效果和微生物群落结构的影响。结果表明,上清液中可降解有机物达到76.2%,具有作为内碳源的潜能;上清液和生活污水按1∶15投入A2O反应器后,氮、磷的去除率分别从63.2%和53.4%提高到了82.1%和94.7%;上清液明显改变了微生物群落结构,使除磷菌Actinobacteia和反硝化聚磷菌Sphingobacterium富集。 相似文献
146.
为有效去除发电厂烟气中产生的NOx,利用介质阻挡放电(DBD)产生低温等离子体并结合催化剂Ag/Al2O3进行烟气脱硝实验,研究了在加入乙烯的条件下,平均负载量、催化温度和装置的布置方式对NOx脱除的影响。结果表明,随着负载的增多,NO脱除率呈现先增大后减小的趋势,5种负载量中最佳为1.76%;随着催化温度的升高,NO脱除率同样呈现先增大后减小的趋势,最佳的催化温度为150℃左右;3种不同布置方式对NO和NOx脱除有明显差别,单独催化剂在NO和NOx的脱除率都比较低;单独介质阻挡放电NO脱除率很高,但是NOx很却很低;而两者结合在NO和NOx都达到了很好的效果。 相似文献
147.
采用强电离介质阻挡放电方法制取高浓度氧活性粒子(O+2、O3)并注入气体外排烟道中,实现O+2、O3氧化NO转化成资源酸(HNO3)的等离子化学反应。描述强电离放电的氧活性粒子产生器,讨论烟道中O+2、O3氧化NO成HNO3等离子体反应机制,分析回收酸液的NO-2、NO-3离子种类及浓度。考察强电离放电等离子体源的输入功率、水体积百分比、气体温度、气体流速对NOx氧化率的影响。氧化率为97.2%的最佳实验条件是:O+2浓度为1.38×1010个/cm3,O3浓度为210 mg/L,烟气温度为65℃,H2O体积浓度为5.6%,停留时间为0.94 s。 相似文献
148.
研究了辉光放电等离子体降解水中典型的环境内分泌干扰物邻苯二甲酸二丁酯(DBP)及降解过程中过氧化氢(H2O2)的生成规律。考察了电解质种类、共存污染物(甲醇、叔丁醇)及催化剂等条件对DBP降解及H2O2生成的影响。结果表明,在硫酸钠溶液中DBP降解效率和H2O2生成速率最高;甲醇、叔丁醇等共存污染物对DBP降解和H2O2生成有抑制作用;Fe2+,Fe3+和Cu2+对DBP的降解有催化作用,其催化效果为Fe2+>Fe3+>Cu2+。用高效液相色谱、离子色谱及气质联用仪等仪器分析了降解中间产物,提出了可能的降解机理。 相似文献
149.
Anju A. Kenge Ping H. Liao Kwang V. Lo 《Journal of environmental science and health. Part. B》2013,48(6):606-612
The microwave enhanced advanced oxidation process (MW/H2O2-AOP) was used to treat separated solid dairy manure for nutrient release and solids reduction. The MW/H2O2-AOP was conducted at a microwave temperature of 120°C for 10 minutes, and at three pH conditions of 3.5, 7.3 and 12. The hydrogen peroxide dosage at approximately 2 mL per 1% TS for a 30 mL sample was used in this study, reflecting a range of 0.53–0.75 g H2O2/g dry sludge. The results indicated that substantial quantities of nutrients could be released into the solution at pH of 3.5. However, at neutral and basic conditions only volatile fatty acids and soluble chemical oxygen demand could be released. The analyses on orthophosphate, soluble chemical oxygen demands and volatile fatty acids were re-examined for dairy manure. It was found that the orthophosphate concentration for untreated samples at a higher % total solids (TS) was suppressed and lesser than actual. To overcome this difficulty, the initial orthophosphate concentration had to be measured at 0.5% TS. 相似文献
150.
Amjad A. Ahmad Ali Fares Sivapatham Paramasivam Moustafa A. Elrashidi Reza M. Savabi 《Journal of environmental science and health. Part. B》2013,48(7):742-754
Two field experiments were conducted at the Waimanalo research station on the island of O'ahu, Hawaii to study the effect of chicken (CM) and dairy (DM) manures on biomass and nutrient concentration in sweet corn roots and shoots. Sweet corn (super sweet 10, Zea Mays L. subsp. mays) was grown for two consecutive growing seasons under four rates of application (0, 168, 337, and 672 kg ha? 1 total N equivalent) and one time (OTA) or two time (TTA) applications of organic manure types and rates. There were significant effects of types, rates, and number of manure applications on dry biomass and macro- and micro-nutrient concentration in roots and shoots tissues. Results of root tissue indicated a significant accumulation of N and C under CM and DM treatments compared with the control treatment. Manure application rates significantly increased the accumulation of N and C in root tissue. Dry weight of roots and shoots and both macro- and micro-nutrient contents in the plant tissues significantly increased under TTA treatment compared with OTA treatment. There was a significant correlation (r2 = 0.46 to 0.81) between root biomass, macro-, and micro-nutrient contents during both growing seasons. The results of the study indicates that amending soils with CM at the highest application rate provided the best crop performance in terms of root and shoot biomass, crop N, C, and other macro- and micro-nutrients. 相似文献