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81.
Sulphate, Nitrogen and Base Cation Budgets at 21 Forested Catchments in Canada, the United States and Europe 总被引:1,自引:0,他引:1
Watmough SA Aherne J Alewell C Arp P Bailey S Clair T Dillon P Duchesne L Eimers C Fernandez I Foster N Larssen T Miller E Mitchell M Page S 《Environmental monitoring and assessment》2005,109(1-3):1-36
To assess the concern over declining base cation levels in forest soils caused by acid deposition, input-output budgets (1990s
average) for sulphate (SO4), inorganic nitrogen (NO3-N; NH4-N), calcium (Ca), magnesium (Mg) and potassium (K) were synthesised for 21 forested catchments from 17 regions in Canada,
the United States and Europe. Trend analysis was conducted on monthly ion concentrations in deposition and runoff when more
than 9 years of data were available (14 regions, 17 sites). Annual average SO4 deposition during the 1990s ranged between 7.3 and 28.4 kg ha−1 per year, and inorganic nitrogen (N) deposition was between 2.8 and 13.8 kg ha−1 per year, of which 41–67% was nitrate (NO3-N). Over the period of record, SO4 concentration in deposition decreased in 13/14 (13 out of 14 total) regions and SO4 in runoff decreased at 14/17 catchments. In contrast, NO3-N concentrations in deposition decreased in only 1/14 regions, while NH4-N concentration patterns varied; increasing at 3/14 regions and decreasing at 2/14 regions. Nitrate concentrations in runoff
decreased at 4/17 catchments and increased at only 1 site, whereas runoff levels of NH4-N increased at 5/17 catchments. Decreasing trends in deposition were also recorded for Ca, Mg, and K at many of the catchments
and on an equivalent basis, accounted for up to 131% (median 22%) of the decrease in acid anion deposition. Base cation concentrations
in streams generally declined over time, with significant decreases in Ca, Mg and K occurring at 8, 9 and 7 of 17 sites respectively,
which accounted for up to 133% (median 48%) of the decrease in acid anion concentration. Sulphate export exceeded input at
18/21 catchments, likely due to dry deposition and/or internal sources. The majority of N in deposition (31–100%; median 94%)
was retained in the catchments, although there was a tendency for greater NO3-N leaching at sites receiving higher (<7 kg ha-1 per year) bulk inorganic N deposition. Mass balance calculations show that export of Ca and Mg in runoff exceeds input at
all 21 catchments, but K export only exceeds input at 16/21 sites. Estimates of base cation weathering were available for
18 sites. When included in the mass balance calculation, Ca, Mg and K exports exceeded inputs at 14, 10 and 2 sites respectively.
Annual Ca and Mg losses represent appreciable proportions of the current exchangeable soil Ca and Mg pools, although losses
at some of the sites likely occur from weathering reactions beneath the rooting zone and there is considerable uncertainty
associated with mineral weathering estimates. Critical loads for sulphur (S) and N, using a critical base cation to aluminium
ratio of 10 in soil solution, are currently exceeded at 7 of the 18 sites with base cation weathering estimates. Despite reductions
in SO4 and H+ deposition, mass balance estimates indicate that acid deposition continues to acidify soils in many regions with losses of
Ca and Mg of primary concern.
The U.S. Government's right to retain a non-exclusive, royalty free licence in and to any copyright is acknowledged.
The Canadian Crown reserves the right to retain a non-exclusive, royalty free licence in and to any copyright. 相似文献
82.
Lake V?nern, the largest lake in Sweden, has been seriously contaminated with mercury during the 20th century. In the 1970's and 80's the direct load, mainly from a chlor-alkali industry in the area, of mercury was drastically reduced as a response to new legislation, from three to five tons down to between five and ten kg yr(-1). Large amounts of the disposed pollutant have accumulated in the sediments. The question posed in this work is now, is the effect of the drastic load reduction after more than two decades visible in the sediments? The question is relevant as large areas still are blacklisted for fishing, but also as a follow-up of a major remedy action. The lake also serves as a freshwater reservoir for even Sweden's second largest city. This work synthesises and compares data of mercury in the sediments from three major field programs, in 1974, 1984 and 1998. The interest is focused on both spatial heterogeneity and temporal trends. In 1974, the surface concentrations are significantly higher than in subsequent surveys. Significant differences are also found between 1984 and 1998. Significant spatial differences within the lake are found for respective year. The most contaminated area is located in the north, close to the major point source (a former chlor-alkali industry). This is also the area with the largest improvement, as a direct response to the reduction in load. Further from the outlet, the recovery is more affected by burial and transport processes out into the deeper basins. 相似文献
83.
Kimpo metropolitan landfill has received various kinds of wastessince January 1992. The leachate level was measured to be 10.3 m in May 1995 and the level increased to 12.2 m in August 1996. Therefore, to prove the reason for the increasing leachate level, we calibrated hydraulic conductivity of each waste andintermediate layer using the HELP (Hydrologic Evaluation ofLandfill Performance) model. The leachate generation data measured from February 1993 to October 1995 was used in the model calibration. As a result of a model calibration, we obtained anaverage infiltration ratio and used this in analysis of the total water balance to predict elevation of leachate level. Main causes of the elevation of the leachate level were the high water content of the waste and the degradation of the leachate-drainage system caused by the subsidence of a naturalbarrier layer. 相似文献
84.
博乐市空气质量变化趋势分析 总被引:2,自引:0,他引:2
分析了博乐市2001-2005年空气质量监测数据在不同月份、不同年份、不同污染因子的变化趋势,并结合当地能源结构、地理位置、气候特征、城市环境综合发展水平。指出影响博乐市空气质量的主要因素,为防治或减轻博乐地区的空气污染提供了科学依据。 相似文献
85.
博斯腾湖水质矿化度模型及预测研究 总被引:6,自引:0,他引:6
根据博斯腾湖1985~1995年水质监测数据和出入湖水量等水文数据观测值,采用水质扩散模型和盐量平衡关系推导出博斯腾湖大湖区(简称博湖)水质矿化度模型,并预测了几种情况下博湖水质矿化度及近几年变化趋势,分析了影响博湖水质矿化度的主要因素,为博湖的近期和远期环境保护规划、环境管理等提供科学依据. 相似文献
86.
用StrandenE.推荐的测量方法对哈密地区环境空气中220Rn子体α潜能浓度测量结果表明,室内、外平均值分别为56.1和10.2(×10-7J·m-3)。室内外220Rn/222Rn子体α潜能浓度比值分别为0.84和032。220Rn子体所致居民有效剂量当量为228μSv·a-1(集体有效剂量当量为0.9×02man·Sv)。 相似文献
87.
对北京中央电视塔周围25 km2区域电磁环境质量分别进行了射频的网格法手工监测和车载巡测自动监测,通过SPSS软件等对两种监测方法获取的数据进行了统计对比分析,发现两组数据在总体水平及数值分布特征上较为接近,因此车载巡测监测可以替代网格法监测。以车载巡测数据为基础,绘制了实测数据的道路电磁地图,利用插值法绘制了区域电磁地图,对区域电磁环境质量进行了直观表征。从回应公众关注和城市电磁规划出发,建议今后可利用车载巡测监测加强时域和频域的监测。 相似文献
88.
89.
90.
J. Franzaring 《Environmental monitoring and assessment》1997,46(3):209-220
Up to now only very few studies in biomonitoring of organic air pollutants have been published taking into account the strong influence mean temperatures have on the accumulation process into plants during the course of the exposition. Temperature governed sorption as well as the plants vitality pose a major source of uncertainty making inter-study comparisons difficult. Different surface-to-volume ratios of plant foliage lead to strongly varying concentration effects in different plant species. Moreover a plants content of waxes and lipids must be considered in order to relate xenobiotic concentrations to the compounds being most efficient in the bioaccumulation process. Some of these factors are evaluated in regard to the use of plants as biomonitors for organic air pollutants. Another aim is to deduce the mean ambient gas phase concentrations from PAH concentrations determined in the biomonitor plants using vegetation-air partitioning coefficients which have been corrected for temperature dependent sorption as well as the plants lipid content. Restrictions of such approaches and methods of biomonitoring in general are discussed. 相似文献