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901.
902.
Antonius Indarto Jae-Wook Choi Hwaung Lee Hyung Keun Song 《International Journal of Green Energy》2013,10(3):309-321
Decomposition of dichloromethane (CH2Cl2) using a gliding plasma was examined and reported in this paper. The effects of initial concentrations of CH2Cl2, total gas flow rates, and input frequency have been studied to evaluate the performance of gliding arc on CH2Cl2 decomposition. Using atmospheric pressure air as the carrier gas, experimental results indicate that the maximum conversion of CH2Cl2 was 95.1% at a total gas flow rate of 180 L/hr containing 1% by volume of CH2Cl2. The reaction occurred at an exothermic condition and gaseous products are dominated by CO, CHCl3, and Cl2. CO2 and CCl4 are also detected in the product stream in small amounts. The conversion of CH2Cl2 increases with the increasing applied voltage and decreasing total gas flow rate. 相似文献
903.
Carbon dioxide is the major greenhouse gas responsible for global warming. Man-made CO2 emissions contribute approximately 63% of greenhouse gases and the cement industry is responsible for approximately 5% of CO2 emissions emitting nearly 900 kg of CO2 per 1000 kg of cement. CO2 from a cement plant was captured and purified to 98% using the monoethanolamine (MEA) based absorption process. The capture cost was $51 per tonne of CO2 captured, representing approximately 90% of total cost. Steam was the main operating cost representing 39% of the total capture cost. Switching from coal to natural gas reduces CO2 emissions by about 18%. At normal load, about 36 MW of waste heat is available for recovery to satisfy the parasitic heat requirements of MEA process; however, it is very difficult to recover. 相似文献
904.
《International Journal of Green Energy》2013,10(2):217-231
This article is concerned with control issues related to the design of a semi-closed O 2/CO 2 gas turbine cycle for CO 2 capture. Some control strategies and their interaction with the process design are discussed. One control structure is implemented on a dynamic simulation model using a predictive controller, and simulations assess the performance and compare its merits with a conventional PI structure. The results indicate that it can be advantageous for operability to allow a varying (as opposed to fixed) compressor inlet pressure, at the cost of a more expensive design. Furthermore, the results show that a predictive controller has some advantages with respect to the simpler conventional PI control structure, in particular in terms of constraint handling. 相似文献
905.
Summary The balance of evidence suggests a perceptible human influence on global ecosystems. Human activities are affecting the global
ecosystem, some directly and some indirectly. If researchers could clarify the extent to which specific human activities affect
global ecosystems, they would be in a much better position to suggest strategies for mitigating against the worst disturbances.
Sophisticated statistical analysis can help in interpreting the influence of specific human activities on global ecosystems
more carefully. This study aims at identifying significant or influential human activities (i.e. factors) on CO2 emissions using statistical analyses. The study was conducted for two cases: (i) developed countries and (ii) developing
countries. In developed countries, this study identified three influential human activities for CO2 emissions: (i) combustion of fossil fuels, (ii) population pressure on natural and terrestrial ecosystems, and (iii) land
use change. In developing countries, the significant human activities causing an upsurge of CO2 emissions are: (i) combustion of fossil fuels, (ii) terrestrial ecosystem strength and (iii) land use change. Among these
factors, combustion of fossil fuels is the most influential human activity for CO2 emissions both in developed and developing countries. Regression analysis based on the factor scores indicated that combustion
of fossil fuels has significant positive influence on CO2 emissions in both developed and developing countries. Terrestrial ecosystem strength has a significant negative influence
on CO2 emissions. Land use change and CO2 emissions are positively related, although regression analysis showed that the influence of land use change on CO2 emissions was still insignificant. It is anticipated, from the findings of this study, that CO2 emissions can be reduced by reducing fossil-fuel consumption and switching to alternative energy sources, preserving exiting
forests, planting trees on abandoned and degraded forest lands, or by planting trees by social/agroforestry on agricultural
lands. 相似文献
906.
Model‐Based Nitrogen and Phosphorus (Nutrient) Criteria for Large Temperate Rivers: 2. Criteria Derivation 下载免费PDF全文
Michael W. Suplee Kyle F. Flynn Steven C. Chapra 《Journal of the American Water Resources Association》2015,51(2):447-470
Nitrogen and phosphorus criteria were developed for 233 km of the Yellowstone River, one of the first cases where a mechanistic model has been used to derive large river numeric nutrient criteria. A water quality model and a companion model which simulates lateral algal biomass across transects were used to simulate effects of increasing nutrients on five variables (dissolved oxygen, total organic carbon, total dissolved gas, pH, and benthic algal biomass in depths ≤1 m). Incremental increases in nutrients were evaluated relative to their impact on predefined thresholds for each variable; the first variable to exceed a threshold set the nutrient criteria. Simulations were made at a low flow, the 14Q5 (lowest average 14 consecutive day flow, July‐September, recurring one in five years), which was derived using benthic algae growth curves and EPA guidance on excursion frequency. An extant climate dataset with an annual recurrence was used, and tributary water quality and flows were coincident with the river's 10 lowest flow years. The river had different sensitivities to nutrients longitudinally, pH being the most sensitive variable in the upstream reach and algal biomass in the lower. Model‐based criteria for the Yellowstone River are as follows: between the Bighorn and Powder river confluences, 55 μg TP/l and 655 μg TN/l; from the Powder River confluence to Montana state line, 95 μg TP/l and 815 μg TN/l. Pros and cons of using steady‐state models to derive river nutrient criteria are discussed. 相似文献
907.
908.
《环境科学学报(英文版)》2023,35(7):152-160
Urea oxidation reaction (UOR) provides a method for hydrogen production besides wastewater treatment, but the current limited catalytic activity has prevented the application. Herein, we develop a novel H2O2 treatment strategy for tailoring the surface oxygen ligand of NiFe-layered double hydroxides (NiFe-LDH). The sample after H2O2 treatment (NiFeO-LDH) shows significant enhancement on UOR efficiency, with the potential of 1.37 V (RHE) to reach a current density of 10 mA/cm2. The boost is attributed to the richness adsorption O ligand on NiFeO-LDH as revealed by XPS and Raman analysis. DFT calculation indicates formation of two possible types of oxygen ligands: adsorbed oxygen on the surface and exposed from hydroxyl group, lowered the desorption energy of CO2 product, which lead to the lowered onset potential. This strategy is further extended to NiFe-LDH nano sheet on Ni foam to reach a higher current density of 440 mA/cm2 of UOR at 1.8 V (RHE). The facile surface O ligand manipulation is also expected to give chance to many other electro-catalytic oxidations. 相似文献
909.
910.