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201.
F. Benoit-Marquié C. de Montety V. Gilard R. Martino M. T. Maurette M. Malet-Martino 《Environmental Chemistry Letters》2004,2(2):93-97
We studied the hydrolysis and TiO2 photocatalysis of the pesticide dichlorvos at pH 2.6–9 using phosphorus-31 nuclear magnetic resonance (31P NMR). We found that the hydrolysis of dichlorvos led to the formation of dimethyl phosphate at pH 5.6–9. On the other hand, TiO2 photocatalysis decomposed dichlorvos into dimethyl phosphate, which further reacted to form monomethyl phosphate at pH 2.6 and 9. Monomethylphosphate was hydrolysed into phosphate at pH 2.6. 31P NMR is therefore a promising tool to study the degradation of organophosphorus pesticides. 相似文献
202.
利用大气污染源和环境质量监测等资料,计算分析了锦州市区大气污染现状。结果表明:在锦州市区空气污染以煤烟类为主,汽车尾气成为大气污染源之一。PM10和SO2超过二级标准的天数将近95%出现在采暖期。提出了可行的具体措施,指出采用以集中供热、推广使用天然气、小型锅炉改造工程和控制汽车尾气为主要措施,廉顾绿化,制定市区大气污染治理方案比较合理。 相似文献
203.
Fearnside Philip M. Lashof Daniel A. Moura-Costa Pedro 《Mitigation and Adaptation Strategies for Global Change》2000,5(3):239-270
Many proposed activities formitigating global warming in the land-use change and forestry(LUCF) sector differ from measures to avoid fossilfuel emissions because carbon (C) may be held out ofthe atmosphere only temporarily. In addition, thetiming of the effects is usually different. Many LUCFactivities alter C fluxes to and from the atmosphereseveral decades into the future, whereas fossil fuelemissions avoidance has immediate effects. Non-CO2 greenhouse gases (GHGs), which are animportant part of emissions from deforestation inlow-latitude regions, also pose complications forcomparisons between fossil fuel and LUCF, since themechanism generally used to compare these gases(global warming potentials) assumes simultaneousemissions. A common numeraire is needed to expressglobal warming mitigation benefits of different kindsof projects, such as fossil fuel emissions reduction,C sequestration in forest plantations, avoideddeforestation by creating protected areas and throughpolicy changes to slow rates of land-use changes suchas clearing. Megagram (Mg)-year (also known as`ton-year') accounting provides a mechanism forexpressing the benefits of activities such as these ona consistent basis. One can calculate the atmosphericload of each GHG that will be present in each year,expressed as C in the form of CO2 and itsinstantaneous impact equivalent contributed by othergases. The atmospheric load of CO2-equivalent Cpresent over a time horizon is a possible indicator ofthe climatic impact of the emission that placed thisload in the atmosphere. Conversely, this index alsoprovides a measure of the benefit of notproducing the emission. One accounting methodcompares sequestered CO2 in trees with theCO2 that would be in the atmosphere had thesequestration project not been undertaken, whileanother method (used in this paper) compares theatmospheric load of C (or equivalent in non-CO2GHGs) in both project and no-project scenarios.Time preference, expressed by means of a discount rateon C, can be applied to Mg-year equivalencecalculations to allow societal decisions regarding thevalue of time to be integrated into the system forcalculating global warming impacts and benefits. Giving a high value to time, either by raising thediscount rate or by shortening the time horizon,increases the value attributed to temporarysequestration (such as many forest plantationprojects). A high value for time also favorsmitigation measures that have rapid effects (such asslowing deforestation rates) as compared to measuresthat only affect emissions years in the future (suchas creating protected areas in countries with largeareas of remaining forest). Decisions on temporalissues will guide mitigation efforts towards optionsthat may or may not be desirable on the basis ofsocial and environmental effects in spheres other thanglobal warming. How sustainable development criteriaare incorporated into the approval and creditingsystems for activities under the Kyoto Protocol willdetermine the overall environmental and social impactsof pending decisions on temporal issues. 相似文献
204.
205.
Will Simplified Modalities and Procedures Make More Small-Scale Forestry Projects Viable Under the Clean Development Mechanism? 总被引:2,自引:0,他引:2
Bruno Locatelli Lucio Pedroni 《Mitigation and Adaptation Strategies for Global Change》2006,11(3):621-643
Simplified modalities and procedures (M&P) are expected to increase the viability of small-scale project activities under
the Clean Development Mechanism (CDM). A small-scale afforestation or reforestation (AR) project is defined as a project removing
less than 8 kilotons of carbon dioxide equivalent (CO2e) per year. Depending on the project type and the method for measuring scale, 8 kilotons of CO2e per year correspond to highly diverse areas, possibly ranging from 200 to 6000 ha. Using a model to calculate the minimum
project scale above which the CDM is a positive financial incentive for eligible AR project activities, the paper analyzes
whether a reduction of transaction costs under simplified M&P will be a sufficient incentive to motivate small-scale participation
in the CDM. Model results show that, even under optimistic assumptions on carbon market conditions and transaction costs,
small-scale project activities will not benefit from simplified M&P. Results also show that project activities removing more
than 8 kilotons of CO2e per year and registered as small-scale would be the ones that could benefit the most from simplified M&P. It is concluded
that the participation of small-scale project activities to the CDM requires more than simplified M&P, the price of expiring
Certified Emission Reductions being one of the most critical parameters. 相似文献
206.
Based on hourly measurements of NOx NO2 and O3 and meteorological data, an ordinary least squares (OLS) model and a first-order autocorrelation (AR) model were developed to analyse the regression and prediction of NOx and NO2 concentrations in London. Primary emissions and wind speed are the most important factors influencing NOx concentrations; in addition to these two, reaction of NO with O3 is also a major factor influencing NO2 concentrations. The AR model resulted in high correlation coefficients (R > 0.95) for the NOx and NO2 regression based on a whole year's data, and is capable of predicting NO2 (R = 0.83) and NOx (R = 0.65) concentrations when the explanatory variables were available. The analysis of the structure of regression models by Principal Component Analysis (PCA) indicates that the regression models are stable. The results of the OLS model indicate that there was an exceptional NO2 source, other than primary emission and reaction of NO with O3, in the air pollution episode in London in December 1991. 相似文献
207.
208.
209.
新型二氧化铅电极处理有机染料废水的研究 总被引:6,自引:0,他引:6
研究了高压塑片法制备新型二氧化铅电极的工艺,通过循环伏安、X衍射和扫描电镜等手段对电极性能的考察表明,该电极不仅具有高电催化活性,还有很好的抗腐蚀性能.通过与普通石墨电极的对比实验,进一步探讨了该电极降解中性枣红染料的机制和工艺条件.结果表明,该电极在脱色和COD降解方面都有明显的优越性.在含磷酸盐和氯离子的体系中,降解效率尤为突出. 相似文献
210.
通过比较二氧化硫测定值与紫外灯强度、紫外检测器调节值及光电倍增管高压值的关系,提出二氧化硫测定值与紫外灯强度、光电倍增管高压值成正比,与紫外检测调节值成反比的结论,并对仪器校准提出了有效性建议。 相似文献