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1.
The vertical distribution of the 236U/238U isotopic ratio was investigated in soil samples from three different locations on La Palma (one of the seven Canary Islands, Spain). Additionally the 240Pu/239Pu atomic ratio, as it is a well establish tool for the source identification, was determined. The radiochemical procedure consisted of a U separation step by extraction chromatography using UTEVA® Resin (Eichrom Technologies, Inc.). Afterwards Pu was separated from Th and Np by anion exchange using Dowex 1x2 (Dow Chemical Co.). Furthermore a new chemical procedure with tandem columns to separate Pu and U from the matrix was tested. For the determination of the uranium and plutonium isotopes by alpha spectrometry thin sources were prepared by microprecipitation techniques. Additionally these fractions separated from the soil samples were measured by Accelerator Mass Spectrometry (AMS) to get information on the isotopic ratios 236U/238U, 240Pu/239Pu and 236U/239Pu, respectively. The 236U concentrations [atoms/g] in each surface layer (∼2 cm) were surprisingly high compared to deeper layers where values around two orders of magnitude smaller were found. Since the isotopic ratio 240Pu/239Pu indicated a global fallout signature we assume the same origin as the probable source for 236U. Our measured 236U/239Pu value of around 0.2 is within the expected range for this contamination source. 相似文献
2.
Spatial distribution of 238U and 226Ra activities in sediment columns along the Krka River and estuary, were studied using gamma spectrometry. Markedly different 238U and 226Ra activities between riverine, estuarine and marine sediments were observed. Distribution of these radionuclides, as well as their anthropogenic and natural origin, was evaluated by activity measurements, taking into account sedimentation rates estimated by 137Cs distribution in sediment columns. 相似文献
3.
Environmental 238U and 232Th concentration measurements in an area of high level natural background radiation at Palong, Johor, Malaysia 总被引:1,自引:0,他引:1
Concentrations of uranium-238 and thorium-232 in soil, water, grass, moss and oil-palm fruit samples collected from an area of high background radiation were determined using neutron activation analysis (NAA). U-238 concentration in soil ranged from 4.9 mg kg(-1) (58.8 Bq kg(-1)) to 40.4 mg kg(-1) (484.8 Bq kg(-1)), Th-232 concentration ranged from 14.9 mg kg(-1) (59.6 Bq kg(-1)) to 301.0 mg kg(-1) (1204 Bq kg(-1)). The concentration of U-238 in grass samples ranged from below the detection limit to 0.076 mg kg(-1) (912 mBq kg(-1)), and Th-232 ranged from 0.008 mg kg(-1) (32 mBq kg(-1)) to 0.343 mg kg(-1) (1.372 Bq kg(-1)). U-238 content in water samples ranged from 0.33 mg kg(-1) (4.0 Bq L(-1)) to 1.40 mg kg(-1) (16.8 Bq L(-1)), and Th-232 ranged from 0.19 mg kg(-1) (0.76 Bq L(-1)) to 0.66 mg kg(-1) (2.64 Bq L(-1)). It can be said that the concentrations of environmental U-238 and Th-232 in grass and water samples in the study area are insignificant. Mosses were found to be possible bio-radiological indicators due to their high absorption of the heavy radioelements from the environment. 相似文献
4.
Arbuscular mycorrhizal fungi can decrease the uptake of uranium by subterranean clover grown at high levels of uranium in soil 总被引:7,自引:0,他引:7
Rufyikiri G Huysmans L Wannijn J Van Hees M Leyval C Jakobsen I 《Environmental pollution (Barking, Essex : 1987)》2004,130(3):427-436
Subterranean clover inoculated or not with the arbuscular mycorrhizal (AM) fungus Glomus intraradices was grown on soil containing six levels of 238U in the range 0-87 mg kg(-1). Increasing U concentration in soil enhanced the U concentration in roots and shoots of both mycorrhizal and nonmycorrhizal plants but had no significant effects on plant dry matter production or root AM colonization. Mycorrhizas increased the shoot dry matter and P concentration in roots and shoots, while in most cases, it decreased the Ca, Mg and K concentrations in plants. The AM fungus influenced U concentration in plants only in the treatment receiving 87 mg U kg(-1) soil. In this case, U concentration in shoots of nonmycorrhizal plants was 1.7 times that of shoots of mycorrhizal plants. These results suggested that mycorrhizal fungi can limit U accumulation by plants exposed to high levels of U in soil. 相似文献
5.
以西南某低放废物处置库地质环境中板岩和土壤介质为研究对象,开展了238U和239Pu核素在这两种地质介质中的动态迁移实验研究,通过氚穿透实验(地下水流速=1 mL.min-1、实验柱连续淋洗时间=180 d)得到氚在板岩中的弥散系数DL为0.027 cm2.min-1,弥散度αL为0.324 cm,在土壤中的弥散系数DL为0.064 cm.2min-1,弥散度αL为0.895 cm.通过淋滤实验(地下水流速=0.1 mL.h-1、实验柱连续淋洗时间=350 min),得到了238U在板岩和土壤介质中的迁移速度分别为6.1—8.1 cm.a-1和7.3—8.5 cm.a-1,239Pu在板岩和土壤介质中的迁移速度分别为4.1—6.1 cm.a-1和3.7—4.9 cm.a-1. 相似文献
6.
Some important naturally occurring α- and β-radionuclides in drinking water samples collected in Italy were determined and the radiological quality evaluated. The mean activity concentrations (mBq L−1) of the radionuclides in the water samples were almost in the order: 26 ± 36 (234U) > 21 ± 30 (238U) > 8.9 ± 15 (226Ra) > 4.8 ± 6.3 (228Ra) > 4.0 ± 4.1 (210Pb) > 3.2 ± 3.7 (210Po) > 2.7 ± 1.2 (212Pb) > 1.4 ± 1.8 (224Ra) > 1.1 ± 1.3 (235U) > 0.26 ± 0.39 (228Th) > 0.0023 ± 0.0009 (230Th) > 0.0013 ± 0.0006 (232Th). The mean estimated dose (μSv yr−1) to an adult from the water intake was in this order: 2.8 ± 3.3 (210Po) > 2.4 ± 3.2 (228Ra) > 2.1 ± 2.1 (210Pb) > 1.8 ± 3.1 (226Ra) > 0.94 ± 1.30 (234U) > 0.70 ± 0.98 (238U) > 0.069 ± 0.087 (224Ra) > 0.036 ± 0.044 (235U) > 0.014 ± 0.021 (228Th) > 0.012 ± 0.005 (212Pb) > 0.00035 ± 0.00029 (230Th) > 0.00022 ± 0.00009 (232Th). It is obvious that 210Po, 228Ra, 210Pb and 226Ra are the most important dose contributors in the drinking water intake. As far as the seventeen brands of analysed drinking water were concerned, the committed effective doses were in the range of 2.81–38.5 μSv yr−1, all well below the reference level of the committed effective dose (100 μSv yr−1) recommended by the WHO. These data throw some light on the scale of the radiological impact on the public from some naturally occurring radionuclides in drinking water, and can also serve as a comparison for the dose contribution from artificial radionuclides released to the environment as a result of human practices. Based on the radionuclide composition in the analysed waters, comment was made on the new screening level for gross α activity in guidelines for drinking-water quality recommended by the WHO, 2004. 相似文献
7.
F. Gharbi S. Baccouche W. Abdelli M. Samaali M. Oueslati A. Trabelsi 《Journal of environmental radioactivity》2010,101(8):589-590
234U and 238U activity concentrations and their relative effective doses have been determined in 10 bottled mineral waters in Tunisia. Alpha spectrometry was used as technique to measure uranium isotopes. The obtained isotopic ratio 234U/238U varies between 1.1 and 3 which means that the two isotopes are not in radioactive equilibrium. Measured activity concentration varies between 3.2 and 40 mBq/l for 234U and between 1.5 and 26.3 mBq/l for 238U. Effective doses (assuming 2 litres per day of water consumption) coming from this two isotopes are found to vary between 0.16 and 2.02 μSv/a which is lower than the maximum recommended dose level by the WHO. 相似文献
8.
Samples from a marine sediment core from the Irish Sea (54.416 N, 3.563 W) were analyzed for the isotopic composition of uranium, plutonium and americium by a combination of radiometric methods and AMS. The radiochemical procedure consisted of a Pu separation step by anion exchange, subsequent U separation by extraction chromatography using UTEVA® and finally Am separation with TRU® Resin.Additionally to radiometric determination of these isotopes by alpha spectrometry, the separated samples were also used for the determination of 236U/238U and plutonium isotope ratios by Accelerator Mass Spectrometry (AMS) at the VERA facility. 相似文献
9.
Jha SK Gothankar S Iongwai PS Kharbuli B War SA Puranik VD 《Journal of environmental radioactivity》2012,103(1):1-6
The concentration of naturally occurring radionuclides 232Th, 238U was determined using Instrumental Neutron Activation Analysis (INAA) in different food groups namely cereals, vegetables, leafy vegetables, roots and tubers cultivated and consumed by tribal population residing around the proposed uranium mine. The study area is a part of rural area K. P. Mawthabah (Domiasiat) in the west Khasi Hills District of Meghalaya, India located in the tropical region of high rainfall that remains steeped in tribal tradition without much outside influence. Agriculture by Jhum (slash and burn) cultivation and animal husbandry are the main occupation of the tribal populations. A total of 89 samples from locally grown food products were analyzed. The concentration of 238U and 232Th in the soil of the study area was found to vary 1.6-15.5 and 2.0-5.0 times respectively to the average mean value observed in India. The estimated daily dietary intake of 238U and 232Th were 2.0 μg d−1 (25 mBq d−1) and 3.4 μg d−1 (14 mBq d−1) is comparable with reported range 0.5-5.0 μg d−1 and 0.15-3.5 μg d−1 respectively for the Asian population. 相似文献
10.
本文对近年文献报导中水、食品和人体中的~(234)U和~(238)U含量,比活度比值的调查结果,并估算出了人体所受的内照射剂量,作了评述,引用文献19篇,表格14张. 相似文献