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1.
Carbon coated monolith was prepared by sucrose solution 65 wt.% via dip-coating method. Sulfonation of incomplete carbonized carbon coated monolith was carried out in order to synthesize solid acid catalyst. The textural structure characteristics of the solid acid catalyst demonstrated a low surface area and pore volume. Palm fatty acid distillate (PFAD), a by-product of palm oil refineries, was utilized as oil source in biodiesel production. The esterification reaction subjected to different reaction conditions was performed by using the sulfonated carbon coated monolith as heterogeneous catalyst. The sulfonation process had been performed by using vapour of concentrated H2SO4 that was much easier and efficient than liquid phase sulfonation. Total acidity value of carbon coated monolith was measured for unsulfonated sample (0.5 mmol/g) and sulfonated sample (4.2 mmol/g). The effect of methanol/oil ratio, catalyst amount and reaction time were examined. The maximum methyl ester content was 89% at the optimum condition, i.e. methanol/oil molar ratio (15:1), catalyst amount (2.5 wt.% with respect to PFAD), reaction time (240 min) and temperature 80 °C. The sugar catalyst supported on the honeycomb monolith showed comparable reactivity compared with the sugar catalyst powder. However, the catalyst reusability studies showed decrease in FFA% conversion from 95.3% to 68.8% after four cycles as well as the total acidity of catalyst dropped from the value 4.2 to 3.1 mmol/g during these cycles. This might be likely due to the leaching out of SO3H group from the sulfonated carbon coated monolith surface. The leaching of active species reached a plateau state after fourth cycle. 相似文献
2.
本文通过对影响街道空气中一氧化碳污染的因素进行了大量的监测及综合分析,找出乌鲁木齐市主要街道空气中一氧化碳的污染规律,为控制我市汽车污染提供科学依据. 相似文献
3.
4.
城市高架道路建设对机动车尾气污染的影响分析 总被引:3,自引:0,他引:3
通过现场观测和对比,分析了城市一般道路上和城市高架道路下机动车排放污染物浓度差异的原因,分析结果表明,扩散条件对城市机动车尾气污染有着重要影响,例举日本对城市高架道路建设的有关规定,提出应重视城市高架道路建设的环境预评估等。 相似文献
5.
煤烟型大气污染解决方法 总被引:3,自引:0,他引:3
重点介绍了新型燃煤工艺——水平火焰无烟工业炉及其特点,并提出排烟尾气处理的资源化方案。 相似文献
6.
Developing Canada's National Forest Carbon Monitoring, Accounting and Reporting System to Meet the Reporting Requirements of the Kyoto Protocol 总被引:2,自引:0,他引:2
The rate of carbon accumulation in the atmosphere can be reduced by decreasing emissions from the burning of fossil fuels
and by increasing the net uptake (or reducing the net loss) of carbon in terrestrial (and aquatic) ecosystems. The Kyoto Protocol
addresses both the release and uptake of carbon. Canada is developing a National Forest Carbon Monitoring, Accounting and
Reporting System in support of its international obligations to report greenhouse gas sources and sinks. This system employs
forest-inventory data, growth and yield information, and statistics on natural disturbances, management actions and land-use
change to estimate forest carbon stocks, changes in carbon stocks, and emissions of non-CO2 greenhouse gases. A key component of the system is the Carbon Budget Model of the Canadian Forest Sector (CBM-CFS). The model
is undergoing extensive revisions to enable analyses at four spatial scales (national, provincial, forest management unit
and stand) and in annual time steps. The model and the supporting databases can be used to assess carbon-stock changes between
1990 and the present, and to predict future carbon-stock changes based on scenarios of future disturbance rates and management
actions. 相似文献
7.
根据炭黑疏水性的特点 ,本试验采用油团聚工艺成功地处理了炭黑废水。经处理后 ,出水中炭黑含量小于 5.0 mg/ L,出水可回用 ,回收的炭黑用四氯化碳处理后 ,经过滤干燥可得到含水率小于 1 .0 %的炭黑 ,油相可回用。 相似文献
8.
水量衡算条件下人工湿地对有机物的去除研究 总被引:1,自引:0,他引:1
构建了芦苇和无植物2种人工湿地,在系统水量衡算的基础上比较了2种湿地对生活污水中有机物的去除效果。结果证明,在植物收割后的冬季,芦苇湿地对有机物的去除率低于无植物湿地系统约2%;在其他季节,芦苇湿地对污水CODcr的去除率比无植物湿地高出3.3%-5%。但对BOD5的去除率却比无植物湿地低了1.9%-2.7%。因此,芦苇湿地对有机物的去除效果比无植物湿地高,但提高不多。比较了2种系统的氧化还原电位,芦苇湿地比无植物湿地的高(P〈0.05),这种提高主要集中在湿地水面以下约10cm的深度;从整个湿地床体来看。2块连续运行的潜流水平湿地内部氧化还原状态大部分相同。主要是厌氧状态。比较了2种人工湿地基质中降解有机物的细菌,放线菌和真菌的数量,二者没有明显的差别。考察了湿地进水有机负荷与去除量的关系,二者呈现显著的线性相关性(R^2〉0.99)。 相似文献
9.
The Kyoto Protocol is the first step towards achieving the objectives of the United Nations Framework Convention on Climate Change and aims among others to promote ‘the protection and enhancement of carbon sinks and reservoirs’. To encourage afforestation for carbon sequestration a project must be economically viable. This study uses a model to analyse the impact on project viability of a range of carbon monitoring options, international carbon credit value and discount rate, applied to a Pinus radiata afforestation project in New Zealand. Monitoring carbon in conjunction with conventional forest inventory shows the highest return. Long-term average carbon accounting has lower accounting costs, compared to annual and 5 yearly accounting, as monitoring is only required every 5–10 years until the long-term average is attained. In this study we conclude that monitoring soil carbon stocks is not economically feasible using any of the accounting methods, when carbon is valued at US$ 10/t. This conclusion may be relevant to forest carbon sequestration projects elsewhere in the world and suggests care is needed in selecting the appropriate carbon monitoring options to avoid the risk that costs could be higher than any monetary benefits from terrestrial carbon sequestration. This would remove any commercial incentive to afforest for carbon sequestration reasons and severely limit the use of forest sinks as part of any package of measures addressing the ultimate objective of the UNFCCC. 相似文献
10.
《环境科学学报(英文版)》2023,35(3):831-842
This study represents the first quantitative evaluation of pollution transport budget within the boundary layer of typical cities in the Beijing-Tianjin-Hebei (BTH) region from the perspective of horizontal and vertical exchanges and further discusses the impact of the atmospheric boundary layer (ABL)-free troposphere (FT) exchange on concentration of fine particulate matter (PM2.5) within the ABL during heavy pollution. From the perspective of the transport flux balance relationship, differences in pollution transport characteristics between the two cities is mainly reflected in the ABL-FT exchange effect. The FT mainly flowed into the ABL in BJ, while in SJZ, the outflow from the ABL to the FT was more intense. Combined with an analysis of vertical wind profile distribution, BJ was found to be more susceptible to the influence of northwest cold high prevailing in winter, while sinking of strong cold air allowed the FT flowing into the ABL influence the vertical exchange over BJ. In addition, we selected a typical pollution event for targeted analysis to understand mechanistic details of the influence of ABL-FT exchange on the pollution event. These results showed that ABL-FT interaction played an important role in PM2.5 concentration within the ABL during heavy pollution. Especially in the early stage of heavy pollution, FT transport contributed as much as 82.74% of PM2.5 within the ABL. These findings are significant for improving our understanding of pollution transport characteristics within the boundary layer and the effect of ABL-FT exchange on air quality. 相似文献