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891.
Since 1972, at the University of Hohenheim in Stuttgart, Germany, airborne particulate matter (PM12 and then PM10) was continuously collected on filters and analyzed for environmentally relevant elements by X-ray fluorescence analysis. The resulting long-term time series are suitable for the investigation of trends and of seasonal variation. For the period 1972-2005, monthly and annual concentration mean values of 13 elements (Br, Ca, Cr, Cu, Fe, K, Mn, Ni, Pb, S, Ti, V, and Zn) in the air are presented. Trend curves were fitted and the mean yearly variation of the concentration for these elements was calculated and represented graphically. All trend curves show a diminution of the air pollution during this period, but to different extents. Mean trends in percent per year were calculated for each element both for the entire investigation period and for three data subsets of 10-11 years. Possible explanations are discussed in detail. 相似文献
892.
Fernandez C Monna F Labanowski J Loubet M van Oort F 《Environmental pollution (Barking, Essex : 1987)》2008,156(3):1083-1091
The role of land use on fate of metals in soils is poorly understood. In this work, we studied the incorporation of lead in two neighboring soils with comparable pedogenesis but under long-term different agricultural management. Distributions of anthropogenic Pb were assessed from concentrations and isotopic compositions determined on bulk horizon samples, systematical 5-10 cm increment samples, and on 24-h EDTA extracts. Minor amounts of anthropogenic lead were detected until 1-m depth under permanent grassland, linked to high earthworm activity. In arable land, exogenous Pb predominantly accumulated at depths <60 cm. Although the proximity between the two sites ensured comparable exposition regarding atmospheric Pb deposition, the isotopic compositions clearly showed the influence of an unidentified component for the cultivated soil. This work highlights the need for exhaustive information on historical human activities in such anthropized agrosystems when fate of metal pollution is considered. 相似文献
893.
Pei Gu Ren Fang Shen Yi Ding Chen 《Environmental science and pollution research international》2008,15(3):273-277
BACKGROUND: The Yangtze Delta is one of the most developed regions in China and includes Shanghai, eight cities in Jiangsu province and eight cities in Zhejiang province. Meat consumption in this region has increased with economic growth, and most of the consumed meat is produced locally. The water quality of surface waters has deteriorated in recent years. An example was the huge blue-green algae bloom in Tai Lake in late May 2007, which affected millions of people's daily drinking water. However, animal husbandry is considered to be one of the main pollution sources. METHODS: Pollutants (NH3-N, total phosphorus (TP), and total nitrogen (TN)) excreted by livestock and poultry, and the resultant COD (chemical oxygen demand) and BOD (biochemical oxygen demand), were estimated using two different methods based on different data sets. RESULTS: The number of livestock and poultry has remained stable in the Yangtze Delta over the four years from 1999 to 2002, with the average number of pigs, cattle, sheep and poultry being 21.1 M, 0.4 M, 7.7 M and 597.6 M, respectively. Pollutants in livestock and poultry excreta estimated by Method I were: 0.12 Mt NH3-N, 0.11 Mt TP and 0.29 Mt TN, resulting in COD and BOD of 1.34 Mt and 1.30 Mt, respectively, while the estimations based on Method II were: 0.18 Mt NH3-N, 0.15 Mt TP and 0.40 Mt TN, resulting in COD and BOD of 1.95 Mt and 1.80 Mt, respectively. DISCUSSION: Pollutants excreted annually by livestock and poultry in the Yangtze Delta are estimated to be: 0.17 Mt NH3-N, 0.16 Mt TP and 0.42 Mt TN, giving rise to a COD of 1.86 Mt and a BOD of 1.72 Mt. Approximately 25% of this pollution was estimated to enter water bodies, which means that the annual pollutant load is 43,700 t NH3-N, 39,400 tTP, 104,600t TN with a COD of 465,000 tand a BOD of 430,100 t. Pollutants from animal husbandry were similar in magnitude to those from industrial wastewater. Pigs produced the most pollution, followed by poultry, cattle and sheep. The pollution load from animal husbandry in the Yangtze Delta is about twice the average level of the whole of China. CONCLUSIONS: Domestic wastewater was the main pollution source in the Yangtze Delta, followed by pollution from raising livestock and poultry and from industrial wastewater. The pollution load in Shanghai and Jiaxing were the greatest, followed by 7 cities of Jiangsu province (except Suzhou) and other cities of Zhejiang province and Suzhou. Pigs and poultry produced about 90% of the total pollutants from animal husbandry. RECOMMENDATIONS AND PERSPECTIVES: The local governments, especially in Shanghai and Jiaxing, should focus their attention on the pollution produced by livestock and poulrry. Controlling pollution from pigs and poultry will have the greatest impact in this region. Control of pollution will be facilitated by the development of large-scale livestock and poultry farming units and a shift away from small scale husbandry. 相似文献
894.
基于SWAT模型的流域面源污染模拟影响分析 总被引:4,自引:0,他引:4
针对流域面源污染模型往往忽略或简化河道内污染物变化过程的缺陷,探讨了河道水质模型对流域面源污染模拟的影响.以太湖流域浙西区的西苕溪流域为研究对象,选取具有一定物理机制的分布式面源污染模型SWAT模型,分别以激活和不激活其嵌套的河道水质模型QUAL2E,即SWAT模型与QUAL2E模型紧密耦合和松散耦合两种情况进行模拟,并比较了对TN及TP的模拟效果.结果表明,丰水期与平水期的模拟结果并没有显著差别;但在枯水期,由于水量较小,河道内污染物变化过程对模拟结果影响较大.同时引入QUAL2K模型,分析认为改进河道水质模型对提高SWAT模型模拟精度有一定的效果. 相似文献
895.
覆冰输电塔-线体系风致动力响应分析 总被引:4,自引:1,他引:3
依据流体诱发振动原理,结合已有覆冰计算模型,考虑降雨的分类,模拟了输电塔-线体系不同高度导线的覆冰和风荷载。以东北地区某输电塔为例,对覆冰输电塔-线体系在稳定风速激励下的动力响应进行分析,并与不考虑塔线耦联的导线舞动分析结果及覆冰塔线拟静力的分析结果进行对比,对塔位移、输电线位移、钢材应力进行了分析。研究结果表明:塔-线耦联体系对覆冰导线风振有很大影响,覆冰输电塔抗风设计安全度需要进一步提高。 相似文献
896.
Marcos A. dos Santos Cynthia F. Illanes Adalgiza Fornaro Jairo J. Pedrotti 《Water, Air, & Soil Pollution: Focus》2007,7(1-3):85-92
During the period from July 2002 to June 2004, the chemical characteristics of the rainwater samples collected in downtown São Paulo were investigated. The analysis of 224 wet-only precipitation samples included pH and electrical conductivity, as well as major ions (Na+, $ \rm NH^{ + }_{4} During the period from July 2002 to June 2004, the chemical characteristics of the rainwater samples collected in downtown
S?o Paulo were investigated. The analysis of 224 wet-only precipitation samples included pH and electrical conductivity, as
well as major ions (Na+, , K+, Ca2+, Mg2+, Cl−, , ) and carboxylic acids (acetic, formic and oxalic) using ion chromatography. The volume weighted mean, VWM, of the anions
, and Cl− was, respectively, 20.3, 12.1 and 10.7 μmol l−1. Rainwater in S?o Paulo was acidic, with 55% of the samples exhibiting a pH below 5.6. The VWM of the free H+ was 6.27 μmol l−1), corresponding to a pH of 5.20. Ammonia (NH3), determined as (VWM = 32.8 μmol l−1), was the main acidity neutralizing agent. Considering that the H+ ion is the only counter ion produced from the non-sea-salt fraction of the dissociated anions, the contribution of each anion
to the free acidity potential has the following profile: (31.1%), (26.0%), CH3COO− (22.0%), Cl− (13.7%), HCOO− (5.4%) and (1.8%). The precipitation chemistry showed seasonal differences, with higher concentrations of ammonium and calcium during
autumn and winter (dry period). The marine contribution was not significant, while the direct vehicular emission showed to
be relevant in the ionic composition of precipitation. 相似文献
897.
Naszradi T Badacsonyi A Keresztényi I Podar D Csintalan Z Tuba Z 《Environmental monitoring and assessment》2007,134(1-3):279-285
Moss transplants of Tortula ruralis were used as active biomonitoring organisms as part of a monitoring study to assess the metals (Al, Cd, Cu, Cr, Fe, Ni, Pb, V and Zn) associated with ambient particles on mosses in Budapest, the capital town of Hungary. The moss samples were collected in a nature conservation area from a semi-arid sand grassland (Festucetum vaginatae danubiale), less than 1 month before transplantation. Moss cushions were exposed to pollution in Budapest during October–November 1993 and February–March 1994. In the study area, 16 sites were marked out as measuring sites, in accordance with the structure of the city. A similar stand was established in the Botanical Gardens of the Szent István University in Gödöll? as a control site. ICP-AES analysis of moss for metals showed the ability of Tortula ruralis to accumulate the metals under study. Control site showed lower impact in comparison to the other sites. 相似文献
898.
Lemly AD 《Environmental monitoring and assessment》2007,125(1-3):361-375
This paper gives step-by-step instructions for assessing aquatic selenium hazards associated with mining. The procedure was
developed to provide the U.S. Forest Service with a proactive capability for determining the risk of selenium pollution when
it reviews mine permit applications in accordance with the National Environmental Policy Act (NEPA). The procedural framework
is constructed in a decision-tree format in order to guide users through the various steps, provide a logical sequence for
completing individual tasks, and identify key decision points. There are five major components designed to gather information
on operational parameters of the proposed mine as well as key aspects of the physical, chemical, and biological environment
surrounding it — geological assessment, mine operation assessment, hydrological assessment, biological assessment, and hazard
assessment. Validation tests conducted at three mines where selenium pollution has occurred confirmed that the procedure will
accurately predict ecological risks. In each case, it correctly identified and quantified selenium hazard, and indicated the
steps needed to reduce this hazard to an acceptable level. By utilizing the procedure, NEPA workers can be confident in their
ability to understand the risk of aquatic selenium pollution and take appropriate action. Although the procedure was developed
for the Forest Service it should also be useful to other federal land management agencies that conduct NEPA assessments, as
well as regulatory agencies responsible for issuing coal mining permits under the authority of the Surface Mining Control
and Reclamation Act (SMCRA) and associated Section 401 water quality certification under the Clean Water Act. Mining companies
will also benefit from the application of this procedure because priority selenium sources can be identified in relation to
specific mine operating parameters. The procedure will reveal the point(s) at which there is a need to modify operating conditions
to meet environmental quality goals. By recognizing concerns early in the NEPA process, it may be possible for a mining company
to match operational parameters with environmental requirements, thereby increasing the likelihood that the permit application
will be approved. 相似文献
899.
A biennial integrated survey, based on the use of vascular plants for the bioindication of the effects of tropospheric ozone together with the use of automatic analysers of ozone, as well as the mapping of lichen biodiversity was performed in the area of Castelfiorentino (Tuscany, central Italy). Photochemically produced ozone proved to be a fundamental presence during the warm season, with maximum hourly means reaching 114 ppb, exceeding the information threshold as fixed by EU: the use of supersensitive tobacco Bel-W3 confirmed the opportunity of carrying out detailed cost-effective monitoring surveys. The potential for didactical and educational implications of this methodology are appealing. Critical levels set up for the protection of vegetation have exceeded considerably. The comparison of biomass productivity in sensitive and resistant individuals (NC-S and NC-R white clover clones, in the framework of an European network) provided evidence that ambient ozone levels are associated with relevant reduction (up to 30%) in the performance of sensitive material; effects on flowering were also pronounced. The economic assessment of such an impact deserves attention. Mapping of epiphytic lichen biodiversity – which has been used to monitor air quality worldwide – was not related to ozone geographical distribution as depicted by tobacco response. 相似文献
900.
An air quality sampling program was designed and implemented to collect the baseline concentrations of respirable suspended
particulates (RSP = PM10), non-respirable suspended particulates (NRSP) and fine suspended particulates (FSP = PM2.5). Over a three-week period, a 24-h average concentrations were calculated from the samples collected at an industrial site
in Southern Delhi and compared to datasets collected in Satna by Envirotech Limited, Okhla, Delhi in order to establish the
characteristic difference in emission patterns. PM2.5, PM10, and total suspended particulates (TSP) concentrations at Satna were 20.5 ± 6.0, 102.1 ± 41.1, and 387.6 ± 222.4 μg m−3 and at Delhi were 126.7 ± 28.6, 268.6 ± 39.1, and 687.7 ± 117.4 μg m−3. Values at Delhi were well above the standard limit for 24-h PM2.5 United States National Ambient Air Quality Standards (USNAAQS; 65 μg m−3), while values at Satna were under the standard limit. Results were compared with various worldwide studies. These comparisons
suggest an immediate need for the promulgation of new PM2.5 standards. The position of PM10 in Delhi is drastic and needs an immediate attention. PM10 levels at Delhi were also well above the standard limit for 24-h PM10 National Ambient Air Quality Standards (NAAQS; 150 μg m−3), while levels at Satna remained under the standard limit. PM2.5/PM10 values were also calculated to determine PM2.5 contribution. At Satna, PM2.5 contribution to PM10 was only 20% compared to 47% in Delhi. TSP values at Delhi were well above, while TSP values at Satna were under, the standard
limit for 24-h TSP NAAQS (500 μg m−3). At Satna, the PM10 contribution to TSP was only 26% compared to 39% in Delhi. The correlation between PM10, PM2.5, and TSP were also calculated in order to gain an insight to their sources. Both in Satna and in Delhi, none of the sources
was dominant a varied pattern of emissions was obtained, showing the presence of heterogeneous emission density and that nonrespirable
suspended particulate (NRSP) formed the greatest part of the particulate load. 相似文献