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11.
Mei Li Yao Zhang Chenglei Pei Jinwen Zhang Chunlei Cheng Xiufeng Lian Mubai Chen Bo Huang Zhong Fu Zhen Zhou 《环境科学学报(英文版)》2023,35(2):806-822
The real-time detection of the mixing states of polycyclic aromatic hydrocarbons (PAHs) and nitro-PAHs in ambient particles is of great significance for analyzing the source, aging process, and health effects of PAHs and nitro-PAHs; yet there is still few effective technology to achieve this type of detection. In this study, 11 types of PAH and nitro-PAH standard samples were analyzed using a high performance-single particle aerosol mass spectrometer (HP-SPAMS) in lab studies. The identification principles ‘parent ions’ and ‘mass-to-charge (m/z) = 77’ of each compound were obtained in this study. It was found that different laser energies did not affect the identification of the parent ions. The comparative experiments of ambient atmospheric particles, cooking and biomass burning emitted particles with and without the addition of PAHs were conducted and ruled out the interferences from primary and secondary organics on the identification of PAHs. Besides, the reliability of the characteristic ions extraction method was evaluated through the comparative study of similarity algorithm and deep learning algorithm. In addition, the real PAH-containing particles from vehicle exhaust emissions and ambient particles were also analyzed. This study improves the ability of single particle mass spectrometry technology to detect PAHs and nitro-PAHs, and HP-SPAMS was superior to SPAMS for detecting single particles containing PAHs and nitro-PAHs. This study provides support for subsequent ambient observations to identify the characteristic spectrum of single particles containing PAHs and nitro-PAHs. 相似文献
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Xiaolan Li Guiqian Tang Liguang Li Weijun Quan Yangfeng Wang Ziqi Zhao Ningwei Liu Ye Hong Yanjun Ma 《环境科学学报(英文版)》2022,34(3):300-310
Visibility observed at different altitudes is favorable to understand the causes of air pollution. We conducted 4-years of observations of visibility at 2.8 and 60 m and particulate matter(PM) concentrations from 2015 to 2018 in Shenyang, a provincial city in Northeast China. The results indicated that visibility increased with the increasing height in winter(especially at night), and decreased with height in summer(especially at the daytime). PM concentration exhibited opposite vertical variati... 相似文献
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Guanyu Jiang Can Wang Lu Song Xing Wang Yangyang Zhou Chunnan Fei He Liu 《Frontiers of Environmental Science & Engineering》2021,15(3):46
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Litao Wang Joshua S. Fu Wei Wei Zhe Wei Chenchen Meng Simeng Ma Jiandong Wang 《Frontiers of Environmental Science & Engineering》2018,12(3):13
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植被覆盖度与沙尘暴形成条件分析 总被引:1,自引:0,他引:1
以归一化差值植被指数(Normalized Difference Vegetation Index,NDVI)为指标分析了我国1981年到1998年期间植被覆盖变化情况,给出了植被急剧减少产生新沙源的实例。通过对1998年4月强沙尘暴的分析,指出影响沙尘暴产生和运移的因素除了地形、风速、风向、大气稳定度外,当地植被覆盖和土壤因素也是关键因素之一。并通过对植被覆盖度(NDVI)与浮尘指数(Aerosol Index)进行定量分析,发现二者之间存在明显的负相关关系,表明植被的存在可以从一定程度上抑制浮尘现象的产生。因此,在沙尘运移路径上,采取封山封荒,植树种草,增加植被覆盖度以固结当地土壤和泥沙的措施,可以在一定程度上抑制沙尘暴灾害的发生。 相似文献
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Stringent quarantine measures during the Coronavirus Disease 2019 (COVID-19) lockdown period (January 23, 2020 to March 15, 2020) have resulted in a distinct decrease in anthropogenic source emissions in North China Plain compared to the paralleled period of 2019. Particularly, 22.7% decrease in NO2 and 3.0% increase of O3 was observed in Tianjin, nonlinear relationship between O3 generation and NO2 implied that synergetic control of NOx and VOCs is needed. Deteriorating meteorological condition during the COVID-19 lockdown obscured the actual PM2.5 reduction. Fireworks transport in 2020 Spring Festival (SF) triggered regional haze pollution. PM2.5 during the COVID-19 lockdown only reduced by 5.6% in Tianjin. Here we used the dispersion coefficient to normalize the measured PM2.5 (DN-PM2.5), aiming to eliminate the adverse meteorological impact and roughly estimate the actual PM2.5 reduction, which reduced by 17.7% during the COVID-19 lockdown. In terms of PM2.5 chemical composition, significant NO3? increase was observed during the COVID-19 lockdown. However, as a tracer of atmospheric oxidation capacity, odd oxygen (Ox = NO2 + O3) was observed to reduce during the COVID-19 lockdown, whereas relative humidity (RH), specific humidity and aerosol liquid water content (ALWC) were observed with noticeable enhancement. Nitrogen oxidation rate (NOR) was observed to increase at higher specific humidity and ALWC, especially in the haze episode occurred during 2020SF, high air humidity and obvious nitrate generation was observed. Anomalously enhanced air humidity may response for the nitrate increase during the COVID-19 lockdown period. 相似文献
18.
Bushra Khali Ayesha Khali Sidra Muslim Ammara Habi Kishwar Khan Debora Souza Alvim Sehrish Shakoor Sonia Mustaf Sana Zaheer Momel Zoon Azmat Hayat Khan Sana Ilyas Bin Chen 《环境科学学报(英文版)》2021,33(1):28-39
This study finds out seasonal and monthly variations in Aerosol Optical Depth (AOD) over eastern and western routes of China Pakistan Economic Corridor (CPEC) and the relationship between AOD and meteorological parameters (i.e., temperature, rainfall and wind speed). The Moderate Resolution Imaging Spectroradiometer (MODIS) and Multi-angle Imaging Spectroradiometer (MISR) data was used from the terra satellite for the period of 2000-2016. This study aims to overtake the conventional view of the purpose of using the satellite datasets. This study takes on to the concept that validated satellite data sets rather should be used for the analysis instead of just validation specifically for our study region. Hence, after comparing MODIS AOD with MISR AOD, only MISR AOD dataset is used for further analysis. The results show a decreasing trend of AOD in summer season, a positive relationship between temperature and AOD during winter and spring seasons whereas a positive relationship between wind speed and AOD in winter and spring seasons over eastern and western routes. Periodic analysis of MODIS AOD and MISR AOD depicts May-Aug as the peak period of aerosol concentration over central Pakistan. The inter-annual analysis shows the aerosol trend remained higher during summer season however rainfall shows the washout effect. Eastern route has higher standard deviation and larger values for aerosol prevalence as compared to western route. The trajectory analysis using the HYSPLIT model suggests the bias of air mass trajectory caused deviation in the aerosol trend in the year 2014. 相似文献
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文章评述了气溶胶中多环芳烃污染源类型识别的几种方法,即:比值法、轮廓图法、特征化合物法和多元统计方法等.比值法简单可行,应用较多,但常因苯并(a)芘的不稳定性而带来误差,建议与轮廓图法、特征化合物法等配合使用,多元统计法要求样品数多,并且运算复杂,目前应用尚不多见,但其潜力很大。 相似文献