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Yongjiao Xiong Xiangfeng Huang Lexue Li Wanqi Liu Jialu Zhang Mengfan He Jia Liu Lijun Lu Kaiming Peng 《环境科学学报(英文版)》2022,34(8):112-121
The separation of ultrafine oil droplets from wasted nanoemulsions stabilized with high concentration of surfactants is precondition for oil reuse and the safe discharge of effluent. However, the double barriers of the interfacial film and network structures formed by surfactants in nanoemulsions significantly impede the oil-water separation. To destroy these surfactant protective layers, we proposed a newly-developed polyethyleneimine micelle template approach to achieve simultaneous surface charge manipulation and morphology transformation of magnetic nanospheres to magnetic nanorods. The results revealed that positively charged magnetic nanospheres exhibited limited separation performance of nanoemulsions, with a maximum chemical oxygen demand (COD) removal of 50%, whereas magnetic nanorods achieved more than 95% COD removal in less than 30 s. The magnetic nanorods were also applicable to wasted nanoemulsions from different sources and exhibited excellent resistance to wide pH changes. Owing to their unique one-dimensional structure, the interfacial dispersion of magnetic nanorods was significantly promoted, leading to the efficient capture of surfactants and widespread destruction of both the interfacial film and network structure, which facilitated droplet merging into the oil phase. The easy-to-prepare and easy-to-tune strategy in this study paves a feasible avenue to simultaneously tailor surface charge and morphology of magnetic nanoparticles, and reveals the huge potential of morphology manipulation for producing high-performance nanomaterials to be applied in complex interfacial interaction process. We believe that the newly-developed magnetic-nanorods significantly contribute to hazardous oily waste remediation and advances technology evolution toward problematic oil-pollution control. 相似文献
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Shigeru Matsumoto 《Resources, Conservation and Recycling》2011,55(3):325-334
Recent studies have predicted that the costs and benefits of curbside recycling programs will vary considerably across municipalities. In this paper, we examine how the characteristics of municipalities are reflected in curbside recycling policies. Our analysis of Japanese municipal data reveals that municipalities implement recycling programs that fit the demographic profiles of their residents. Municipalities with a considerable number of single-recycler households tend to implement simple waste separation programs. The labor market positions of spouses have different impacts on recycling policies. We further find that the municipalities implementing comprehensive recycling programs collect plastic bottles and containers more frequently than do other municipalities. This implies that the municipalities need to take measures to effectively execute comprehensive recycling programs after implementing them. 相似文献
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在黄棕壤和棕红壤上施用磷肥,经三年室内湿润条件下培养,用石灰性土壤无机磷分级方法测定各形态磷含量.各形态用增量的分配比例表明,Fe-P居首位,其次为Al-P和O-P.三级Ca-P之和在20%以下.经培养的土壤种植黑麦草,其生物量和吸磷量与各形态磷量的相关系数除Ca10-P外,均达到极显著水准.土壤有效磷与各形态磷的相关性表明,Ca2-P是土壤有效磷的直接给源(r=0.992),Fe-P、Al-P是有效磷的重要潜在性给源(r分别为0.982和0.914),O-P、Ca10-P为无效态磷(r=-0.168). 相似文献
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In order to upgrade polymer waste during recycling, separation should take place at high purity. The present research was aimed to develop a novel, alternative separation opportunity, where the polymer fractions were separated by centrifugal force in melted state. The efficiency of the constructed separation equipment was verified by two immiscible plastics (polyethylene terephthalate, PET; low density polyethylene, LDPE), which have a high difference of density, and of which large quantities can also be found in the municipal solid waste. The results show that the developed equipment is suitable not only for separating dry blended mixtures of PET/LDPE into pure components again, but also for separating prefabricated polymer blends. By this process it becomes possible to recover pure polymer substances from multi-component products during the recycling process. The adequacy of results was verified by differential scanning calorimetry (DSC) measurement as well as optical microscopy and Raman spectroscopy. 相似文献
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采用液膜分离工艺处理含酚、氰农药废水,处理废水量36t/d,通过工业应用实例试运行,效果一直很好。达到了设计要求。 相似文献
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