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21.
《环境科学学报(英文版)》2023,35(3):319-331
Oxidation-absorption technology is a key step for NOx removal from low-temperature gas. Under the condition of low O3 concentration (O3/NO molar ratio = 0.6), F-TiO2 (F-TiO2), which is cheap and environmentally friendly, has been prepared as ozonation catalysts for NO oxidation. Catalytic activity tests performed at 120°C showed that the NO oxidation efficiency of F-TiO2 samples was higher than that of TiO2 (about 43.7%), and the NO oxidation efficiency of F-TiO2-0.15 was the highest, which was 65.3%. Combined with physicochemical characteristics of catalysts and the analysis of active species, it was found that there was a synergistic effect between F sites and oxygen vacancies on F-TiO2, which could accelerate the transformation of monomolecular O3 into multi-molecule singlet oxygen (1O2), thus promoting the selective oxidation of NO to NO2. The oxidation reaction of NO on F-TiO2-0.15 follows the Eley-Rideal mechanism, that is, gaseous NO reacts with adsorbed O3 and finally form NO2. 相似文献
22.
Chinese life cycle impact assessment factors 总被引:5,自引:0,他引:5
IntroductionLifecycleassessment(LCA)isanenvironmentalmanagementtoolthatisusedtoexamineandevaluatetheenvironmentalimpactsassociatedwiththeexistenceofproducts(Jensen,1998;Weidema,1997;Wenzel,1997).ThefocusofLCAisontheentirelifecycleoftheproduct,i.e.fromtheextracti… 相似文献
23.
《环境科学学报(英文版)》2023,35(3):309-318
Accurate quantification of dissolved organic nitrogen (DON) has been a challenge due to the cumulative analytical errors in the conventional method via subtracting dissolved inorganic nitrogen species (DIN) from total dissolved nitrogen (TDN). Size exclusion chromatography coupled with an organic nitrogen detector (SEC-OND) has been developed as a direct method for quantification and characterization of DON. However, the applications of SEC-OND method still subject to poor separations between DON and DIN species and unsatisfied N recoveries of macromolecules. In this study, we packed a series of SEC columns with different lengths and resin materials for separation of different N species and designed an independent vacuum ultraviolet (VUV) oxidation device for complete oxidation converting N species to nitrate. To guarantee sufficient N recoveries, the operation conditions were optimized as oxidation time ≥ 30 min, injection mass (sample concentration × injection volume) < 1000 µL × mg-N/L for macromolecular proteins, and neutral pH mobile eluent. The dissolved O2 concentration in SEC mobile phase determined the upper limit of VUV oxidation at a specific oxidation time. Compared to conventional HW50S column (20 × 250 mm), HW40S column (20 × 350 mm) with mobile phase comprising of 1.5 g/L Na2HPO4·2H2O + 2.5 g/L KH2PO4 (pH = 6.85) could achieve a better separation of DON, nitrite, nitrate, and ammonia. When applied to river water, lake water, wastewater effluent, groundwater, and landfill leachate, the SEC-OND method could quantify DON as well as DIN species accurately and conveniently even the DIN/TDN ratio reached 0.98. 相似文献
24.
中国东南沿海中生代火山作用基本特征 总被引:3,自引:0,他引:3
中国东南沿海自晚侏罗世到白垩纪火山活动分为二期、四个旋回,在空间上有迁移性,在时间上与侵入活动呈交替式演变。建立火山碎屑流等五种岩相模式,岩浆爆发占主导地位,同时存在蒸气岩浆爆发。确定破火山口、火山穹隆和锥火山为火山构造基本类型。由火山作用与区域构造作用、沉积作用控制形成火山沉积洼地、火山构造洼地和火山构造隆起。提出不同类型火山构造组合形式和相互演化关系。火山岩系列属高钾钙碱系列,晚期则具双模式性质。它们的地球化学型式兼具大陆边缘和大陆板内双重特性。 相似文献
25.
对京津区域1980-1992年间能源利用状况进行分析,并通过模式计算该区域大气污染物的扩散规律,结果表明,大气污染物随能源利用增加而增加,其增加速率NOx大于OS2,经预测,至2004年京津地区SO2排放量增咖11.40%,NOx增加56.80%,由于气象和地形条件所致,该区域内不利于大气污染物远距离输送,这使箱型区域内物料平衡计算可以简化。 相似文献
26.
炼油装置运行周期评估技术通过统计、分析装置故障数据,计算特定时间段装置的可靠性,进而获得装置可靠性随时间的变化规律和装置可靠性最差设备排序。介绍了该技术在某常减压装置的应用,应用结果表明,该评估技术为科学确定炼油装置运行周期提供了决策依据。 相似文献
27.
Integrated environmental assessment and pollution prevention in Vietnam: the case of anthracite production 总被引:1,自引:0,他引:1
Loi Dinh Chinh Shabbir H. Gheewala Sbastien Bonnet 《Journal of Cleaner Production》2007,15(18):1768-1777
Using the concept of life cycle analysis, the whole life cycle of anthracite production in Vietnam was assessed and the environmental “hot-spots” were identified. These include (i) dust pollution at coal transfer points or piles in storage; (ii) noise pollution resulting from the usage of heavy equipment, and (iii) high volume of acid and turbid mine water discharged into the environment.Pollution prevention and treatment options were identified and discussed in this study which consists of wet treatment of dust, planning, collection and treatment of mine water, planting of trees for dust and noise reduction as well as minimization of erosion. Some recommendations are made for pollution abatement from coal production and improvement of anthracite production in the region. 相似文献
28.
构建"生产-运输-使用-废弃处置"的外卖全产业链,通过大样本企业调研与外卖平台大数据分析,计算8个样本城市不同材质与规格的外卖餐盒、餐具、包装袋的市场使用比例,挖掘骑手配送的海量数据,收集城市垃圾处理处置情况,系统评估外卖全过程的环境影响.结果表明,外卖包装物全产业链中生产环节(45%)与废弃处置环节(50%)为环境影响的主要来源,严重程度依次为固废排放、水污染、资源能源消耗和大气污染.所在城市及选用包装物材质的不同,外卖行业造成的环境影响会有显著区别,全产业链上的各环节需相互配合,多主体共同承担环境责任,采取差别化的减缓应对措施. 相似文献
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