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Kuo LJ Louchouarn P Herbert BE Brandenberger JM Wade TL Crecelius E 《Environmental pollution (Barking, Essex : 1987)》2011,159(4):983-990
Reconstructions of 250 years historical inputs of two distinct types of black carbon (soot/graphitic black carbon (GBC) and char-BC) were conducted on sediment cores from two basins of the Puget Sound, WA. Signatures of polycyclic aromatic hydrocarbons (PAHs) were also used to support the historical reconstructions of BC to this system. Down-core maxima in GBC and combustion-derived PAHs occurred in the 1940s in the cores from the Puget Sound Main Basin, whereas in Hood Canal such peak was observed in the 1970s, showing basin-specific differences in inputs of combustion byproducts. This system showed relatively higher inputs from softwood combustion than the northeastern U.S. The historical variations in char-BC concentrations were consistent with shifts in climate indices, suggesting an influence of climate oscillations on wildfire events. Environmental loading of combustion byproducts thus appears as a complex function of urbanization, fuel usage, combustion technology, environmental policies, and climate conditions. 相似文献
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Trends of perfluorochemicals in Greenland ringed seals and polar bears: Indications of shifts to decreasing trends 总被引:1,自引:0,他引:1
Time-series of perfluorinated alkylated substances (PFASs) in East Greenland polar bears and East and West Greenland ringed seals were updated in order to deduce whether a response to the major reduction in perfluoroalkyl production in the early 2000s had occurred. Previous studies had documented an exponential increase of perfluorooctane sulphonate (PFOS) in liver tissue from both species. In the present study, PFOS was still the far most dominant compound constituting 92% (West Greenland ringed seals), 88% (East Greenland ringed seals) and 85% (East Greenland polar bears). The PFOS concentrations increased up to 2006 with doubling times of approximately 6 years for the ringed seal populations and 14 years in case of polar bears. Since then a rapid decrease has occurred with clearing half-lives of approximately 1, 2 and 4 years, respectively. In polar bears perfluorohexane sulphonate (PFHxS) and perfluorooctane sulphonamide (PFOSA) also showed decreasing trends in recent years as do perfluorodecanoic acid (PFDA) and perfluoroundecanoic acid (PFUnA). For the West Greenland ringed seal population perfluorooctanoic acid (PFOA), perfluorononanoic acid (PFNA), PFDA and PFUnA peaked in the mid 2000s, whereas PFNA, PFDA and PFUnA in the East Greenland population have been stable or increasing in recent years. The peak of PFASs in Greenland ringed seals and polar bears occurred at a later time than in Canadian seals and polar bears and considerably later than observed in seal species from more southern latitudes. We suggest that this could be explained by the distance to emission hot-spots and differences in long-range transport to the Arctic. 相似文献
16.
Marie Vanden Berghe Stéphanie Polain Jean-Pierre Thomé 《Environmental pollution (Barking, Essex : 1987)》2010,158(5):1570-1575
A previous study has shown a simultaneous increase of vitamin A and PCBs in grey seal (Halichoerus grypus) milk at late lactation (Debier et al., 2004). Here we sought to understand this unexpected relationship by comparing the dynamics of vitamin A and PCBs in the different tissue compartments of transfer. Lactating grey seals and their pups were sampled longitudinally in Scotland during the 2006 breeding season. As blubber reserves decreased, concentrations of vitamin A and PCBs increased during lactation in the inner layer of maternal blubber. A concomitant rise was observed in milk and consequently in the serum of suckling pups. The similar dynamics of vitamin A and PCBs in milk and inner blubber suggest a common mechanism of mobilisation from maternal body stores and transfer into the milk. A panel data analysis highlighted a negative impact of PCBs in milk and pup serum on vitamin A status in pup serum. 相似文献
17.
A hierarchical approach to fisheries planning and modeling in the Columbia River Basin 总被引:1,自引:0,他引:1
The Columbia River Basin is the scene of a massive effort to restore populations of Pacific salmon (Oncorhynchus spp.) and steelhead (O. mykiss). Efficient restoration is confounded by a high level of complexity, competing sociopolitical goals and values, and uncertainty
about key system properties. Simulation models and other tools of systems analysis are important to development of a comprehensive,
regionally acceptable strategy. Hierarchy theory provides a useful paradigm for organized complexity within the Columbia Basin
and the basis for a trilevel hierarchical structure for organizing and integrating models. Life-stage models compose the most
basic simulation units at the lowest level in the proposed hierarchical modeling structure. Each life-stage model simulates
a distinct period in the life cycle of anadromous salmonids. Population models at the intermediate level simulate the complete
life cycles of salmon and steelhead populations. At the highest level in the hierarchy, interpopulation models simulate extensive,
long-term processes that affect multiple species and stocks. A hierarchical system of models is preferable to a single model
or to a group of models lacking formal structure. A principal advantage is that models have the correct spatial and temporal
resolution for analyzing questions at different scales. A hierarchical structure also facilitates the flow of information
among models, and aids in understanding the impacts of uncertainty. Constructing a hierarchy of models should involve both
bottom-up and top-down perspectives that maintain logical consistency among models, while allowing unique model structures
appropriate for each level in the hierarchy. 相似文献
18.
Leonard G. Pearlstine Wiley M. Kitchens Pamela J. Latham Richard D. Bartleson 《Journal of the American Water Resources Association》1993,29(6):1009-1019
ABSTRACT: Construction of a tide gate at the mouth of the north channel of the Savannah River in Georgia has resulted in significant changes in salinities influencing marsh community changes. The tide gate is directly responsible for a 2 to 6 mile upstream displacement of salt water in the river. In the marsh, soil salinities ranged from 0.0 ppt at upstream sites to 12 ppt at downstream sites when the tide gate was in operation. Within two months of taking the tide gate out of operation, interstitial salinities at the downstream sites dropped to 4 ppt. Influences of the tide gate on marsh vegetation were modeled in a geographic information system. With the tide gate out of operation, the model predicts that freshwater marsh would increase in area by 340 percent. 相似文献
19.
To evaluate the accounts of local fishermen, Landsat TM images (1986, 1993, 1999) were examined to assess potential losses
in the mangrove forests of the Teacapán–Agua Brava lagoon system, Mexico. A binary change mask derived from image differencing
of a band 4/3 ratio was employed to calculate any changes within this forested wetland. The results indicate that by 1986
approximately 18% (or 86 km2) of the mangrove area under study was either dead or in poor condition. The majority of this damage had occurred in the eastern
section of the Agua Brava basin, which coincides, with the reports of the elderly fishermen. Examination of aerial photographs
from 1970 revealed no adverse impacts in this area and would suggest, as postulated by the fishermen and other scientists,
that modifications in environmental conditions following the opening of a canal, Cuautlá canal, in 1972 may have initiated
the large-scale mortality. Although these areas of impact are still developing, the results from the satellite data indicate
that the majority of the more recent changes are occurring elsewhere in the system. Obvious in the 1999 satellite data, but
not so in the 1993, are large areas of mangrove degradation in the northern section of the Teacapán region. In the Agua Brava
basin, the more recent transformations are appearing on the western side of the basin. Since long-term records of environmental
conditions are absent, it is difficult to determine why these latest changes are occurring or even if the earlier losses were
the result of the canal. Potential agents of change that have recently been observed include a hurricane, a second canal,
and the uncontrolled expansion of the Cuautlá canal since 1994. 相似文献
20.
为解决干冰膨胀烟丝生产线冷端液体工艺泵因机械密封长期超压和气缚现象造成损坏发生CO2泄漏而导致紧急停机抢修的问题,对干冰膨胀线冷端工艺罐系统进行了优化改进。在工艺泵吸口前管路引一根气相平衡管至工艺罐顶部,当泵吸口前管路有CO2液体时,输送管路内气化的CO2气体通过气相平衡管线释放回工艺罐内,不会进入工艺泵体内。应用结果表明,工艺泵内的憋压和气缚现象消失了,机械密封受到保护。改造前机械密封平均一个季度更换一次,改造后机械密封使用5年未损毁,达到保护干冰膨胀线冷端工艺泵机械密封的目的。 相似文献