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21.
The evolution of mass balance models of persistent organic pollutant fate in the environment 总被引:12,自引:0,他引:12
Current approaches to modelling the fate of persistent organic pollutants (POPs) in the environment have evolved in response to four dominant characteristics of these substances; namely: (1) the presence of POPs in virtually all environmental phases and the ease with which they move from one to the other requires multi-compartmental modelling. Describing transport across phase boundaries becomes as, or even more, important as quantifying transport within the phases; (2) POPs may persist in the environment for many decades. For chemicals that 'have time', concepts such as equilibrium partitioning and steady-state become more important than for short-lived substances whose fate is more controlled by the rates of transformation; (3) measuring POPs is difficult and expensive and observed concentrations of POPs are not available in high spatial or temporal resolution. Consequently, high resolution tends not to be a high priority in POP models; and (4) detrimental effects of POPs often manifest themselves in top predators, which has led to a focus on modelling biotic uptake and transfer within food chains. The task of building a POPs model is viewed as combining the four 'building blocks' of partitioning, transport, transformation and source data with the help of the law of the conservation of mass. Process models, evaluative models, models of real local, regional and global fate, as well as biological uptake models are presented and references to numerous examples are provided. An attempt is made to forecast future directions in the field of POPs modelling. It is expected that modelling techniques that do not rely on quantitative emission estimates as well as approaches that take into account spatial, temporal and climatic variability as well as parameter uncertainty will increase in importance. Finally, the relationship between modelling POPs and models of other pollutant issues is addressed, as are potential interactions between POPs and pollutant issues such as eutrophication, acidification and global climate change. 相似文献
22.
23.
Due to the favorable weather, abundant water resources and fertile soil, the area has been known as the homeland for crops and fish. However, being one of the most developed regions in China, the environmental quality of the Pearl River delta has deteriorated due to recent socio-economic changes during the past two decades. The drivers are industrialization and economic growth, population growth and agricultural development; and the pressures are water pollution which include nutrients and suspended solids, pesticides, other persistent toxic substances (PAHs and PCBs) and oil. These have imposed various impacts such as eutrophication, formation of red tides and biomagnification of organic contaminants through food chains. In response to these, regulatory measures have been established by the Environmental Protection Bureau of Guangdong Province, joining forces with environmental protection authorities in all urban cities and most counties, in addition to the Hong Kong Environmental Protection Department, to control pollution in order to prevent further environmental deterioration and economic loss. The present paper is an attempt by following the DPSIR approach promoted by the OECD in the early 1990s and further developed by IGBP LOICZ to review the environmental quality of Pearl River with emphasis on water quality and the impact of rapid socio-economic changes. 相似文献
24.
Burkhard O. Wagner 《Umweltwissenschaften und Schadstoff-Forschung》1998,10(4):245-253
Zusammenfassung UNEP International Register of Potentially Toxic Chemicals (IRPTC) wurde von der ersten VN-Umweltkonferenz 1972 geschaffen.
Sein Einfu? und Zusammenwirken in den 80ziger Jahren mit anderen internationalen Programmen der WHO, FAO, OECD und EG in der
Chemikalienkontrolle wird beschrieben. Nach dem Erdgipfel von Rio 1992 werden im VN-Rahmen drei neue Gremien gebildet, die
das Fachprogramm des Kapitels 19 der Agenda 21 (umweltfreundliches Chemikalienmanagement) umsetzen sollen: die United nations
Commission of Sustainable Development, das Intergovernmental Forum on Chemical Safety und das Interorganization Programme
for the Sound Management of Chemicals. Der Erdgipfel brachte auch für IRPTC eine Neuorientierung. Seit 1996 hat UNEP Chemicals,
wie sich IRPTC nunmehr nennt, drei Aufgaben in sein Arbeitsprogramm aufgenommen, die beschrieben werden: das internationale
übereinkommen zum Prior Informed Consent, das internationale übereinkommen zur Kontrolle der Persistent Organic Pollutants,
und schlie?lich sein traditionelles Arbeitsgebiet des Informations-austausches über Stoffe wird weitergeführt.
Die Aussagen dieses Beitrages sind die Meinung des Autors. Sie müssen nicht mit der Auffassung des Umweitbundesamtes oder von UNEP Chemicals übereinstimmen. 相似文献
Die Aussagen dieses Beitrages sind die Meinung des Autors. Sie müssen nicht mit der Auffassung des Umweitbundesamtes oder von UNEP Chemicals übereinstimmen. 相似文献
25.
M. Turk J. Jakšić M. Vojinović Miloradov J. Klanova 《Environmental Chemistry Letters》2007,5(3):109-113
For the duration of the war accident in former Yugoslavia, several industrial and military targets were burnt and damaged,
resulting in a significant release of persistent organic pollutants. Locations heavily targeted in the attacks were later
defined by UNEP as four “hot spots”: Kragujevac, Novi Sad, Pancevo and Bor. We analyzed concentration levels of pollutants
collected in 2004 and 2005 in air samples from the city of Kragujevac, Serbia, following the war accident of 1999. Pollutants
included polycyclic aromatic hydrocarbons (PAHs), hexachlorocyclohexane (HCH), dichloro-diphenyl-trichloroethane (DDT), dichloro-diphenyl-dichloroethylene
(DDE), dichloro-diphenyl-dichloroethane (DDD) and polychlorinated biphenyls (PCBs). We present results obtained during air
sampling campaign conducted in July 2004 by the active sampling method; and during September 2004–June 2005 by the passive
sampling method. Our findings show the occurrence of residual quantities of DDT, HCH, PCBs and PAHs in air samples. High levels
of PCBs are probably due to the destruction of transformers during the war accident. 相似文献
26.
Persistent organic pollutants control strategy in China 总被引:1,自引:0,他引:1
The development of Persistent Organic Pollutants(POPs) control policy in China in the context of international concerns on POPs was reviewed. The aspects of the Chinese POPs control strategies were analyzed, and compared with those of developed counterparts(e.g. US, EU, Japan). Currently, while the legal framework on POPs management, which complies with intemational guidelines has been established, it should be improved in the areas of special POPs management, risk assessment, the precautionary principle, lifecycle management and technical support capacity. The analysis of Chinese POPs policy and suggestions for strengthening the sciencebased decision making capacity are not only useful for Chinese decision-makers, but also a case study for developing wodd and make a great contribution for the global elimination of POPs to make a toxic-free future. 相似文献
27.
Environmental pollution has become one of the greatest problems in the world, and the concerns about environmental pollutants released by human activities from agriculture and industrial production have been continuously increasing. Although intense efforts have been made to understand the health effects of environmental pollutants, most studies have only focused on direct toxic effects and failed to simultaneously evaluate the long-term adaptive, compensatory and secondary impacts on health. Burgeoning evidence suggests that environmental pollutants may directly or indirectly give rise to disordered element homeostasis, such as for iron. It is crucially important to maintain concerted cellular and systemic iron metabolism. Otherwise, disordered iron metabolism would lead to cytotoxicity and increased risk for various diseases, including cancers. Thus, study on the effects of environmental pollutants upon iron homeostasis is urgently needed. In this review, we recapitulate the available findings on the direct or indirect impacts of environmental pollutants, including persistent organic pollutants (POPs), heavy metals and pesticides, on iron homeostasis and associated adverse health problems. In view of the unanswered questions, more efforts are warranted to investigate the disruptive effects of environmental pollutants on iron homeostasis and consequent toxicities. 相似文献
28.
Paul K.S. Lam 《环境科学学报(英文版)》2015,38(12):172-174
<正>The Three Gorges Dam project(TGDP),with a total static investment of 95.46 billion RMB(US$10.97 billion)based on the 1993 price level,commenced in 1994 and was completed in 2012.The creation of the Three Gorges Reservoir following the completion of the TGDP had brought about significant changes to the Three Gorges Reservoir Region(TGRR),stretching from the town of Sandouping in Hubei Province to the Jiangjin District of Chongqing Municipality.The TGDP has led to progressive urbanization and industrialization of the TGRR,accompanied by increased shipping activities,greater 相似文献
29.
Hanzhong Jia Yafang Shi Xiaofeng Nie Song Zhao Tiecheng Wang Virender K. Sharma 《Frontiers of Environmental Science & Engineering》2020,14(4):73
30.
Jun Kobayashi Takeo Sakurai Kaoruko Mizukawa Kyoko Kinoshita Nozomi Ito Shunji Hashimoto Daisuke Nakajima Toru Kawai Yoshitaka Imaizumi Hideshige Takada Noriyuki Suzuki 《Chemosphere》2013
We investigated the respiratory uptake kinetics of polychlorinated biphenyls (PCBs), organohalogen pesticides (OCPs), polycyclic aromatic hydrocarbons (PAHs), and 2,2′,4,4′-tetrabrominated diphenyl ether (BDE #47) in a marine benthic fish, Pseudopleuronectes yokohamae. The respiratory uptake efficiencies (EW) of the chemicals, of which there have been no reports for the majority of persistent organic pollutants (POPs), were obtained by measuring the respiratory uptake rate constants (k1) and the oxygen consumption rates of fish. Fish were exposed to water in which these chemicals were dissolved at environmentally relevant concentrations for 28 d, followed by 168 d of depuration in clean seawater. The k1 and EW values for 99 compounds were obtained, and they ranged from 2000 to 42 000 L kg-lipid−1 d−1 and from 0.060 to 1.3, respectively. The EW values of the chemicals, except for PAHs, tended to increase with increasing values of the log octanol–water partition coefficients (KOW) of the chemicals up to a log KOW of 5. For log KOW in the range 3–5, the EW values in this study were much lower than those in a published study (about one-third). As a result of analysis by a two-phase resistance model, the resistance of transport rates to the lipid phase in this study was lower than was the case in the published study. These findings indicate that the EW predicted by the published study for log KOW in the range 3–5 may differ among fish species and water temperature, and further study is needed. 相似文献