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41.
Over the last years, great progress in the research on speciation of butyltins has been made. Many coupling techniques have been successfully developed, with better applications to sediments samples in the environment. Sediments were collected from 1999 to 2000 to elucidate butyltin pollution in Theoule harbour. Most of the analysed samples showed evidence of butyltin compounds. The results show that the concentration of Tributyltin (TBT) was in the range 20–200?µg/kg in March 1999, 20–340?µg/kg in June 1999, 180–1280?µg/kg in July 2000, and 55–820?µg/kg in October 2000. A comparison of the MBT, DBT, and TBT results show that in 1999 the concentrations were in the order TBT?DBT?>?MBT, with some exceptions. The patterns observed in many sediment cores show a great disparity of organotin input concentration among the cores collected during one month and also during two different months, and from one season to the other. This paper provides information on the use of the acetic acid leaching system in the determination of butyltin. The method is applied to evaluate the occurrence of these species in sediments from the Theoule harbour, between 1999 and 2000. In this study, a GC/AES was applied, complemented with acetic acid leaching and monitored using two certified reference materials: PACS-2 reference sediment and BCR 462 (Report EUR 18406 EN, 1998). 相似文献
42.
Drinking water quality should remain constant from the drinking water treatment plant to the consumer's tap. However, water quality characteristics might be affected by interactions with pipe materials. This review describes the iron, copper, lead, zinc, aluminum, chromium, and cadmium in drinking water leached from the pipe material present in drinking water, as well as the factors and mechanisms that affect leaching processes. Data analysis suggests that monitoring the water quality in distribution systems is important for their proper management; however, the low measured concentrations highlight the need for sensitive sensors. In addition, further research is necessary to anticipate possible future effects before the installation of new materials/infrastructure or changes in water source/treatment. 相似文献
43.
B. Patti A. Bonanno G. Basilone S. Goncharov S. Mazzola G. Buscaino 《Chemistry and Ecology》2013,29(5):365-375
The main results of research work carried out since 1998 with regard to the application of hydro-acoustic technologies for the evaluation of biomass and distribution of small pelagic fish species off the southern coast of Sicily are presented, taking into account information from hydrology and from ecology of the fish populations targeted. The biomass estimates and the population‐density charts presented concern the two main species, i.e. sardine Sardina pilchardus (Walbaum, 1792) and anchovy Engraulis encrasicolus (Linnaeus, 1758). Both the sardine and anchovy populations experienced large inter-annual fluctuations, with biomass estimates ranging from 6000 to over 36,000 tonnes (t) (sardine) and from about 7000 to 23,000 t (anchovy). Acoustic estimates are largely consistent with landings recorded in Sciacca (the main fishing port for small pelagic species in the study area) during the year following the evaluation surveys. In addition, trends in sardine and anchovy biomass estimates appears to be negatively correlated with the mean sea surface temperature calculated over the time intervals January–September (sardine) and June–November (anchovy) of the preceding year, which correspond to larval and juvenile growth periods of target species. Observed patterns would suggest the importance of enrichment processes relevant to the survival of early stages, so determining recruitment success and finally higher population sizes. 相似文献
44.
Danuta Baralkiewicz Hanka Gramowska Ryszard Gołdyn Wiesław Wasiak Katarzyna Kowalczewska-Madura 《Chemistry and Ecology》2013,29(2):93-103
Sediment samples were analysed for mercury and methylmercury content in different parts of the bottom sediment of Swarz ?dzkie Lake, which were influenced by different external pollution sources. The results of determination with two methods of mineralization using two separate media (HNO3/H2O2 and HF) were compared. The accuracy of the studied methods was analysed using certified reference material IAEA 405 of river sediment. The recovery of mercury was satisfactory and ranged from 97.5 to 98.8%. Methylmercury compounds in the studied sediments were found in limited concentrations. Their concentrations ranged from 0.26 to 58.1 μg kg?1, i.e. 1.0–7.4% of the total mercury content. The depth profile displayed high values of both total and methylmercury content at a depth of 10–20 cm, related to the heavy pollution of the lake in the 1980s. Canonical analysis displayed the relationship of both total mercury and methylmercury concentrations with organic matter and phosphorus content in bottom sediments. 相似文献
45.
46.
George P. Ingersoll M. Alisa Mast Donald H. Campbell David W. Clow Leora Nanus John T. Turk 《Atmospheric environment (Oxford, England : 1994)》2008,42(24):6098-6113
Seasonal snowpack chemistry data from the Rocky Mountain region of the US was examined to identify long-term trends in concentration and chemical deposition in snow and in snow-water equivalent. For the period 1993–2004, comparisons of trends were made between 54 Rocky Mountain Snowpack sites and 16 National Atmospheric Deposition Program wetfall sites located nearby in the region. The region was divided into three subregions: Northern, Central, and Southern. A non-parametric correlation method known as the Regional Kendall Test was used. This technique collectively computed the slope, direction, and probability of trend for several sites at once in each of the Northern, Central, and Southern Rockies subregions. Seasonal Kendall tests were used to evaluate trends at individual sites.Significant trends occurred during the period in wetfall and snowpack concentrations and deposition, and in precipitation. For the comparison, trends in concentrations of ammonium, nitrate, and sulfate for the two networks were in fair agreement. In several cases, increases in ammonium and nitrate concentrations, and decreases in sulfate concentrations for both wetfall and snowpack were consistent in the three subregions. However, deposition patterns between wetfall and snowpack more often were opposite, particularly for ammonium and nitrate. Decreases in ammonium and nitrate deposition in wetfall in the central and southern rockies subregions mostly were moderately significant (p<0.11) in constrast to highly significant increases in snowpack (p<0.02). These opposite trends likely are explained by different rates of declining precipitation during the recent drought (1999–2004) and increasing concentration. Furthermore, dry deposition was an important factor in total deposition of nitrogen in the region. Sulfate deposition decreased with moderate to high significance in all three subregions in both wetfall and snowpack. Precipitation trends consistently were downward and significant for wetfall, snowpack, and snow-telemetry data for the central and southern rockies subregions (p<0.03), while no trends were noted for the Northern Rockies subregion. 相似文献
47.
Source characterization of ambient fine particles at multiple sites in the Seattle area 总被引:2,自引:0,他引:2
To identify major PM2.5 (particulate matter ≤2.5 μm in aerodynamic diameter) sources with a particular emphasis on the ship engine emissions from a major port, integrated 24 h PM2.5 speciation data collected between 2000 and 2005 at five United State Environmental Protection Agency's Speciation Trends Network monitoring sites in Seattle, WA were analyzed. Seven to ten PM2.5 sources were identified through the application of positive matrix factorization (PMF). Secondary particles (12–26% for secondary nitrate; 17–20% for secondary sulfate) and gasoline vehicle emissions (13–31%) made the largest contributions to the PM2.5 mass concentrations at all of the monitoring sites except for the residential Lake Forest site, where wood smoke contributed the most PM2.5 mass (31%). Other identified sources include diesel vehicle emissions, airborne soil, residual oil combustion, sea salt, aged sea salt, metal processing, and cement kiln. Residual oil combustion sources identified at multiple monitoring sites point clearly to the Port of Seattle suggesting ship emissions as the source of oil combustion particles. In addition, the relationship between sulfate concentrations and the oil combustion emissions indicated contributions of ship emissions to the local sulfate concentrations. The analysis of spatial variability of PM2.5 sources shows that the spatial distributions of several PM2.5 sources were heterogeneous within a given air shed. 相似文献
48.
Regional ecosystem monitoring is a central form of knowledge sharing and collaboration amongst scientists and decision makers on environmental health, land use change, and science-policy development. Despite the proliferation of such research networks on long-term monitoring on many continents, little has been achieved in Africa. This study aims to assess and examine the spatiotemporal trend and categorical patterns in ecosystem monitoring-related research in Africa for the benefits of conserving biodiversity and sustaining natural resource sectors for well-being and livelihood security, environmental planning, and ecological stewardship. A systematic review was conducted using bibliometric tools. Based on a set of search terms and peer-reviewed publications retrieved from various ecosystem monitoring networks and journal databases, further analysis was conducted using social network approaches, mapping tools, and content analysis. About 1442 scientific publications on ecosystem monitoring and related research were documented from 1987 to 2014 mostly published in English. The number of publication increased progressively since 1992 after the Convention on Biodiversity was signed and this trend peaked till 2008. South African Journal of Science was the most leading journal and Nature the most cited. Internationally coauthored and collaborative articles represented majority of the findings with the United Kingdom at the central position in the research network due to colonial relationships. Regional collaboration amongst countries is limited owing to language barriers and other institutional constraints such as funding and short-term projects. These findings have implication for prioritizing national and regional policies toward biodiversity science and its contribution to human well-being, food security, and global change responses. 相似文献
49.
针对2018年3月9—15日京津冀地区的一次空气重污染过程,进行了基于地基颗粒物激光雷达组网的星载-地基联合观测分析。颗粒物激光雷达观测到污染前期为局地污染累积过程,中期有明显的污染物区域传输过程,北京受太行山沿线城市污染输送影响较大。风廓线激光雷达观测结果表明:此次污染过程近地面主要为偏南风且风力较弱,冷空气到来时风向转为较强东北风,导致污染消散。微波辐射计观测到保定在污染过程中出现持续6 d的逆温层,同时在污染过程中近地面相对湿度较高,逆温层被打破后污染开始消散。在污染过程的各个阶段中,污染团的空间分布与变化特征均被很好地反映出来,可见地天联合观测对污染物的累积与输送研究有较大的意义,能对京津冀及周边地区的大气污染联防联控提供有力支持。 相似文献
50.