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201.
印染污泥特性及其掺煤焚烧处置的环境影响研究 总被引:1,自引:0,他引:1
对佛山6家印染厂污泥的基本性质和重金属污染进行了分析研究。结果表明:印染污泥有机质含量较高;对照农用污泥污染物限值和城镇污水处理污泥处置混合填埋用泥质标准,Cr、Ni、Cu、Zn不同程度超标,说明印染污泥既不能农用,也不能混合填埋。污泥浸出液中重金属浓度远低于危险废物浸出毒性限值和城镇污水处理厂污泥单独焚烧用泥质的污染物限值。污泥与煤掺混焚烧烟道气中二恶英浓度在0.0125~0.022 ngTEQ/Nm3,远低于GB 18485—2001《生活垃圾焚烧污染控制标准》限值和GB/T 24602—2009《城镇污水处理厂污泥处置单独焚烧用泥质》限值。 相似文献
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Lin Wang Yonglong Lu Guizhen He Arthur P. J. Mol Tieyu Wang Jorrit Gosens Kun Ni 《环境科学学报(英文版)》2014,26(7):1513-1522
Analyzing determinants that influence polychlorinated dibenzo-p-dioxin and polychlorinated dibenzofuran(PCDD/F) emissions is helpful for decision-makers to find effective and efficient ways to mitigate PCDD/F emissions. The PCDD/F emissions and the contributions of the scale effect, structure effect and technology effect to emissions from eight main industrial sectors in2006, 2008 and 2010 in Shandong Province, were calculated in this article. Total PCDD/F emissions in Shandong increased by 52.8% in 2008(614.1 g I-TEQ) and 49.7% in 2010(601.8 g I-TEQ) based on 2006(401.9 g I-TEQ). According to the decomposition method, the largest influencing factor on PCDD/F emission changes was the composition effect(contributed 43.4%in 2008 and 120.6% in 2010 based on 2006), which was also an emission-increasing factor.In this case, the present industrial restructuring policy should be adjusted to control the proportion of production capacities with high emission factors, such as iron ore sintering and steelmaking and the secondary non-ferrous metal sector. The scale effect increased the emissions in 2008(contributed 21.9%) and decreased the emissions in 2010(contributed-28.0%). However, as a source control measure, the excess capacity control policy indeed had a significant role in emission reduction. The main reason for the technology effect(contributed 34.7% in 2008 and 7.4% in 2010 based on 2006) having an emission-increasing role was the weakness in implementing policies for restricting industries with outdated facilities. Some specific suggestions were proposed on PCDD/F reduction for local administrators at the end. 相似文献
205.
Zhenyu Tian Haifeng Li Huiting Xie Chen Tang Ying Han Mengjing Wang Wenbin Liu 《环境科学学报(英文版)》2014,26(10):2041-2047
Concentrations of Polychlorinated dibenzo-p-dioxins and dibenzofurans(PCDD/Fs) and polychlorinated biphenyls(PCBs) in soil samples from Tibetan Plateau were determined. The average concentration of total 2,3,7,8-PCDD/Fs was(2.30 ± 1.02) pg/g, and World Health Organization Toxicity Equivalency(WHO-TEQ) average concentration was(0.013 ± 0.010)pg WHO-TEQ/g. The average concentration of ∑PCBs(7 indicator PCB and 12 dioxin like-PCB congeners) was(16.2 ± 9.25) pg/g, and WHO-TEQ average concentration was 0.043 ±0.049 pg WHO-TEQ/g. Comparing to previous studies in similar environmental conditions,PCDD/Fs and PCBs in this study showed a relatively lower concentration. The altitude dependences of PCDD/Fs and PCBs were also studied. Total organic carbon(TOC) normalized concentrations presented a quadratic relation with the altitudes, and an inflection could be found on the parabola of the total concentrations and some congeners of high concentration.The concentrations decreased with altitudes below about 4500 m above sea level(a.s.l.), while they increased with altitudes above it. These phenomena indicate that cold condensation of PCDD/Fs and PCBs would happen above 4500 m a.s.l, on the Tibetan Plateau. 相似文献
206.
Dielectric barrier discharges (DBD) have been used in the degradation of dioxins due to the large number of excimers and free radicals produced in discharge process. In this article, the density functional theory (DFT) is used to study the degradation mechanism of octachlorinated dibenzo-p-dioxin (OCDD) with the atomic oxygen O(3P) in DBD reactor. The reactants, intermediates, transition states and products are optimized at the MPWB1K/6- 31 + G(d,p) level. The vibrational frequencies have been calculated at the same level. The reaction pathways and mechanisms are analyzed in detail. The effect of removing the chlorine atom on environment also has been discussed. 相似文献
207.
The effect of ammonium sulfate ((NH4)2SO4) and urea (CO(NH2)2) on polychlorinated dibenzo-p-dioxin and dibenzofuran (PCDD/F) formation from active carbon was investigated in this study. Both additives could significantly inhibit PCDD/F formation, and PCDD/F (TEQ) generation was reduced to 98.5% (98%) or 64.5% (77.2%) after 5% (NH4)2S04 or CO(NH2)2 was added into model ash, respectively. The inhibition efficiency of PCDDs was higher than the value of PCDFs, however, the reduction of PCDD/F yield was mainly from PCDFs decreasing. In addition, the solid-phase products were reduced more than the gas-phase compounds by inhibitors. By the measurement of chlorine emission in the phase of ion (Cl[Cl^-]) and molecule gas (Cl[Cl2]), it was observed that both Cl[Cl^-] and Cl[Cl2] were reduced after inhibitors were added into ash. Cl[Cl2] was reduced to 51.0% by urea addition, which was supposed as one possible mechanism of PCDD/F inhibition. 相似文献
208.
本文主要针对焚烧垃圾烟气中,二恶英对大气环境的影响情况进行了分析与评价,望引起各方重视与关注。 相似文献
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1999年比利时二恶英鸡污染事件 总被引:6,自引:0,他引:6
当四川资阳猪链球菌病点燃了2005年国内食品污染的导火线时,人们对食品安全的神经再次绷紧。食品安全和公共卫生再度成为公众聚焦的话题。在泛黄的记忆里,这不由得让我们想起了1999年震撼世界的比利时二恶英鸡污染事件,事件的影响范围之广,成为继英国疯牛病危机之后欧洲最大的一起食品污染案。 相似文献