A study of the atmospheric dispersion of a high release of krypton-85 above a complex coastal terrain, comparison with the predictions of Gaussian models (Briggs, Doury, ADMS4)

Atmospheric releases of krypton-85, from the nuclear fuel reprocessing plant at the AREVA NC facility at La Hague (France), were used to test Gaussian models of dispersion. In 2001-2002, the French Institute for Radiological Protection and Nuclear Safety (IRSN) studied the atmospheric dispersion of 15 releases, using krypton-85 as a tracer for plumes emitted from two 100-m-high stacks. Krypton-85 is a chemically inert radionuclide. Krypton-85 air concentration measurements were performed on the ground in the downwind direction, at distances between 0.36 and 3.3 km from the release, by neutral or slightly unstable atmospheric conditions. The standard deviation for the horizontal dispersion of the plume and the Atmospheric Transfer Coefficient (ATC) were determined from these measurements. The experimental results were compared with calculations using first generation (Doury, Briggs) and second generation (ADMS 4.0) Gaussian models. The ADMS 4.0 model was used in two configurations; one takes account of the effect of the built-up area, and the other the effect of the roughness of the surface on the plume dispersion. Only the Briggs model correctly reproduced the measured values for the width of the plume, whereas the ADMS 4.0 model overestimated it and the Doury model underestimated it. The agreement of the models with measured values of the ATC varied according to distance from the release point. For distances less than 2 km from the release point, the ADMS 4.0 model achieved the best agreement between model and measurement; beyond this distance, the best agreement was achieved by the Briggs and Doury models.     

Automated radioxenon monitoring for the comprehensive nuclear-test-ban treaty in two distinctive locations: Ottawa and Tahiti

In preparation for verification of the Comprehensive Nuclear-Test-Ban-Treaty, automated radioxenon monitoring is performed in two distinctive environments: Ottawa and Tahiti. These sites are monitored with SPALAX (Systeme de Prelevement d'air Automatique en Ligne avec l'Analyse des radioXenons) technology, which automatically extracts radioxenon from the atmosphere and measures the activity concentrations of (131m,133m,133,135)Xe. The resulting isotopic concentrations can be useful to discern nuclear explosions from nuclear industry xenon emissions. Ambient radon background, which may adversely impact analyser sensitivity, is discussed. Upper concentration limits are reported for the apparently radioxenon free Tahiti environment. Ottawa has a complex radioxenon background due to proximity to nuclear reactors and medical isotope facilities. Meteorological models suggest that, depending on the wind direction, the radioxenon detected in Ottawa can be characteristic of the normal radioxenon background in the Eastern United States, Europe, and Japan or distinctive due to medical isotope production.     

Lead-210 and Beryllium-7 fallout rates on the southeastern coast of Brazil

Total ²¹⁰Pb and ⁷Be fallout rates were measured on the coastal region of Niteroi, Brazil. The monthly depositional flux of ²¹⁰Pb and ⁷Be varied by a factor of 26, from 1.7 to 43.3 mBq cm⁻² year⁻¹ and ∼27, from 7.5 to 203.5 mBq cm⁻² year⁻¹, respectively. The relatively large oscillations in the depositional flux of ²¹⁰Pb at this study site were likely due to variations in air mass sources, while the ⁷Be fluctuations may be driven by a combination of weather conditions. Local geology could support the periodic high fluxes of ²¹⁰Pb from continental air masses, as shifting oceanic wind sources were affirmed by the uncorrelated ²¹⁰Pb and ⁷Be fallout activities and ⁷Be/²¹⁰Pb ratios. The ²¹⁰Pb atmospheric deposition was found to be in agreement with local sediment inventories, an important consideration in geochemical studies that estimate sedimentation processes.     

Influence of atmospheric stability on the mass concentration and chemical composition of atmospheric particles: a case study in Rome, Italy

PM(10) concentration and chemical composition (ions and carbon compounds) at three sampling stations in Rome and in its surroundings was determined daily during a one-month field study, carried out during December 2003. PM concentration at the traffic station was considerably higher than at the urban background and semi-rural stations; elemental carbon was detected as one of the chemical components responsible for this increase. The difference in the concentration of sulphate and ammonium was negligible, as it was expected for secondary pollutants. A negative artefact in the determination of ammonium nitrate by means of heated automatic monitors was highlighted. The dilution properties of the lower atmosphere were traced by means of a natural radioactivity monitor. This parameter has been found to play an essential role in pollution buildup. A considerable increase in PM concentration was observed to coincide with periods of atmospheric stability. The main difference in PM composition between periods of high concentration and periods of "clean" air was found to be in the increase of ammonium nitrate concentration.     

Deposition of artificial radionuclides from atmospheric Nuclear Weapon Tests estimated by soil inventories in French areas low-impacted by Chernobyl

Soil inventories of anthropogenic radionuclides were investigated in altitudinal transects in 2 French regions, Savoie and Montagne Noire. Rain was negligible in these 2 areas the days after the Chernobyl accident. Thus anthropogenic radionuclides are coming hypothetically only from Global Fallout following Atmospheric Nuclear Weapon Tests. This is confirmed by the isotopic signatures (²³⁸Pu/^239+240Pu; ¹³⁷Cs/^239+240Pu; and ²⁴¹Am/^239+240Pu) close to Global Fallout value. In Savoie, a peat core age-dated by ²¹⁰Pb_ex confirmed that the main part of deposition of anthropogenic radionuclides occurred during the late sixties and the early seventies. In agreement with previous studies, the anthropogenic radionuclide inventories are well correlated with the annual precipitations. However, this is the first time that a study investigates such a large panel of annual precipitation and therefore of anthropogenic radionuclide deposition. It seems that at high-altitude sites, deposition of artificial radionuclides was higher possibly due to orographic precipitations.     

论大气环境污染与人体肺癌发生率

大气环境污染和人体肺癌发生率密切相关。工业和交通排放大气污染物、厨房污染、吸烟、复印机和居室装饰等造成的大气环境污染过程均能造成居民肺癌发病率的上升。应通过控制工业污染、改变能源结构、戒烟及绿化造林等措施加以解决。     

大气环境质量分析与评价研究的新进展

简要地介绍了人工神经网络（ANN）、物元可拓集（MEES）、集对分析（SPA）、遗传算法（GA）和投影寻踪技术（PP）等的基本思想和特点,评述了近年来国内外将这些新理论和新技术应用于大气环境质量分析与评价取得的最新成果,指出了大气环境质量分析与评价研究的可能发展前景。     

近地层氮氧化物和臭氧的区域分布研究

介绍了近地层氮氧化物和臭氧的区域分布研究方法,使用简化的区域尺度大气污染物传输模型和光化学反应模型,模拟计算了1990年中国主要城市排放氮氧化物的情景下,夏季(7月)主要城市的氮氧化物和相应的臭氧在近地层的浓度分布。