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81.
青岛市港口船舶大气污染排放清单的建立及应用 总被引:11,自引:3,他引:8
2002~2006年青岛市环保局与瑞典国际开发合作署合作开发了青岛市空气环境质量管理系统,建立青岛市海上交通源大气污染排放清单是其中的一项子专题,范围涉及青岛沿岸分布的港口,重点考虑船舶停泊港口及航线过程的大气污染物排放,划分了20条航线。建立的青岛市海上交通源大气污染排放清单在开发的基于GIS地理信息系统EnviMan复合源大气扩散模型中得到较好应用,实现了对沿海主要大气污染物排放量的空间模拟测算,解析出大气污染排放清单建立年度青岛市港口、航运排放的大气污染物对市区环境空气中的SO2、NOX浓度贡献分别约占8.0%、12.9%。 相似文献
82.
Junhua Li Shangchao Xiong Jianjun Chen Hao Liu Wenzhe Si Yue Peng Xuecheng Wu Huan Liu 《环境科学学报(英文版)》2023,123(1):400-416
In most of the world's building material industries, the control of flue gas pollutants mainly focuses on a single pollutant. However, given the large capacity and high contribution of China's building materials industry to global air pollution, the need to develop multi-pollutant emission reduction technology is urgent. Recently, China has focused on reducing the emissions of flue gas pollutants in the building materials industry, established many key research and development projects, and gradually implemented more stringent pollutant emission limits. This project focuses on the most recent advances in flue gas emission control technology in China's building materials industry, including denitration, dust removal, desulfurization, synergistic multi-pollutant emission reduction, and the construction of pilot research and demonstration projects for pollutant removal in several building material industries. On this basis, revised pollutant limits in flue gas emitted in China's building material industry are proposed. 相似文献
83.
Junyu Zheng Bowen Shi Xin Yuan Chuanzeng Zheng Yufan Yu Zhijiong Huang 《环境科学学报(英文版)》2023,123(1):430-445
Because of the recent growth in ground-level ozone and increased emission of volatile organic compounds (VOCs), VOC emission control has become a major concern in China. In response, emission caps to control VOC have been stipulated in recent policies, but few of them were constrained by the co-control target of PM2.5 and ozone, and discussed the factor that influence the emission cap formulation. Herein, we proposed a framework for quantification of VOC emission caps constrained by targets for PM2.5 and ozone via a new response surface modeling (RSM) technique, achieving 50% computational cost savings of the quantification. In the Pearl River Delta (PRD) region, the VOC emission caps constrained by air quality targets varied greatly with the NOx emission reduction level. If control measures in the surrounding areas of the PRD region were not considered, there could be two feasible strategies for VOC emission caps to meet air quality targets (160 µg/m3 for the maximum 8-hr-average 90th-percentile (MDA8-90%) ozone and 25 µg/m3 for the annual average of PM2.5): a moderate VOC emission cap with <20% NOx emission reductions or a notable VOC emission cap with >60% NOx emission reductions. If the ozone concentration target were reduced to 155 µg/m3, deep NOx emission reductions is the only feasible ozone control measure in PRD. Optimization of seasonal VOC emission caps based on the Monte Carlo simulation could allow us to gain higher ozone benefits or greater VOC emission reductions. If VOC emissions were further reduced in autumn, MDA8-90% ozone could be lowered by 0.3-1.5 µg/m3, equaling the ozone benefits of 10% VOC emission reduction measures. The method for VOC emission cap quantification and optimization proposed in this study could provide scientific guidance for coordinated control of regional PM2.5 and O3 pollution in China. 相似文献
84.
In India coal combustion is the single largest source of emission of mercury which is a wide-spread persistent global toxicant, travelling across international borders through air and water. As a party to the Minamata convention, India aims to monitor and reduce Hg emissions and stricter norms are introduced for mercury emissions from power plants (30 μg/Nm3for flue gas in stack).This paper presents the results obtained during the experimental studies performed on mercury emissions at four coal-fired and one lignite-fired power plants in India. The mercury concentration in the feed coal varied between 0.12–0.27 mg/Kg. In the mercury mass balance, significant proportion of feed coal mercury has been found to be associated with fly ash, whereas bottom ash contained very low mercury. 80%–90% of mercury was released to air through stack gas. However, for circulating fluidised bed boiler burning lignite, about 64.8% of feed mercury was found to get captured in the fly ash and only 32.4% was released to air. The mercury emission factor was found to lie in the range of 4.7–15.7 mg/GJ. 相似文献
85.
D. Valiulis D.
eburnis J.
akalys K. Kvietkus 《Atmospheric environment (Oxford, England : 1994)》2002,36(39-40)
A new approach for the estimation of trace metal emissions in Vilnius city was implemented, using vertical concentration profiles in the urban boundary layer and road tunnel measurement data. Heavy metal concentrations were examined in fine and coarse particle fractions using a virtual impactor (cut-off size diameter 2.5 μm). Negative vertical concentration gradients were obtained for all metals (Ba, Pb, V, Sb, Zn) and both fractions. It was estimated that the vertical concentration gradient was formed due to emissions from an area of about 12 km2. Road tunnel measurements indicated that trace metal concentrations on fine particles were lower than those on coarse particles, which suggested that re-emitted road dust was highly enriched in trace metal due to historic emissions within the tunnel. Emission rates of different pollutants in the road tunnel were calculated using pollutant concentration differences at the tunnel entrance and exit and traffic flow data. Heavy metal emission rates from the area of Vilnius city were estimated using the vertical gradient of heavy metal concentrations and the coefficient of turbulent mixing, as derived from meteorological measurement data. The emission values calculated by the two different methods coincided reasonably well, which indicated that the main source of airborne trace metals in Vilnius city is traffic. The potential of the vertical concentration gradient method for the direct estimation of urban heavy metal emissions was demonstrated. 相似文献
86.
Claudio Carnevale Giovanna Finzi Enrico Pisoni Marialuisa Volta 《Ecological modelling》2009,217(3-4):219
To assess the impact of three different emission reduction scenarios on PM10 concentrations in Northern Italy, the TCAM multiphase model has been applied in the framework of the CityDelta III-CAFE EU project. The considered domain, that is characterized by high urban and industrial emissions and a dense road traffic, due to frequently stagnating meteorological conditions is often affected by severe PM10 levels, far from the European standard regulations. The impact evaluation has been performed in terms of both yearly mean values and 50 g/m3 exceedance days for the 2004 Base Case simulation. The results show that the three selected emission reduction scenarios up to 2020 improve air quality all over the domain, in particular, in the area with higher emission density. 相似文献
87.
Combustion and inorganic bromine emission of waste printed circuit boards in a high temperature furnace 总被引:1,自引:0,他引:1
High temperature combustion experiments of waste printed circuit boards (PCBs) were conducted using a lab-scale system featuring a continuously-fed drop tube furnace. Combustion efficiency and the occurrence of inorganic bromine (HBr and Br2) were systematically studied by monitoring the main combustion products continuously. The influence of furnace temperature (T) was studied from 800 to 1400 °C, the excess air factor (EAF) was varied from 1.2 to 1.9 and the residence time in the high temperature zone (RTHT) was set at 0.25, 0.5, or 0.75 s.Combustion efficiency depends on temperature, EAF and RTHT; temperature has the most significant effect. Conversion of organic bromine from flame retardants into HBr and Br2 depends on temperature and EAF. Temperature has crucial influence over the ratio of HBr to Br2, whereas oxygen partial pressure plays a minor role. The two forms of inorganic bromine seem substantially to reach thermodynamic equilibrium within 0.25 s. High temperature is required to improve the combustion performance: at 1200 °C or higher, an EAF of 1.3 or more, and a RTHT exceeding 0.75 s, combustion is quite complete, the CO concentration in flue gas and remained carbon in ash are sufficiently low, and organobrominated compounds are successfully decomposed (more than 99.9%).According to these results, incineration of waste PCBs without preliminary separation and without additives would perform very well under certain conditions; the potential precursors for brominated dioxins formation could be destroyed efficiently. Increasing temperature could decrease the volume percentage ratio of Br2/HBr in flue gas greatly. 相似文献
88.
89.
An air quality sampling program was designed and implemented to collect the baseline concentrations of respirable suspended
particulates (RSP = PM10), non-respirable suspended particulates (NRSP) and fine suspended particulates (FSP = PM2.5). Over a three-week period, a 24-h average concentrations were calculated from the samples collected at an industrial site
in Southern Delhi and compared to datasets collected in Satna by Envirotech Limited, Okhla, Delhi in order to establish the
characteristic difference in emission patterns. PM2.5, PM10, and total suspended particulates (TSP) concentrations at Satna were 20.5 ± 6.0, 102.1 ± 41.1, and 387.6 ± 222.4 μg m−3 and at Delhi were 126.7 ± 28.6, 268.6 ± 39.1, and 687.7 ± 117.4 μg m−3. Values at Delhi were well above the standard limit for 24-h PM2.5 United States National Ambient Air Quality Standards (USNAAQS; 65 μg m−3), while values at Satna were under the standard limit. Results were compared with various worldwide studies. These comparisons
suggest an immediate need for the promulgation of new PM2.5 standards. The position of PM10 in Delhi is drastic and needs an immediate attention. PM10 levels at Delhi were also well above the standard limit for 24-h PM10 National Ambient Air Quality Standards (NAAQS; 150 μg m−3), while levels at Satna remained under the standard limit. PM2.5/PM10 values were also calculated to determine PM2.5 contribution. At Satna, PM2.5 contribution to PM10 was only 20% compared to 47% in Delhi. TSP values at Delhi were well above, while TSP values at Satna were under, the standard
limit for 24-h TSP NAAQS (500 μg m−3). At Satna, the PM10 contribution to TSP was only 26% compared to 39% in Delhi. The correlation between PM10, PM2.5, and TSP were also calculated in order to gain an insight to their sources. Both in Satna and in Delhi, none of the sources
was dominant a varied pattern of emissions was obtained, showing the presence of heterogeneous emission density and that nonrespirable
suspended particulate (NRSP) formed the greatest part of the particulate load. 相似文献
90.
This study deals with the emission of methane in relation to changing environmental conditions and human impact, in three
mangrove ecosystems of south India. Time-varying fluxes of methane adopting the close chamber technique were used to estimate
CH4 emission from an unpolluted site (Pichavaram mangroves) and two polluted sites viz. (1) Ennore Creek mangroves (affected
by fertilizer effluents and crude oil discharges) and (2) Adyar estuary mangroves (affected by the discharges of organic and
industrial wastes), covering monthly and seasonal variations. The results indicate annual average CH4 emissions of 7.4, 5.02 and 15.4 mg m−2 h−1 from the sediment–water interface of the Pichavaram, Ennore Creek and Adyar estuary respectively. Emission characteristics
obtained at Pichavaram mangroves represent a natural variability with changing physico-chemical factors, whereas the emission
characteristics at Ennore Creek and Adyar estuary mangroves show anthropogenic influence. Several environmental factors such
as oxygen availability, organic matter, soil physical and chemical properties, in addition to human-mediated interventions
have been identified as influencing emission rates in the mangrove ecosystems. Preliminary CH4 emission estimates for the mangrove ecosystems along the Indian sub- continent and the tropical and subtropical coastline
of the world by linear extrapolation based on surface area range from 0.05 to 0.37 and 2.8 to 19.25 Tg CH4 year−1 respectively. Our results also highlight the impact of human activities on future emission of methane from the mangrove ecosystems.
Received: 3 March 1999 / Accepted: 14 September 1999 相似文献