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51.
Poliana Dutra Mai Laurence Maurice Emmanuel Tessier David Amouroux Daniel Coss Patricia Moreira-Turcq Henri Etcheber 《环境科学学报(英文版)》2018,30(6):24-40
Seasonal variability of dissolved and particulate methylmercury(F-MeHg, P-MeHg) concentrations was studied in the waters of the Amazon River and its associated Curuai floodplain during hydrological year 2005–2006, to understand the MeHg exchanges between these aquatic systems. In the oxic white water lakes, with neutral pH, high F-MeHg and P-MeHg concentrations were measured during the rising water stage(0.70 ± 0.37 pmol/L, n = 26) and flood peak(14.19 ± 9.32 pmol/g, n = 7) respectively, when the Amazon River water discharge into the lakes was at its maximum. The lowest mean values were reported during the dry season(0.18 ± 0.07 pmol/L F-MeHg, n = 10 and 1.35 ± 1.24 pmol/g P-MeHg, n = 8), when water and suspended sediments were outflowing from the lakes into the River. In these lakes,the MeHg concentrations were associated to the aluminium and organic carbon/nitrogen changes. In the black water lakes, with acidic pH and reducing conditions, elevated MeHg concentrations were recorded(0.58 ± 0.32 pmol/L F-MeHg, n = 16 and 19.82 ± 15.13 pmol/g PMeHg, n = 6), and correlated with the organic carbon and manganese concentrations. Elevated values of MeHg partition coefficient(4.87 Kd 5.08 log(L/kg) indicate that MeHg is mainly transported associated with the particulate phase. The P-MeHg enrichment detected in all lakes suggests autochthonous MeHg inputs from the sediments into the water column. The MeHg mass balance showed that the Curuai floodplain is not the source of P-MeHg for the Amazon River. 相似文献
52.
本文以三峡库区重庆忠县黄冲子小流域和工农沟小流域为研究区域,依据塘库修建时间(1955年)、退耕还林工程启动时间(2000年)和~(137)Cs示踪技术,确定了小流域不同时期产沙量及产沙模数,并分析比较了不同小流域的塘库沉积物~(137)Cs含量和产沙模数。研究结果表明,黄冲子小流域和工农沟小流域1955~1963年、1963~2000年、2001~2014年的产沙模数均呈下降趋势,库区小流域生态环境得到明显改善;黄冲子小流域不同时期产沙模数均大于工农沟小流域,工农沟塘库沉积物1963年~(137)Cs峰值和表层泥沙~(137)Cs浓度均小于黄冲子塘库,主要与小流域的土地利用类型以及侵蚀方式有关。在以后的研究中,应该加强库区小流域沟道侵蚀产沙量的定量估算,为长江经济带生态环境建设提供参考依据。 相似文献
53.
利用静态箱-气相色谱法对夏季(7月、8月和9月)长江河口湿地芦苇植被CO_2、CH_4和N_2O的叶面通量、茎秆扩散速率以及沉积物通量的日变化进行研究。结果显示,通过芦苇叶片排放的N_2O与CH_4的量分别为2.99μg/(m~2·h)和15.36μg/(m~2·h),CO_2则呈现白天吸收(-120.86 mg/(m~2·h))、夜间排放(69.39 mg/(m~2·h))的特点。芦苇茎秆N_2O、CH_4和CO_2平均扩散速率分别为1.96μg/h、142.45μg/h和10.69 mg/h,沉积物平均排放通量为N_2O 8.18μg/(m~2·h)、CH_41.58 mg/(m~2·h)、CO_2169.66 mg/(m~2·h)。芦苇茎秆和沉积物界面CH_4和CO_2的排放均呈现出明显的"单峰型"昼夜变化规律,其排放峰值集中在日照及温度最高的9:00至15:00。芦苇植株是影响温室气体排放变化的因素之一。芦苇植株在光合作用下吸收CO_2并促进CH_4的排放,而芦苇发达的根系及茎秆是温室气体排放的主要途径。同时,Pearson相关性分析表明温度对芦苇群落CH_4和NO2的排放影响显著,但与CO_2通量的相关性不明显。土壤氧化还原电位对3种气体的排放均有显著影响。 相似文献
54.
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56.
Evaluation of Water Quality in the Chillán River (Central Chile) Using Physicochemical Parameters and a Modified Water Quality Index 总被引:4,自引:0,他引:4
Debels P Figueroa R Urrutia R Barra R Niell X 《Environmental monitoring and assessment》2005,110(1-3):301-322
The Chillán River in Central Chile plays a fundamental role in local society, as a source of irrigation and drinking water,
and as a sink for urban wastewater. In order to characterize the spatial and temporal variability of surface water quality
in the watershed, a Water Quality Index (WQI) was calculated from nine physicochemical parameters, periodically measured at
18 sampling sites (January–November 2000). The results indicated a good water quality in the upper and middle parts of the
watershed. Downstream of the City of Chillán, water quality conditions were critical during the dry season, mainly due to
the effects of the urban wastewater discharge. On the basis of the results from a Principal Component Analysis (PCA), modifications
were introduced into the original WQI to reduce the costs associated with its implementation. WQIDIR2 and WQIDIR, which are both based on a laboratory analysis (Chemical Oxygen Demand) and three (pH, temperature and conductivity), respectively,
four field measurements (pH, temperature, conductivity and Dissolved Oxygen), adequately reproduce the most important spatial
and temporal variations observed with the original index. They are proposed as useful tools for monitoring global water quality
trends in this and other, similar agricultural watersheds in the Chilean Central Valley. Possibilities and limitations for
the application of the used methodology to watersheds in other parts of the world are discussed. 相似文献
57.
固定化微生物处理有机污染物的研究进展 总被引:4,自引:0,他引:4
综述了近年来固定化微生物技术用于有机污染物治理中的最新进展,这些有机污染物包括难降解有机污染物(酚类、芳香烃类等)及其它化合物(DMP、甲硫醇恶臭气体、制药废水等)。此外,对藻类固定化技术作了简介,并对固定化技术的应用前景及存在问题进行了评述。 相似文献
58.
Thomas W. May Michael J. Walther Jimmie D. Petty James F. Fairchild Jeff Lucero Mike Delvaux Jill Manring Mike Armbruster David Hartman 《Environmental monitoring and assessment》2001,72(2):179-206
The Republican River Basin of Colorado,Nebraska, and Kansas lies in a valley which contains PierreShale as part of its geological substrata. Selenium is anindigenous constituent in the shale and is readily leached intosurrounding groundwater. The Basin is heavily irrigated throughthe pumping of groundwater, some of which is selenium-contaminated, onto fields in agricultural production. Water,sediment, benthic invertebrates, and/or fish were collected from46 sites in the Basin and were analyzed for selenium to determinethe potential for food-chain bioaccumulation, dietary toxicity,and reproductive effects of selenium in biota. Resultingselenium concentrations were compared to published guidelines orbiological effects thresholds. Water from 38% of the sites (n = 18) contained selenium concentrations exceeding 5 g L-1, which is reported to be a high hazard for selenium accumulation into the planktonic food chain. An additional 12 sites (26% of the sites) contained selenium in water between 3–5 g L-1, constituting a moderate hazard. Selenium concentrations in sedimentindicated little to no hazard for selenium accumulation fromsediments into the benthic food chain. Ninety-five percent ofbenthic invertebrates collected exhibited selenium concentrationsexceeding 3 g g-1, a level reported as potentially lethal to fish and birds that consume them. Seventy-five percent of fish collected in 1997, 90% in 1998, and 64% in 1999 exceeded 4 g g-1selenium, indicating a high potential for toxicity andreproductive effects. However, examination of weight profilesof various species of collected individual fish suggestedsuccessful recruitment in spite of selenium concentrations thatexceeded published biological effects thresholds for health andreproductive success. This finding suggested that universalapplication of published guidelines for selenium may beinappropriate or at least may need refinement for systems similarto the Republican River Basin. Additional research is needed todetermine the true impact of selenium on fish and wildliferesources in the Basin. 相似文献
59.
Land use change is an important topic in the field of global environmental change and sustainable development. Land use change
modeling has attracted substantial attention because it helps researchers understand the mechanisms of land use change and
assists regulatory bodies in formulating relevant policies. Maotiao River Basin is located in the province of Guizhou, China,
which has a developed agricultural industry in the karst mountain areas. This paper selected biophysical and social–economic
factors as independent variables, and constructed a multiple logistic regression of farmland spatial distribution probability
by random sampling. Then, by using GIS technology and integrating the 2000 data, this study predicted the farmland spatial
pattern. When the predicted map was compared with the actual farmland map for 2000, we noted that 71% of the simulation is
in accordance with the 2000 farmland pattern. The result satisfactorily proves the reasonability and applicability of our
model. 相似文献
60.
博斯腾湖水质矿化度模型及预测研究 总被引:6,自引:0,他引:6
根据博斯腾湖1985~1995年水质监测数据和出入湖水量等水文数据观测值,采用水质扩散模型和盐量平衡关系推导出博斯腾湖大湖区(简称博湖)水质矿化度模型,并预测了几种情况下博湖水质矿化度及近几年变化趋势,分析了影响博湖水质矿化度的主要因素,为博湖的近期和远期环境保护规划、环境管理等提供科学依据. 相似文献