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排序方式: 共有198条查询结果,搜索用时 15 毫秒
1.
Larisse Montero Matthew Duane Urbano Manfredi Covadonga Astorga Giorgio Martini Massimo Carriero Alois Krasenbrink B.R. Larsen 《Atmospheric environment (Oxford, England : 1994)》2010,44(18):2167-2175
The present paper presents results from the analysis of 29 individual C2–C9 hydrocarbons (HCs) specified in the European Commission Ozone Directive. The 29 HCs are measured in exhaust from common, contemporary vehicle/engine/fuel technologies for which very little or no data is available in the literature. The obtained HC emission fingerprints are compared with fingerprints deriving from technologies that are being phased out in Europe. Based on the total of 138 emission tests, thirteen type-specific fingerprints are extracted (Mean ± SD percentage contributions from individual HCs to the total mass of the 29 HCs), essential for receptor modelling source apportionment. The different types represent exhaust from Euro3 and Euro4 light-duty (LD) diesel and petrol-vehicles, Euro3 heavy-duty (HD) diesel exhaust, and exhaust from 2-stroke preEuro, Euro1 and Euro2 mopeds. The fuels comprise liquefied petroleum gas, petrol/ethanol blends (0–85% ethanol), and mineral diesel in various blends (0–100%) with fatty acid methyl esters, rapeseed methyl esters palm oil methyl esters, soybean oil methyl or sunflower oil methyl esters. Type-specific tracer compounds (markers) are identified for the various vehicle/engine/fuel technologies.An important finding is an insignificant effect on the HC fingerprints of varying the test driving cycle, indicating that combining HC fingerprints from different emission studies for receptor modelling purposes would be a robust approach.The obtained results are discussed in the context of atmospheric ozone formation and health implications from emissions (mg km?1 for LD and mopeds and mg kW h?1 for HD, all normalised to fuel consumption: mg dm?3 fuel) of the harmful HCs, benzene and 1,3-butadiene.Another important finding is a strong linear correlation of the regulated “total” hydrocarbon emissions (tot-HC) with the ozone formation potential of the 29 HCs (ΣPO3 = (1.66 ± 0.04) × tot-RH; r2 = 0.93). Tot-HC is routinely monitored in emission control laboratories, whereas C2–C9 are not. The revealed strong correlations broadens the usability of data from vehicle emission control laboratories and facilitates the comparison of the ozone formation potential of HCs in exhaust from of old and new vehicle/engine/fuel technologies. 相似文献
2.
River channel migration and cutoff events within large river riparian corridors create heterogeneous and biologically diverse
landscapes. However, channel stabilization (riprap and levees) impede the formation and maintenance of riparian areas. These
impacts can be mitigated by setting channel constraints away from the channel. Using a meander migration model to measure
land affected, we examined the relationship between setback distance and riparian and off-channel aquatic habitat formation
on a 28-km reach of the Sacramento River, California, USA. We simulated 100 years of channel migration and cutoff events
using 11 setback scenarios: 1 with existing riprap and 10 assuming setback constraints from about 0.5 to 4 bankfull channel
widths (bankfull width: 235 m) from the channel. The percentage of land reworked by the river in 100 years relative to current
(riprap) conditions ranged from 172% for the 100-m constraint setback scenario to 790% for the 800-m scenario. Three basic
patterns occur as the setback distance increases due to different migration and cutoff dynamics: complete restriction of cutoffs,
partial restriction of cutoffs, and no restriction of cutoffs. Complete cutoff restriction occurred at distances less than
about one bankfull channel width (235 m), and no cutoff restriction occurred at distances greater than about three bankfull
widths (∼700 m). Managing for point bars alone allows the setbacks to be narrower than managing for cutoffs and aquatic habitat.
Results suggest that site-specific “restriction of cutoff” thresholds can be identified to optimize habitat benefits versus
cost of acquired land along rivers affected by migration processes. 相似文献
3.
Michele Citterio Mikael K. Sejr Peter L. Langen Ruth H. Mottram Jakob Abermann Signe Hillerup Larsen Kirstine Skov Magnus Lund 《Ambio》2017,46(1):146-159
Terrestrial freshwater runoff strongly influences physical and biogeochemical processes at the fjord scale and can have global impacts when considered at the Greenland scale. We investigate the performance of the HIRHAM5 regional climate model over the catchments delivering freshwater to Tyrolerfjord and Young Sound by comparing to the unique Greenland Ecological Monitoring database of in situ observations from this region. Based on these findings, we estimate and discuss the fraction of runoff originating from glacierized and non-glacierized land delivered at the daily scale between 1996 and 2008. We find that glaciers contributed on average 50–80% of annual terrestrial runoff when considering different sections of Tyrolerfjord–Young Sound, but snowpack depletion on land and consequently runoff happens about one month earlier in the model than observed in the field. The temporal shift in the model is a likely explanation why summer surface salinity in the inner fjord did not correlate to modelled runoff. 相似文献
4.
Eric S. Larsen Michael J. Pilat 《Journal of the Air & Waste Management Association (1995)》2013,63(9):1199-1206
An activated carbon moving bed system (10 to 100 acf m air flow) was tested for controlling VOC emissions from a commercial aircraft painting facility. The cross-flow moving adsorbent bed showed a VOC collection efficiency in the 77.1 to 99.6 percent range over a superficial gas velocity range of 27 to 185 ft/min (0.14-0.94 m/sec). The collection efficiencies were neither affected by a change in carbon flow rates from 5 to 8 Ib/hr (2.3 to 3.6 kg/hr) nor by a change in the gas superficial velocity from 27 to 185 ft/min. The VOC concentration in the emission stream from the painting hangar was found to vary by at least a factor of 20 (from 0.18 to 15 ppm) both over the five month period (during which the 15 system tests of about three hours each were conducted) and within a single eight hour work shift. 相似文献
5.
Riparian Bird Communities as Indicators of Human Impacts Along Mediterranean Streams 总被引:1,自引:0,他引:1
Riparian areas link aquatic and terrestrial habitats, supporting species-rich bird communities, which integrate both terrestrial
and aquatic processes. For this reason, inclusion of riparian birds in stream bioassessment could add to the information currently
provided by existing programs that monitor aquatic organisms. To assess if bird community metrics could indicate stream conditions,
we sampled breeding birds in the riparian zone of 37 reaches in 5 streams draining watersheds representing a gradient of agricultural
intensity in central Italy. As a more direct indicator of water quality, stream macroinvertebrates were also sampled for computation
of the Italian Extended Biotic Index (IBE). An anthropogenic index was calculated within 1 km of sampled reaches based on
satellite-derived land-use classifications. Predictive models of macroinvertebrate integrity based on land-use and avian metrics
were compared using an information-theoretic approach (AIC). We also determined if stream quality related to the detection
of riverine species. Apparent bird species diversity and richness peaked at intermediate levels of land-use modification,
but increased with IBE values. Water quality did not relate to the detection of riverine species as a guild, but two species,
the dipper Cinclus cinclus and the grey wagtail Motacilla cinerea, were only observed in reaches with the highest IBE values. Small-bodied insectivorous birds and arboreal species were detected
more often in reaches with better water quality and in less modified landscapes. In contrast, larger and granivorous species
were more common in disturbed reaches. According to the information-theoretic approach, the best model for predicting water
quality included the anthropogenic index, bird species diversity, and an index summarizing the trophic structure of the bird
community. We conclude that, in combination with landscape-level information, the diversity and trophic structure of riparian
bird communities could serve as a rapid indicator of stream-dwelling macroinvertebrates and, therefore, degradation of in-stream
biotic integrity. 相似文献
6.
Five 14C-labelled polychlorinated biphenyls: 2,4′,5-trichlorobiphenyl, 2,2′,4,5′-tetrachlorobiphenyl, 2,2′,4,5,5′-pentachlorobiphenyl, 2,2′,3,4,4′-pentachlorobiphenyl and 2,2′,4,4′,5,5′-hexachlorobiphenyl were administered orally to bile-cannulated rats. The activity secreted in the bile, excreted in the feces and the urine was determined. Residues of radioactivity in certain tissues and the carcass were also measured.The trichlorobiphenyl showed the highest absorption (93.8%±5.4) from the gastrointestinal tract and biliary secretion of radioactivity (87.6%±6.1 of the dose). The hexachlorobiphenyl showed the lowest absorption and biliary secretion, 28.2%±1.4 and 18.6%±1.3, respectively. The urinary excretion was low and the radioactive residues in the eviscerated carcasses increased with the chlorine content of the biphenyls. 相似文献
7.
Ana B. Payá-Pérez Mohammed S. Rahman Helle Skejø-Andresen Bo R. Larsen 《Environmental science and pollution research international》1996,3(4):183-188
The soil/water partition coefficient (Kd) of hexachlorobenzene (HCB) ranged from 220 1/kg to 1800 1/kg for eight soils having a wide range of physico-chemical properties. Kd normalised to soil organic carbon (Koc) was found to be 28000 ± 4800 1/kg. Anionic surfactant dodecylsulphate (DS) present at concentrations above the critical micellar concentration (CMC) caused reductions in the apparent soil/water partition coefficient (Kd *) in the range of 3–26 times for most soils and up to 36–91 times for sandy soils. Below CMC, at environmentally relevant surfactant concentrations, Kd * was reduced by a factor of 1–13. For clay and calcareous soils significant adsorption/complexation/precipitation of DS occurred. At the lowest DS concentration this produced a two-fold increase in Kd *. At increasing DS concentrations this effect was shielded by the solubihzing effect from DS. Monomer (Kmn) and micellar (Kmc) surfactant/water partition coefficients for HCB were determined to be, 980 ± 190 1/kg and 21000 ± 1600 1/kg, respectively. 相似文献
8.
Ralph I. Larsen Ph.D. William W. Stalker Charles R. Claydon 《Journal of the Air & Waste Management Association (1995)》2013,63(11):529-534
This progress report describes the National Air Pollution Technical Information Center currently under development in the Division of Air Pollution, Public Health Service. It briefly reviews the report "Science, Government, and Information" (Weinberg Report) and the White House delegation of responsibility to the Department of Health, Education, and Welfare for handling air pollution technical information. 相似文献
9.
Pryor SC Larsen SE Sørensen LL Barthelmie RJ 《Environmental pollution (Barking, Essex : 1987)》2008,152(3):667-678
This paper reports a study designed to test, evaluate and compare micro-meteorological methods for determining the particle number flux above forest canopies. Half-hour average particle number fluxes above a representative broad-leaved forest in Denmark derived using eddy covariance range from -7x10(7) m(-2) s(-1) (1st percentile) to 5x10(7) m(-2) s(-1) (99th percentile), and have a median value of -1.6x10(6) m(-2) s(-1). The statistical uncertainties associated with the particle number flux estimates are larger than those for momentum fluxes and imply that in this data set approximately half of the particle number fluxes are not statistically different to zero. Particle number fluxes from relaxed eddy accumulation (REA) and eddy covariance are highly correlated and of almost identical magnitude. Flux estimates from the co-spectral and dissipation methods are also correlated with those from eddy covariance but exhibit higher absolute magnitude of fluxes. 相似文献
10.
Biosensors for detection of mercury in contaminated soils 总被引:1,自引:0,他引:1
Bontidean I Mortari A Leth S Brown NL Karlson U Larsen MM Vangronsveld J Corbisier P Csöregi E 《Environmental pollution (Barking, Essex : 1987)》2004,131(2):255-262
Biosensors based on whole bacterial cells and on bacterial heavy metal binding protein were used to determine the mercury concentration in soil. The soil samples were collected in a vegetable garden accidentally contaminated with elemental mercury 25 years earlier. Bioavailable mercury was measured using different sensors: a protein-based biosensor, a whole bacterial cell based biosensor, and a plant sensor, i.e. morphological and biochemical responses in primary leaves and roots of bean seedlings grown in the mercury-contaminated soil. For comparison the total mercury concentration of the soil samples was determined by AAS. Whole bacterial cell and protein-based biosensors gave accurate responses proportional to the total amount of mercury in the soil samples. On the contrary, plant sensors were found to be less useful indicators of soil mercury contamination, as determined by plant biomass, mercury content of primary leaves and enzyme activities. 相似文献