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Fahime Abedini Seyed Ali Hosseini Aligholi Niaei Dariush Salari Milad Abbasi Shiva Marmarshahi 《International Journal of Green Energy》2018,15(1):20-27
The paper reports the production of syngas from dry reforming of methane (DRM) over La1?xCexNi1?yFeyO3 (x, y = 0–0.4) perovskites. A series of La1?xCexNi1?yFeyO3 were designed by central composite design (CCD) and synthesized by a sol–gel auto combustion method. Artificial neural network (ANN) approach was used to determine the relationship between preparation and operational parameters on the performance of the catalysts in the DRM process. Nickel mole fraction, lanthanum mole fraction, calcination temperature, and reaction temperature were considered as input variables, and conversion of methane was considered as the output variable. An ANN model with nine neurons in the hidden layer was the suitable in predicting conversion of methane. The genetic algorithm (GA) was subsequently used to determine the optimal preparation condition for enhancing the conversion of methane. La0.6Ce0.4Ni0.99Fe0.01O3 catalyst, calcined at 756°C was obtained to be the most active catalyst owing to the optimal composition of nickel and lanthanum in the catalyst formulation. 相似文献
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Parvaneh Nakhostin Panahi Ali Niaei Darush Salari Seyed Mahdi Mousavi Gérard Delahay 《环境科学学报(英文版)》2015,35(9):135-143
The influence of the various preparation methods of Cu-SAPO-34 nanocatalysts on the selective catalytic reduction of NO with NH3 under excess oxygen was studied. Cu-SAPO-34 nanocatalysts were prepared by using four techniques: conventional impregnation (IM), ultrasound-enhanced impregnation (UIM), conventional deposition precipitation (DP) using NaOH and homogeneous deposition precipitation (HDP) using urea. These catalysts were characterized in detail by various techniques such as N2-sorption, XRD, TEM, H2-TPR, NH3-TPD and XPS to understand the catalyst structure, the nature and the dispersed state of the copper species, and the acid sites for NH3 adsorption. All of the nanocatalysts showed high activities for NO removal. However, the activities were different and followed the sequence of Cu-SAPO-34 (UIM) > Cu-SAPO-34 (HDP) > Cu-SAPO-34 (IM) > Cu-SAPO-34 (DP). Based on the obtained results, it was concluded that the NO conversion on Cu-SAPO-34 nanocatalysts was mainly related to the high reducibility of the isolated Cu2 + ions and CuO species, the number of the acid sites and the dispersion of CuO species on SAPO-34. 相似文献
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Daneshvar N Salari D Niaei A Khataee AR 《Journal of environmental science and health. Part. B》2006,41(8):1273-1290
The present work mainly deals with photocatalytic degradation of a herbicide, erioglaucine, in water in the presence of TiO2 nanoparticles (Degussa P-25) under ultraviolet (UV) light illumination (30 W). The degradation rate of erioglaucine was not so high when the photolysis was carried out in the absence of TiO2 and it was negligible in the absence of UV light. We have studied the influence of the basic photocatalytic parameters such as pH of the solution, amount of TiO2, irradiation time and initial concentration of erioglaucine on the photodegradation efficiency of erioglaucine. A kinetic model is applied for the photocatalytic oxidation by the UV/TiO2 system. Experimental results indicated that the photocatalytic degradation process could be explained in terms of the Langmuir-Hinshelwood kinetic model. The values of the adsorption equilibrium constant, K, and the second order kinetic rate constant, k, were 0.116 ppm-1 and 0.984 ppm min-1, respectively. In this work, we also compared the reactivity between the commercial TiO2 Degussa P-25 and a rutile TiO2. The photocatalytic activities of both photocatalysts were tested using the herbicide solution. We have noticed that photodegradation efficiency was different between both of them. The higher photoactivity of Degussa P-25 compared to that of rutile TiO2 for the photodegradation of erioglaucine may be due to higher hydroxyl content, higher surface area, nano-size and crystallinity of the Degussa P-25. Our results also showed that the UV/TiO2 process with Degussa P-25 as photocatalyst was appropriate as the effective treatment method for removal of erioglaucine from a real wastewater. The electrical energy consumption per order of magnitude for photocatalytic degradation of erioglaucine was lower with Degussa P-25 than in the presence of rutile TiO2. 相似文献
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Salari Taghi Ebrahimi Roumiani Ahmad Kazemzadeh Emad 《Environmental science and pollution research international》2021,28(36):49627-49641
Environmental Science and Pollution Research - Nowadays, paying attention to globalization and the consumption of renewable energy on the ecological footprint is one of the most important issues in... 相似文献
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Zulkernain Nur Hanis Basant Nikita Ng Chuck Chuan Kriti Salari Marjan Mallick Shekhar 《Journal of Material Cycles and Waste Management》2023,25(5):2726-2752
Journal of Material Cycles and Waste Management - E-waste, also known as waste from electrical and electronic equipment, is a solid waste that accumulates quickly due to high demand driven by the... 相似文献
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