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Marcel van der Perk Philip N. Owens Lynda K. Deeks Barry G. Rawlins 《Water, Air, & Soil Pollution: Focus》2006,6(5-6):443-451
A spatially extensive geochemical data set of stream water and bed sediment composition across the Tamar catchment in south-west
England was analysed to identify the key bed sediment properties that control the in-stream dissolved reactive phosphorus
(DRP) concentrations during baseflow conditions. Linear regression analysis of the streamwater DRP concentrations and the
distribution coefficient K
d for DRP revealed that the former is positively correlated with total SiO2 and Al2O3, and negatively correlated with K2O. The primary control on these major element distributions is the dominant bedrock geology. The data suggest that streamwater
DRP concentrations are mainly controlled by adsorption to clay minerals. Where P concentrations in streamwater were considerably
elevated by inputs from point sources, DRP concentrations are also controlled by precipitation of hydroxyapatite. 相似文献
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van der Perk M Owens PN Deeks LK Rawlins BG Haygarth PM Beven KJ 《Journal of environmental quality》2007,36(3):694-708
Many models of phosphorus (P) transfer at the catchment scale rely on input from generic databases including, amongst others, soil and land use maps. Spatially detailed geochemical data sets have the potential to improve the accuracy of the input parameters of catchment-scale nutrient transfer models. Furthermore, they enable the assessment of the utility of available, generic spatial data sets for the modeling and prediction of soil nutrient status and nutrient transfer at the catchment scale. This study aims to quantify the unique and joint contribution of soil and sediment properties, land cover, and point-source emissions to the spatial variation of P concentrations in soil, streambed sediments, and stream water at the scale of a medium-sized catchment. Soil parent material and soil chemical properties were identified as major factors controlling the catchment-scale spatial variation in soil total P and Olsen P concentrations. Soil type and land cover as derived from the generic spatial database explain 33.7% of the variation in soil total P concentrations and 17.4% of the variation in Olsen P concentrations. Streambed P concentrations are principally related to the major element concentrations in streambed sediment and P delivery from the hillslopes due to sediment erosion. During base flow conditions, the total phosphorus (<0.45 microm) concentrations in stream water are mainly controlled by the concentrations of P and the major elements in the streambed sediment. 相似文献
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