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Behaviour of selected endocrine-disrupting chemicals in three sewage treatment plants of Beijing, China 总被引:3,自引:0,他引:3
Haidong Zhou Xia Huang Xiaolin Wang Xiahui Zhi Chengdui Yang Xianghua Wen Qunhui Wang Hiroshi Tsuno Hiroaki Tanaka 《Environmental monitoring and assessment》2010,161(1-4):107-121
Occurrence and fate of eight kinds of selected endocrine-disrupting compounds (EDCs) in three sewage treatment plants (STPs) of Beijing, China was investigated. These EDCs, composed of 4-octylphenol (4-OP), 4-n-nonylphenol (4-n-NP), bisphenol A (BPA), estrone (E1), 17α-estradiol (17α-E2), 17β-estradiol (E2), estriol (E3) and 17α-ethinylestradiol (EE2), in every step of STPs, were simultaneously analysed by gas chromatography/mass spectrometry after derivatisation. All the EDCs were detected in the influents of three STPs, and BPA was the most abundant compound. The concentrations of EDCs ranged from 36.6 ng/l of 17α-E2 (STP C) to 1342.3 ng/l of BPA (STP B) in the influent sewages and from below limits of detection of E2 and E3 (STP C) to 142.5 ng/l of E1 (STP B) in the effluent sewages. The STPs could not remove alkylphenols effectively from the aqueous phase with less than 40% reduction. BPA decreased over 90%, and steroid estrogens achieved considerable reductions from 64.8% of E2 to 94.9% of E3. Generally, biological treatment was more effective in removing alkylphenols, BPA and natural estrogens from the aqueous phase than primary treatment. However, the synthetic estrogen, EE2, was mostly removed by the primary treatment with about 63.5% reduction. It is the first time that the concentration of 17α-E2 in the sewage of China was reported in this paper. The compound might have a bearing with the waste effluents of dairy farms around urban area of Beijing. 相似文献
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T.?OkumuraEmail author H.?Nikaido K.?Yoshida M.?Kotaniguchi Y.?Tsuno Y.?Seto T.?Watanabe 《Marine Biology》2005,148(2):347-361
Most pandalid shrimps show protandric hermaphroditism, and male sexual differentiation is considered to be controlled by the androgenic gland. In the present study, we examined the histology of gonadal development during the male phase and sex change and the involvement of the androgenic gland in regulating male reproduction in laboratory-maintained Pandalus hypsinotus. Juvenile shrimps developed testicular tissues in the peripheral part of gonads during the age of 16–31 months and produced spermatozoa between 34 and 36 months. After reaching sexual maturity, male shrimps exhibited seasonal testicular development: active production of spermatozoa (February–May), disappearance of spermatozoa (spent, April–June), increase of spermatocytes (May–November), appearance of spermatids and spermatozoa in the gonads (November–February). The androgenic gland cells became larger and the rough endoplasmic reticulum in the cytoplasm developed at male sexual maturity. The cell structure shows that the androgenic gland hormone is a peptide. Furthermore, bilateral eyestalk ablation on immature male shrimps induced hypertrophy of the androgenic gland and acceleration of male sexual maturation. These results indicate the involvement of androgenic gland hormone and some eyestalk factor in regulating male sexual maturation. Over a 1-year laboratory-rearing period, some male shrimps (16.7%) changed sex. In transitional shrimps, testicular tissues in the gonads and androgenic glands degenerated; on the other hand, oocytes started yolk protein accumulation and hemolymph vitellogenin levels became high. These results suggest that androgenic gland degeneration is a trigger for sex change and that the vitellogenin level is a useful marker for sex change. 相似文献
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Characteristics of electrolysis, ozonation, and their combination process on treatment of municipal wastewater. 总被引:1,自引:0,他引:1
Naoyuki Kishimoto Yukako Morita Hiroshi Tsuno Yuuji Yasuda 《Water environment research》2007,79(9):1033-1042
The characteristics of municipal wastewater treatment by electrolysis, ozonation, and combination processes of electrolysis and aeration using three gaseous species (nitrogen [N2], oxygen [O2], and ozone [O3]) were discussed in this research using ruthenium oxide (RuO2)-coated titanium anodes and stainless-steel (SUS304) cathodes. Electrolysis and electrolysis with nitrogen aeration were characterized by a rapid decrease in 5-day biochemical oxygen demand (BODs) and total nitrogen and a slow decrease in chemical oxygen demand (COD). In contrast, ozonation, electrolysis with oxygen aeration, and electrolysis with ozone aeration were characterized by transformation of persistent organic matter to biodegradable matter and preservation of total nitrogen. The best energy efficiency in removing BOD5 and total nitrogen was demonstrated by electrolysis, as a result of direct anodic oxidation and indirect oxidation with free chlorine produced from the chloride ion (Cl-) at the anodes. However, electrolysis with ozone aeration was found to be superior to the other processes, in terms of its energy efficiency in removing COD and its ability to remove COD completely, as a result of hydroxyl radical (*OH) production via cathodic reduction of ozone. 相似文献
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Yong-Jin Park Hiroshi Tsuno Taira Hidaka Ji-Hoon Cheon 《Journal of Material Cycles and Waste Management》2008,10(1):46-52
In this study, the effect of operational parameters, such as solids retention time (SRT), pH, and substrate total solids (TS)
concentration, on acid fermentation efficiency was investigated. From batch tests, it was shown that the appropriate pH range
for thermophilic acidogens was around 6–7 and that the optimum pH condition was 6. From the continuous experiment, pH and
SRT were shown to be the most important operational parameters for solubilization and organic acid production. In contrast,
TS concentration did not show any obvious effect on chromium chemical oxygen demand (CODcr) solubilization when TS was in
the range 3.5%–10%. The optimum operational conditions for thermophilic acid fermentation were an SRT of 2 days and a pH of
6.
This research was carried as a part of the CREST project of Japan Science and Technology Agency. 相似文献
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