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排序方式: 共有124条查询结果,搜索用时 46 毫秒
1.
Qingtao Sheng Run-Ping Ye Weibo Gong Xiufeng Shi Bang Xu Morris Argyle Hertanto Adidharm Maohong Fan 《环境科学学报(英文版)》2020,32(6):106-117
Direct synthesis of dimethyl ether(DME) by CO_2 hydrogenation has been investigated over three hybrid catalysts prepared by different methods:co-precipitation,sol-gel,and solid grinding to produce mixed Cu,ZnO,ZrO_2 catalysts that were physically mixed with a commercial ferrierite(FER) zeolite.The catalysts were characterized by N_2 physisorption,X-ray diffraction(XRD),transmission electron microscopy(TEM),X-ray photoelectron spectroscopy(XPS),temperature programmed desorption of CO_2(CO_2-TPD),temperature programmed desorption of NH_3(NH_3-TPD),and temperature programmed H2 reduction(H_2-TPR).The results demonstrate that smaller CuO and Cu crystallite sizes resulting in better dispersion of the active phases,higher surface area,and lower reduction temperature are all favorable for catalytic activity.The reaction mechanism has been studied using in situ diffuse reflectance infrared Fourier transform spectroscopy(DRIFTS).Methanol appears to be formed via the bidentate-formate(b-HCOO) species undergoing stepwise hydrogenation,while DME formation occurs from methanol dehydration and reaction of two surface methoxy groups. 相似文献
2.
Citrullinaemia was presumed to be excluded in a fetus at risk by the direct assay of argininosuccinate synthetase in chorionic villi. The diagnosis was confirmed after amniocentesis by normal argininosuccinate synthetase activity in the cultured amniotic fluid cells and by a normal citrulline concentration in the amniotic fluid. The prediction of a normal fetus was confirmed at term by the birth of a non-citrullinaemic boy. 相似文献
3.
孟宗沟小流域是长江源头高寒牧区水土流失综合治理试点。通过沟道与坡面两方面的治理,工程措施与生物措施相结合,增加地面、坡面植被,栏蓄径流,减少泥沙下泄,在防护效能上取得了显著成果。 相似文献
4.
一株硝基苯高效降解菌的筛选及其降解特性 总被引:14,自引:0,他引:14
自南京化工厂下水道底泥和废水处理系统曝气池活性污泥中驯化分离得到一株能快速降解硝基苯的菌株,初步鉴定其为不动杆菌属菌株。该菌株降解硝基苯的最适宜环境条件为温度25℃~35℃,pH7~8,振荡速率大于120r/m。在适宜环境条件下,该菌株能够在24h内全部降解初始浓度不超过400mg/L的硝基苯,该浓度范围内硝基苯的降解过程符合零级动力学特征;当硝基苯的初始浓度超过400mg/L时,降解菌的生长受到毒害作用,该浓度范围内硝基苯的降解在开始有一个明显的停滞期,降解过程不再符合零级或一级动力学特征。 相似文献
5.
Verma Sitaram Sinha Alok 《Environmental science and pollution research international》2023,30(10):25205-25225
Environmental Science and Pollution Research - This study was conducted to inspect the spatial distribution, source identification, and risk assessment of groundwater arsenic (As) in different... 相似文献
6.
Ghosh Shreya Gandhi Mayuri van Hullebusch Eric D. Das Alok Prasad 《Environmental science and pollution research international》2021,28(30):40249-40263
Environmental Science and Pollution Research - There has been alarming depletion of manganese (Mn) reserves owing to the ongoing extensive mining operations for catering the massive industrial... 相似文献
7.
Bang Ho Quoc Nguyen Hiep Duc Vu Khue Hien To Thi 《Environmental Modeling and Assessment》2019,24(3):295-310
Environmental Modeling & Assessment - This paper describes the application of the air pollution model (TAPM-CTM) for photochemical airshed modelling in the Ho Chi Minh region. The model was... 相似文献
8.
Sumit K. Soni Rakshapal Singh Ashutosh Awasthi Alok Kalra 《Environmental science and pollution research international》2014,21(3):1971-1979
Pot culture experiments were conducted in a glasshouse to evaluate the effects of four efficient Cr(VI)-reducing bacterial strains (SUCR44, SUCR140, SUCR186, and SUCR188) isolated from rhizospheric soil, and four arbuscular mycorrhizal fungi (AMF—Glomus mosseae, G. aggregatum, G. fasciculatum, and G. intraradices) alone or in combination, on Zea mays in artificially Cr(VI)-amended soil. Presence of a strain of Microbacterium sp. SUCR140 reduced the chromate toxicity resulting in improved growth and yields of plants compared to control. The bioavailability of Cr(VI) in soil and its uptake by the plant reduced significantly in SUCR140-treated plants; the effects of AMF, however, either alone or in presence of SUCR140 were not significant. On the other hand, presence of AMF significantly restricted the transport of chromium from root to the aerial parts of plants. The populations of AMF chlamydospores in soil and its root colonization improved in presence of SUCR140. This study demonstrates the usefulness of an efficient Cr(VI)-reducing bacterial strain SUCR140 in improving yields probably through reducing toxicity to plants by lowering bioavailability and uptake of Cr(VI) and improving nutrient availability through increased mycorrhizal colonization which also restricted the transport of chromium to the aerial parts. 相似文献
9.
Contamination of groundwater and risk assessment for arsenic exposure in Ha Nam province, Vietnam 总被引:2,自引:0,他引:2
The characteristics of arsenic-contaminated groundwater and the potential risks from the groundwater were investigated. Arsenic contamination in groundwater was found in four villages (Vinh Tru, Bo De, Hoa Hau, Nhan Dao) in Ha Nam province in northern Vietnam. Since the groundwater had been used as one of the main drinking water sources in these regions, groundwater and hair samples were collected in the villages. The concentrations of arsenic in the three villages (Vinh Tru, Bo De, Hoa Hau) significantly exceeded the Vietnamese drinking water standard for arsenic (10 microg/L) with average concentrations of 348, 211, and 325 microg/L, respectively. According to the results of the arsenic speciation testing, the predominant arsenic species in the groundwater existed as arsenite [As(III)]. Elevated concentrations of iron, manganese, and ammonium were also found in the groundwater. Although more than 90% of the arsenic was removed by sand filtration systems used in this region, arsenic concentrations of most treated groundwater were still higher than the drinking water standard. A significant positive correlation was found between the arsenic concentrations in the treated groundwater and in female human hair. The risk assessment for arsenic through drinking water pathways shows both potential chronic and carcinogenic risks to the local community. More than 40% of the people consuming treated groundwater are at chronic risk for arsenic exposure. 相似文献
10.
Tribedi P Sarkar S Mukherjee K Sil AK 《Environmental science and pollution research international》2012,19(6):2115-2124