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1.
Metals and arsenic in soils and corresponding vegetation at Central Elbe river floodplains (Germany) 总被引:1,自引:0,他引:1
Overesch M Rinklebe J Broll G Neue HU 《Environmental pollution (Barking, Essex : 1987)》2007,145(3):800-812
Floodplain soils at the Elbe river are frequently polluted with metals and arsenic. High contents of these pollutants were detected down to subsoil layers. NH4NO3-extractable (phytoavailable) Cd, Ni, and Zn were elevated in horizons with high acidity. Among five common floodplain plant species, Artemisia vulgaris showed highest concentrations of Cd, Cu, and Hg, Alopecurus pratensis of As and Phalaris arundinacea of Ni, Pb, and Zn. Relationships were weak between metal concentrations in plants and phytoavailable stocks in soil. As and Hg uptake seems to be enhanced on long submerged soils. Enrichments of Cd and Hg are linked to a special plant community composition. Grassland herbage sampled in July/August revealed higher concentrations of As (+122%), Hg (+124%), and Pb (+3723%) than in May. To limit harmful transfers into the food chain, low-lying terraces and flood channels revealing highest contaminations or phytoavailabilities should be excluded from mowing and grazing. 相似文献
2.
Santosh Kumar Sarkar Priyanka Mondal Jayanta Kumar Biswas Eilhann E. Kwon Yong Sik Ok Jörg Rinklebe 《Environmental geochemistry and health》2017,39(6):1245-1258
Our objective was to evaluate distribution and accumulation of trace elements (TEs) in surface sediments along the Hooghly (Ganges) River Estuary, India, and to assess the potential risk with view to human health. The TE concentrations (mg kg?1 dry weight) exhibited a wide range in the following order: Al (31.801 ± 15.943) > Fe (23.337 ± 7584) > Mn (461 ± 147) > S (381 ± 235) > Zn (54 ± 18) > V (43 ± 14) > Cr (39 ± 15) > As (34 ± 15) > Cu (27 ± 11) > Ni (24 ± 9) > Se (17 ± 8) > Co (11 ± 3) > Mo (10 ± 2) > Hg (0.02 ± 0.01). Clay, silt, iron, manganese and sulphur were important for the accumulation of TE in the sediments as confirmed by factor analysis and Pearson correlation. The accumulation and dispersal of TEs were most likely to be governed by both tide-induced processes and anthropogenic inputs from point and non-point sources. Enrichment factor analysis and geoaccumulation index revealed serious contamination of the sediments with Se and As, while comparing the consensus-based sediment quality guidelines (SQGs), adverse biological effects to benthic fauna might be caused by As, Cu, Ni and Cr. This investigation may serve as a model study and recommends continuous monitoring of As, Se, Cu, Ni and Cr to ascertain that SQGs with respect to acceptable levels of TEs to safeguard geochemical health and ecology in the vicinity of this estuary. 相似文献
3.
European floodplain soils are frequently contaminated with potentially toxic inorganic substances. We used a multi-surface model to estimate the aqueous concentrations of Cd, Cu, Ni, Pb and Zn in three Mollic Fluvisols from the Central Elbe River (Germany). The model considered complexation in solution and interactions with soil organic matter (SOM), a clay mineral and hydrous Al, Fe and Mn oxides. The amounts of reactive metals were derived from extraction with 0.43 M HNO3. Modelling was carried out as a function of pH (soil pH ± 1.4) because it varies in floodplain soils owing to redox processes that consume or release protons. The fraction of reactive metals, which were dissolved according to the modelling, was predominantly <1%. Depending on soil properties, especially pH and contents of SOM and minerals of the clay fraction, the modelled concentrations partially exceeded the trigger values for the soil–groundwater pathway of the German soil legislation. This differentiation by soil properties was given for Ni, Pb and Zn. On the other hand, Cd was more mobile, i.e., the trigger values were mostly exceeded. Copper represented the opposite, as the modelling did not predict exceeding the trigger values in any horizon. Except for Pb and partially Zn (where oxides were more important), SOM was the most important adsorbent for metals. However, given the special composition and dynamics of SOM in mollic horizons, we suggest further quantitative and qualitative investigations on SOM and on its interaction with metals to improve the prediction of contaminant dynamics. 相似文献
4.
Antić-Mladenović Svetlana Kresović Mirjana Čakmak Dragan Perović Veljko Saljnikov Elmira Ličina Vlado Rinklebe Jörg 《Environmental geochemistry and health》2019,41(1):249-266
Environmental Geochemistry and Health - Extreme flooding in May, 2014 affected the sub-catchments of six major rivers in Serbia. The goal of the study was to evaluate the contents of potentially... 相似文献
5.
Shaheen Sabry M. Antoniadis Vasileios Kwon Eilhann E. Biswas Jayanta K. Wang Hailong Ok Yong Sik Rinklebe Jörg 《Environmental geochemistry and health》2018,40(1):561-562
Environmental Geochemistry and Health - Unfortunately, in the original publication of the article, Prof. Yong Sik Ok’s affiliation was incorrectly published. 相似文献
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7.
Sabry M. Shaheen Ali A. Balbaa Alaa M. Khatab Jörg Rinklebe 《Environmental geochemistry and health》2017,39(6):1305-1324
Soil reclamation via additives can cause contradictory effects on the mobilization of toxic elements in soils under dry and wet conditions. Therefore, our aim was to investigate the impact of compost and sulfur in two rates (1.25 and 2.5%) on fractionation, mobilization, and phyto-availability of cadmium (Cd) and nickel (Ni) to sorghum (dry soil) and barnyard grass (wet soil) in a fluvial soil spiked with 25 mg Cd or 200 mg Ni/kg soil. Compost decreased the solubility and mobilization of Cd (especially in dry soil) and Ni (in both soils). Sulfur increased the solubility of Cd (31% in dry soil—49% in wet soil) and Ni (4.6% in wet soil—8.7% in dry soil). Sulfur altered the carbonate fraction of Cd to the soluble fraction and the residual fraction of Cd and Ni to the non-residual fraction. Compost decreased Cd and increased Ni in sorghum, but enhanced Cd and degraded Ni in grass. Sulfur increased Cd and Ni in both plants, and the increasing rate of Cd was higher in grass than in sorghum, while Ni was higher in sorghum than in grass. These results suggest that compost can be used as an immobilizing agent for Cd in the dry soil and Ni in the wet soil; however, it might be used as mobilizing agent for Cd in the wet soil and Ni in the dry soil. Sulfur (with rate 2.5%) can be used for enhancing the phyto-extraction of Cd and Ni (especially Cd) from contaminated alkaline soils. 相似文献
8.
Tatiane Medeiros Melo Michael Bottlinger Elke Schulz Wilson Mozena Leandro Adelmo Menezes de Aguiar Filho Yong Sik Ok Jörg Rinklebe 《Environmental geochemistry and health》2017,39(6):1351-1364
The hydrothermal carbonization of sewage sludge has been studied as an alternative technique for the conversion of sewage sludge into value-added products, such as soil amendments. We tested the toxicity of biosolid hydrochar (Sewchar) to earthworms. Additionally, the toxicity of Sewchar process water filtrate with and without pH adjustment was assessed, using brine shrimps as a model organism. For a Sewchar application of 40 Mg ha?1, the earthworms significantly preferred the side of the vessel with the reference soil (control) over side of the vessel with the Sewchar treatments. There was no acute toxicity of Sewchar to earthworms within the studied concentration range (up to 80 Mg ha?1). Regarding the Sewchar process water filtrate, the median lethal concentration (LC50) to the shrimps was 8.1% for the treatments in which the pH was not adjusted and 54.8% for the treatments in which the pH was adjusted to 8.5. The lethality to the shrimps significantly increased as the amount of Sewchar process water filtrate increased. In the future, specific toxic substances in Sewchar and its process water filtrate, as well as their interactions with soil properties and their impacts on organisms, should be elucidated. Additionally, it should be identified whether the amount of the toxic compounds satisfies the corresponding legal requirements for the safe application of Sewchar and its process water filtrate. 相似文献
9.
Sarkar Santosh Kumar Mondal Priyanka Biswas Jayanta Kumar Kwon Eilhann E. Ok Yong Sik Rinklebe Jörg 《Environmental geochemistry and health》2018,40(1):567-567
Environmental Geochemistry and Health - Unfortunately, in the original publication of the article, Prof. Yong Sik Ok’s affiliation was incorrectly published. The author’s affiliation is... 相似文献
10.
Melo Tatiane Medeiros Bottlinger Michael Schulz Elke Leandro Wilson Mozena de Aguiar Filho Adelmo Menezes Ok Yong Sik Rinklebe Jörg 《Environmental geochemistry and health》2018,40(1):557-558
Environmental Geochemistry and Health - Unfortunately, in the original publication of the article, Prof. Yong Sik Ok’s affiliation was incorrectly published. The author’s affiliation is... 相似文献