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1.
Processes involved in uptake and release of nitrogen dioxide from soil and building stones into the atmosphere 总被引:1,自引:0,他引:1
Atmospheric NO2 was taken up by samples of various soils and building stones. The NO2 uptake rate constants were highest in soil samples taken during the summer months. However, the NO2 uptake rate constants of the soils and building stones were not significantly correlated with any of the following variables: moisture, pH, ammonium, nitrite, or nitrate. NO2 uptake by soil and stone was not abolished by autoclaving indicating a chemical uptake process. NO2 uptake by acidic and air-dry soils and stones resulted in nearly stoichiometric reduction of NO2 to NO. This reduction was enhanced by the addition of ferrous iron and was further enhanced by incubation under 1 ppmv SO2. The results suggest that NO2 reduction may be coupled to oxidation of ferrous to ferric iron which may be reduced again by atmospheric SO2 thus regenerating the ferrous iron content of the soil or stone. Conversion of NO2 to NO was not observed in neutral or/and moist soils and stones. NO2 was also taken up by purified and sterilized quartz sand moistend with water. This uptake was enhanced by addition of humic material but not by addition of bacteria which both had been extracted from genuine soil. Under most conditions, only uptake but no release of NO2 was observed. However, NO2 was released in air-dry soils that were heated to 45–65°C, or in ammonium-fertilized soil or stone that was drying up at room temperature. Under the latter conditions mimicking field practice, the NO2 release reached rates that were similar to the NO release rates. 相似文献
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Excessive nitrate-N in south-central Minnesota ditches and streams is related to land-use change, and may be contributing to the development of the zone of hypoxia in the Gulf of Mexico. Intensive land-use (agricultural management) has progressively increased as subsurface drainage has improved crop productivity over the past 25 years. We have examined water at varying scales for delta18O and, nitrate-N concentrations. Additionally, analysis of annual peak flows, and channel geomorphic features provided a measure of hydrologic change. Laboratory and field results indicate that agricultural drainage has influenced riverine source waters, concentrations of nitrate-N, channel dimensions and hydrology in the Blue Earth River (BER) Basin. At the mouth of the BER shallow ground water comprises the largest source water component. The highest nitrate-N concentrations in the BER and tributaries typically occurred in May and June and ranged from 7-34 mg L(-1). Peak flows for the 1.01-2-yr recurrence intervals increased by 20-to-206% over the past 25 years. Geomorphic data suggest that small channels (ditches) were entrenched by design, whereas, natural that are disconnected from an accessible riparian corridor. Frequent access to a functioning riparian zone is important for denitrification. 相似文献
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Torvanger Asbjørn Rypdal Kristin Kallbekken Steffen 《Mitigation and Adaptation Strategies for Global Change》2005,10(4):693-715
Carbon dioxide (CO2) capture and storage is increasingly being considered as an important climate change mitigation option. This paper explores
provisions for including geological CO2 storage in climate policy. The storage capacity of Norway's Continental Shelf is alone sufficient to store a large share
of European CO2 emissions for many decades. If CO2 is injected into oil reservoirs there is an additional benefit in terms of enhanced oil recovery. However, there are significant
technical and economic challenges, including the large investment in infrastructure required, with related economies of scale
properties. Thus CO2 capture, transportation and storage projects are likely to be more economically attractive if developed on a large scale,
which could mean involving two or more nations. An additional challenge is the risk of future leakages from storage sites,
where the government must take on a major responsibility. In institutional and policy terms, important challenges are the
unsettled status of geological CO2 storage as a policy measure in the Kyoto Protocol, lack of relevant reporting and verification procedures, and lack of decisions
on how the option should be linked to the flexibility mechanisms under the Kyoto Protocol. In terms of competitiveness with
expected prices for CO2 permits under Kyoto Protocol trading, the relatively high costs per tonne of CO2 stored means that geological CO2 storage is primarily of interest where enhanced oil recovery is possible. These shortcomings and uncertainties mean that
companies and governments today only have weak incentives to venture into geological CO2 storage. 相似文献
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Carl Folke Stephen Polasky Johan Rockstrm Victor Galaz Frances Westley Michle Lamont Marten Scheffer Henrik
sterblom Stephen R. Carpenter F. Stuart Chapin III Karen C. Seto Elke U. Weber Beatrice I. Crona Gretchen C. Daily Partha Dasgupta Owen Gaffney Line J. Gordon Holger Hoff Simon A. Levin Jane Lubchenco Will Steffen Brian H. Walker 《Ambio》2021,50(4):834
The COVID-19 pandemic has exposed an interconnected and tightly coupled globalized world in rapid change. This article sets the scientific stage for understanding and responding to such change for global sustainability and resilient societies. We provide a systemic overview of the current situation where people and nature are dynamically intertwined and embedded in the biosphere, placing shocks and extreme events as part of this dynamic; humanity has become the major force in shaping the future of the Earth system as a whole; and the scale and pace of the human dimension have caused climate change, rapid loss of biodiversity, growing inequalities, and loss of resilience to deal with uncertainty and surprise. Taken together, human actions are challenging the biosphere foundation for a prosperous development of civilizations. The Anthropocene reality—of rising system-wide turbulence—calls for transformative change towards sustainable futures. Emerging technologies, social innovations, broader shifts in cultural repertoires, as well as a diverse portfolio of active stewardship of human actions in support of a resilient biosphere are highlighted as essential parts of such transformations. 相似文献