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1.
Characterization and optimization of long-term controlled release system for groundwater remediation: a generalized modeling approach 总被引:1,自引:1,他引:1
A well-based reactive barrier system using controlled-release KMnO4 has been recently developed as a long-term in situ treatment option for plumes of dense and non-aqueous phase liquids in groundwater. In order to take advantage of the merits of controlled release systems (CRS) in environmental remediation, the release behavior needs to be optimized for the hydrologic and environmental conditions of target treatment zone. Where release systems are expected to be operated over long times, like for the reactive barriers, it may only be practical to describe the long-term behavior numerically. We developed a numerical model capable of describing release characteristics associated with variable forms and structures of long-term CRS. Sensitivity analyses and illustrative simulations showed that the release kinetics and durations would be constrained by changes in agent solubility, bulk diffusion coefficients, or structures of the release devices. The generality of the numerical model was demonstrated through simulations for CRS with monolithic and double-layered matrices. The generalized model was then used for actual design and analyses of an encapsulated-matrix CRS, which can yield constant release kinetics for several years. A well-based reactive barrier system (4.05 x 10(3)m3) using the encapsulated-matrix CRS can release approximately 1.65 kg of active agent (here MnO4(-)) daily over the next 6.6 yr, creating prolonged reaction zone in the subsurface. The generalized model-based, target-specific approach using the long-term CRS could provide practical tool for improving the efficacy of advanced in situ remediation schemes such as in situ chemical oxidation, bioremediation, or in situ redox manipulation. Development of techniques for adjusting the bulk diffusion coefficients of the release matrices and facilitating the lateral spreading of the released agent is warranted. 相似文献
2.
This paper describes an integrated approach for modeling flow and contaminant transport in hydraulically connected stream-aquifer systems. The code, FTSTREAM, extended the capabilities of the ground-water model, FTWORK, to incorporate chemical fate and transport in streams. Flow in the stream network is modeled as an unsteady, spatially varying flow, while transport modeling is based on a one-dimensional advection-dispersion equation. In addition to sorption and decay during transport in ground water, the model incorporates volatilization, settling and decay during transport in surface water. The interaction between surface water and ground water is accommodated by a leakage term and is implemented in the model using an iterative Picard-type procedure to ensure mass conservation across the interface between the two systems. The modeling approach is used to simulate contaminant transport in the Mad River, Ohio, which is hydraulically connected to a buried valley aquifer of sand and gravel outwash. The river is a receiving stream in the upstream part of the modeled area. Downstream, heavy pumping from a municipal well field causes the river to become a loosing stream. Induced infiltration from the river is responsible for a considerable portion of the well yield. The flow and transport model, developed for this study, simulates coupling between flow in the aquifer and the river. Hypothetical sources of contamination are introduced at selected locations in the upstream portion of the aquifer. The model is then used to simulate the expected transport in both the aquifer and the stream. A series of simulations elucidates the role of the river in facilitating the transport of the hypothetical contaminants in ground water and surface water. Effect of sorption, retardation and volatilization on contaminant transport is also examined for the case of the volatile organic compounds. 相似文献
3.
The concept of time perspective balance has attracted increased attention from scholars in the past decade, reflected in published evidence suggesting positive outcomes ranging from enhanced mood to life satisfaction for those individuals possessing balance among their past, present, and future time perspectives, and assumedly able to shift their time perspective to match situational demands. In this paper, we consider the notion of time perspective balance in an organizational setting within which much consequential adaptation often occurs—the team environment—and explore different configurations of time perspective balance in teams facing dynamic task contexts. Drawing from work on situational awareness, we first consider the mechanism by which time perspective balance likely influences individual adaptation in dynamic task-focused situations. Next, we postulate what types of team configurations—ones with more balanced time perspective uniformity or ones with more time perspective variety—might be more appropriate in dynamic contexts given key team conditions. We illustrate our analysis with examples from healthcare team settings and offer ideas for future research. 相似文献
4.
Dale Hattis John M. Wasson Guy S. Page Bonnie Stern Claire A. Franklin 《Journal of the Air & Waste Management Association (1995)》2013,63(9):1060-1066
This paper explores some detailed mechanistic hypotheses for the possible action of acid particles on the tracheobronchial region of the human respiratory system. Because of the buffering capacity and volume of mucus produced per day it appears doubtful that ordinary ambient exposures to acid particles could markedly change the overall pH of tracheobronchial mucus considered as a whole. However it is possible that individual acidic particles could contain enough acid to deliver localized “irritant signals” that could be the triggers for enhanced mucus secretion and cell division in sensitive portions of the bronchial tree, and thereby contribute to the processes involved in chronic bronchitis. Depending on the exact pH depression required for a “signal” to be perceived by the tracheobronchial epithelium, the acid content of the incoming particles per unit weight, and the effect of neutralization by ammonia in the upper respiratory tract, the minimum size of an acidic particle required to deliver a perceptible signal might range from about 0.4 to 0.7 microns for portions of the epithelium that are frequently swept by 4-micron mucus droplets. (For unprotected epithelium, however, it is conceivable that the minimum effective size for acid particles could be less.) Since particle number per unit weight declines dramatically with increasing particle size, the most potent fraction of particles in terms of signals delivered per μg/m3is likely to be just above the minimum size that is needed to produce an effective signal. The model developed here makes predictions of the relative potency of particles of different size and acid delivery capacity that could be tested in both experimental animal systems and human epidemiological studies. 相似文献
5.
We compared measures of ecosystem state across six adjacent land-tenure groups in the intact tropical savanna landscapes of
northern Australia. Tenure groups include two managed by Aboriginal owners, two national parks, a cluster of pastoral leases,
and a military training area. This information is of relevance to the debate about the role of indigenous lands in the Australian
conservation estate. The timing and frequency of fire was determined by satellite imagery; the biomass and composition of
the herb-layer and the abundance of large feral herbivores by field surveys; and weediness by analysis of a Herbarium database.
European tenures varied greatly in fire frequencies but were consistently burnt earlier in the dry season than the two Aboriginal
tenures, the latter having intermediate fire frequencies. Weeds were more frequent in the European tenures, whilst feral animals
were most abundant in the Aboriginal tenures. This variation strongly implies a signature of current management and/or recent
environmental history. We identify indices suitable for monitoring of management outcomes in an extensive and sparsely populated
landscape. Aboriginal land offers a unique opportunity for the conservation of biodiversity through the maintenance of traditional
fire regimes. However, without financial support, traditional practices may prove unsustainable both economically and because
exotic weeds and feral animals will alter fire regimes. An additional return on investment in Aboriginal land management is
likely to be improved livelihoods and health outcomes for these disadvantaged communities. 相似文献
6.
Terrie K. Boguski Robert G. Hunt William E. Franklin 《Resources, Conservation and Recycling》1994,12(3-4)
Life cycle inventory (LCI) is becoming more widely used as a tool to evaluate the resource and energy use and the environmental releases associated with various products. The methodology for handling different recycling scenarios is also becoming increasingly important. Several different methods exist for handling recycling in an LCI. The method described in this paper uses mathematical models to show that the same basic equations can be used to handle a variety of recycling options for multi-product systems. 相似文献
7.
Clay L. Montague Alexander V. Zale H. Franklin Percival 《Environmental management》1987,11(6):743-756
Many coastal resource managers believe estuarine marshes are critically important to estuarine fish and shellfish, not only because of the habitat present for juvenile stages, but also because of the export of detritus and plant nutrients that are consumed in the estuary. Concern has been widely expressed that diking and flooding marshes (impounding) for mosquito control and waterfowl management interferes with these values of marshes. Major changes caused by impoundment include an increase in water level, a decrease in salinity, and a decrease in the exchange of marsh water with estuarine water. Alteration of species composition is dramatic after impoundment. Changes in overall production and transport phenomena, however—and the consequences of these changes— may not be as great in some cases as the concern about these has implied. Although few data are available, a more important concern may be the reduction of access by estuarine fish and shellfish to the abundant foods and cover available in many natural, as well as impounded, marshes. Perhaps even more important is the occasional removal of free access to open water when conditions become unfavorable in impounded marsh that is periodically opened and closed. Collection of comparative data on the estuarine animal use of various configurations of natural and impounded marshes by estuarine animals should lead to improved management of both impounded and unimpounded marshes. 相似文献
8.
Sheryl L. Franklin David R. Maidment 《Journal of the American Water Resources Association》1986,22(4):611-621
ABSTRACT: A cascade model for forecasting municipal water use one week or one month ahead, conditioned on rainfall estimates, is presented and evaluated. The model comprises four components: long term trend, seasonal cycle, autocorrelation and correlation with rainfall. The increased forecast accuracy obtained by the addition of each component is evaluated. The City of Deerfield Beach, Florida, is used as the application example with the calibration period from 1976–1980 and the forecast period the drought year of 1981. Forecast accuracy is measured by the average absolute relative error (AARE, the average absolute value of the difference between actual and forecasted use, divided by the actual use). A benchmark forecast is calculated by assuming that water use for a given week or month in 1981 is the same as the average for the corresponding period from 1976 to 1980. This method produces an AARE of 14.6 percent for one step ahead forecasts of monthly data and 15.8 percent for weekly data. A cascade model using trend, seasonality and autocorrelation produces forecasts with AARE of about 12 percent for both monthly and weekly data while adding a linear relationship of water use and rainfall reduces the AARE to 8 percent in both cases if it is assumed that rainfall is known during the forecast period. Simple rainfall predictions do not increase the forecast accuracy for water use so the major utility of relating water use and rainfall lies in forecasting various possible water use sequences conditioned on sequences of historical rainfall data. 相似文献
9.
S. Taku Ide Kristian Jessen Franklin M. Orr Jr. 《International Journal of Greenhouse Gas Control》2007,1(4):481-491
CO2 can be effectively immobilized during CO2 injection into saline aquifers by residual trapping – also known as capillary trapping – a process resulting from capillary snap-off of isolated CO2 bubbles. Simulations of CO2 injection were performed to investigate the interplay of viscous and gravity forces and capillary trapping of CO2. Results of those simulations show that gas injection processes in which gravitational forces are weak compared to viscous forces (low gravity number Ngv) trap significantly more CO2 than do flows with strong gravitational forces relative to the viscous forces (high Ngv). The results also indicate that over a wide range of gravity numbers (Ngv), significant fractions of the trapping of CO2 can occur relatively quickly. The amount of CO2 that is trapped after injection ceases is demonstrated to correlate with Ngv. For some simulated displacements, effects of capillary pressure and aquifer dip angle on the amount and the rate of trapping are reported. Trapping increases when effects of capillary pressure and aquifer inclination are included in the model. Finally we show that injection schemes such as alternating injection of brine and CO2 or brine injection after CO2 injection can also enhance the trapping behavior. 相似文献
10.
Jerry F. Franklin 《Environmental management》1979,3(1):2-5
Simulation models are becoming increasingly important as tools for synthesizing and applying information in almost all aspects of land management. They are particulary valuable for predicting and comparing outcomes of alternative decisions and assumptions. Models also permit managers to consider and integrate the potential influences of a large number of variables. 相似文献