排序方式: 共有23条查询结果,搜索用时 15 毫秒
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Ma Hongxue Hu Guangchao Zhang Le Huo Xiangtao Guo Min Zhang Mei 《Journal of Material Cycles and Waste Management》2023,25(4):2222-2231
Journal of Material Cycles and Waste Management - This paper utilizes desulfurization ash (DA), fly ash (FA) and ordinary Portland cement (OPC) to prepare unfired high-strength road-base stones by... 相似文献
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基于密度泛函理论,模拟了单壁碳纳米管(SWNTs)对5种碱基的吸附作用.考察了SWNTs直径、电荷转移量、碱基最高占据分子轨道能(EHOMO)和最低未占据分子轨道能(ELUMO)与SWNTs吸附碱基的吸附能之间的关系.结果表明,随着SWNTs直径的增大,SWNTs吸附碱基的吸附能降低.SWNT(6,6)吸附5种碱基的最低吸附能Emin与由碱基转移到SWNTs的电荷转移量(Q)及碱基的EHOMO线性负相关,相关系数分别为-0.966和-0.804(P<0.05).吸附后SWNTs与碱基的前线轨道无重叠,且SWNTs电子结构未受影响,表明吸附行为属于物理吸附. 相似文献
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以黄花夹竹桃(Thevetia peruviana(Pers.)k.Schum.)和芒果(Mangifera indica L.)苗木为材料,研究4种臭氧(O3)体积分数[环境大气NF,φ(O3)=10×10-9~20×10-9;低体积分数处理E50,φ(O3)=50×10-9;中体积分数处理E100,φ(O3)=100×10-9;高体积分数处理E200,φ(O3)=200×10-9]下两种植物叶片膜脂过氧化程度、可溶性蛋白质质量分数、可溶性糖质量分数和保护酶活性的变化情况,旨在揭示地表臭氧体积分数升高条件下2种植物生理代谢活动变化机理及响应规律。结果表明:随臭氧体积分数的增加,2种植物丙二醛含量和膜透性均逐渐上升,且与臭氧体积分数呈显著正相关关系,说明两种植物膜脂过氧化程度加剧;低体积分数O3处理时两种植物可溶性蛋白质量分数均逐渐下降,高φ(O3)处理后小幅回升;黄花夹竹桃可溶性糖质量分数逐渐下降,芒果先上升后下降;2种植物的POD活性均显著上升,但上升幅度有较大差异;2种植物的CAT活性均呈先升高再降低的趋势。研究表明,不同体积分数的臭氧暴露下,黄花夹竹桃和芒果均受到不同程度的伤害,芒果对臭氧表现出较强的抗性,黄花夹竹桃对臭氧较敏感。 相似文献
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Li Guangchao Chen Wei Zhang Xuepeng Yang Zhen Wang Zhe Bi Pengshuai 《Environmental science and pollution research international》2022,29(50):75322-75337
Environmental Science and Pollution Research - Climate change affects the change of vegetation, and the analysis of vegetation change and its drivers in different globe climate zones is important... 相似文献
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Li Guangchao Chen Wei Zhang Xuepeng Bi Pengshuai Yang Zhen Shi Xinyu Wang Zhe 《Environmental science and pollution research international》2022,29(10):14219-14230
Environmental Science and Pollution Research - The increased growth of vegetation has the potential to slow global climate warming. Therefore, analyzing and predicting the response assessment of... 相似文献
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Temporal changes in soil partitioning and bioaccessibility of arsenic, chromium, and lead 总被引:1,自引:0,他引:1
The hazard imposed by trace element contaminants within soils is dependent on their ability to migrate into water systems and their availability for biological uptake. The degree to which a contaminant may dissociate from soil solids and become available to a target organism (i.e., bioaccessibility) is therefore a determining risk factor. We used a physiologically based extraction test (PBET) to estimate the bioaccessible fraction of arsenic-, chromium-, and lead-amended soil. We investigated soils from the A and B horizons of the Melton Valley series, obtained from Oak Ridge National Laboratory site, to address temporal changes in bioaccessibility. Additionally, common extractions that seek to define reactive pools of metals were employed and their correlation to PBET levels evaluated. With the exception of Pb amended to the A horizon, all other treatments exhibited an exponential decrease in bioaccessibility with incubation time. The bioaccessible fraction was less than 0.2 mg kg(-1) within 30 d of incubation for As and Cr in the A horizon and for As and Pb within the B horizon; Cr in the B horizon declined to nearly 0.3 mg kg(-1) within 100 d of aging. The exchangeable fraction declined with incubation period and, with the exception of Pb, was highly correlated with the decline in bioaccessibility. Our results demonstrate limited bioaccessibility in all but one case and the need to address both short-term temporal changes and, most importantly, the soil physiochemical properties. They further reveal the importance of incubation time on the reactivity of such trace elements. 相似文献
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流域社会经济的水环境效应评估新方法及在南四湖的应用 总被引:8,自引:4,他引:4
针对我国湖泊生态安全评估及“一湖一策”工作的需要,初步提出一种流域社会经济的水环境效应评估新方法,与以往思路不同的是,新方法体现了正向作用和逆向反馈、现状水平和未来演变趋势相结合的认知框架,并系统阐述了指标优选、评估标准确定、等级划分和不确定性评估方法.最后,选择水质良好的湖泊代表——南四湖开展案例解析.结果表明:通过当前水平和未来变化速率更能全面认识评估结果,也有利于确定流域社会经济系统调控战略的必要性及潜力、方向和阈值;南四湖评估指数从2000年的“Ⅳ级:较严重”提升到2010年的“Ⅱ级:较轻”,尤其是在2003年和2007年存在2个“跳跃式”提升,但若维持现状规模和高速发展速度,未来20年很可能呈现逐渐缓慢下降趋势,并长期处于“Ⅲ级:一般”水平;为了确保维持现状等级且稳中小幅度上升的趋势,到2030年,建议南四湖流域社会经济发展速度控制在过去11年平均增长速度的75%左右以下,环境响应措施力度可能需要提升到评估标准的Ⅰ级水平. 相似文献
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生物降解性是评估污染物环境持久性的重要依据,也是化学品是否获准生产及进入市场的评价指标。采用17位生物降解领域专家评估的生物降解等级数据,通过功能树(FT)算法建立了包含15个分子结构参数的初级生物降解和最终生物降解预测模型。外部验证结果表明,模型具有较好的预测准确性,初级生物降解性加权准确度(weighted accuracy,WA):训练集WA=84.1%,验证集WA=78.9%;最终生物降解性WA:训练集WA=91.0%;验证集WA=83.6%。预测正确性对化合物的杠杆值作图,表征了生物降解性模型的应用域。 相似文献