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The effect of various types of cement dust on the behaviour of sulphur dioxide in the air was investigated on model systems in different experimental conditions.Experiments were carried out with PC-15z-45s (Portland-blast furnace cement containing 15% blast furnace slag), PC-25p-35s (Portland-pozzolan cement containing 25% pozzolan) and EFD (electrofilter dust).EFD most effectively removed SO2 from the air stream. The next efficacious was PC-15z-45s, whereas PC-25p-35s was the least efficient. The efficacy of cement dusts for SO2 removal from the air stream depended on their chemical and granulometric composition and in particular on the size of specific surface.The rate of reaction was also influenced by experimental conditions—relative humidity, the length of contact, that is, the flow rate of gaseous mixture through the reactor, and the amount of cement dust.The experimental data show that in the contact between SO2 and cement dust catalytic oxidation of SO2 to sulphates takes place. Sulphates remain bound to the surface, from which they cannot be thermally desorbed, but can be released by extraction in the Soxhlet apparatus. 相似文献
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Photoreactivity of humic substances: relationship between fluorescence and singlet oxygen production 总被引:1,自引:0,他引:1
Christian Coelho Ghislain Guyot Alexandra ter Halle Luciano Cavani Claudio Ciavatta Claire Richard 《Environmental Chemistry Letters》2011,9(3):447-451
Humic substances are natural compounds abundantly present in the environment. They play a significant role in the natural
attenuation of pollution in surface water due to their capacity to generate reactive species upon solar light excitation.
Finding physico chemical parameters related to this property would be of a great help in the prediction studies of the organic
pollutants fate. In this work, we investigated relationships between the ability of the humic substances to produce singlet
oxygen and their fluorescence properties. For this, a series of sixteen humic acids, fulvic acids, and water-extractable organic
matter from soils were studied. The steady-state singlet oxygen concentrations in the irradiated humic substances solutions
were measured by monitoring the loss of furfuryl alcohol added as a singlet oxygen scavenger. The emission spectra of the
sixteen samples were also recorded. Values of the steady-state singlet oxygen concentrations and the emission intensities
showed significant variations among the humic samples and a parallel increase. Thus, here we demonstrate that the rate of
singlet oxygen production and the emission intensity of the humic samples are correlated, the best correlation being obtained
for emission wavelengths between 500 and 580 nm. This correlation which was never reported until now can be used to estimate
the singlet oxygen-production capacity of the humic substances based on their fluorescent properties. 相似文献
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中国目前的土壤污染修复资金主要来源于政府财政性投资,融资渠道较为单一。《土壤污染防治行动计划》实施后,如何满足实现土壤污染修复与治理目标的投资需求是一个迫切需要解决的问题,充分创新发挥市场力量,建立长效的融资政策机制是核心内容。本文评估了中国土壤污染修复与治理投融资政策现状,识别了投融资面临的关键问题和挑战,提出了"十三五"时期中国土壤修复与治理的投融资机制建设的政策建议,为"十三五"时期中国土壤修复投融资模式创新提供管理技术支撑。 相似文献
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