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An organo-montmorillonite-supported nanoscale zero-valent iron material(M-NZVI) was synthesized to degrade decabromodiphenyl ether(BDE-209). The results showed that nanoscale zero-valent iron had good dispersion on organo-montmorillonite and was present as a core-shell structure with a particle size range of nanoscale iron between 30–90 nm, characterized by XRD, SEM, TEM, XRF, ICP-AES, and XPS. The results of the degradation of BDE-209 by M-NZVI showed that the efficiency of M-NZVI in removing BDE-209 was much higher than that of NZVI. The efficiency of M-NZVI in removing BDE-209 decreased as the pH and the initial dissolved oxygen content of the reaction solution increased, but increased as the proportion of water in the reaction solution increased. 相似文献
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畜禽养殖业是"十二五"期间氨氮总量减排的重点,其清洁生产与末端治理技术种类繁多,不同技术在不同应用条件下减排效果差别显著。深入分析了国内外畜禽养殖业发展与污染现状,系统归纳了国内畜禽养殖业氨氮总量减排技术区域特征,综合使用层次-灰色综合评判法、费用-效益法、表单法等对氨氮总量减排技术进行了综合性的评价研究,构建了基于面向服务架构(SOA)的氨氮减排技术评估咨询平台。结果表明,氨氮总量减排技术评估方法与平台可大幅度提高技术评价的效率和精确度,可广泛应用于企业和管理部门氨氮减排的工程技术与环境管理工作。 相似文献
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Xiao Chen Yong Wang Jianyu Li Zhongheng Hu Ying Zhou Huayan Liu Hanfeng Lu 《环境科学学报(英文版)》2022,34(6):114-124
The preparation of highly active supported noble metal catalysts with a low noble metal loading has always been the ultimate goal of researchers working on catalysis. Hydrothermally treated Pt/Al2O3 (Pt/Al2O3-H) exhibits better catalytic activity than that (Pt/Al2O3-C) treated via the conventional calcination approach. At the high space velocity of 100,000 mL/(g∙hr), the temperature that correspond to 50% toluene conversion (T50) of Pt/Al2O3-H is 115°C lower than that of Pt/Al2O3-C, and the turnover frequency (TOF) value can reach 0.0756 sec−1. The mechanism by which the hydrothermal approach enhances Pt/Al2O3 activity has been investigated. The structure associated with the high catalytic activity of Pt nanoparticles (NPs) can be retained via hydrothermal treatment. Furthermore, the support is transformed to AlO(OH) with numerous surface hydroxyl groups, which in turn can facilitate the adsorption of toluene. And the synergistic effects of Pt NPs and AlO(OH) increases the contents of Pt in oxidation state and active oxygen, which are beneficial for toluene oxidation. 相似文献
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应用江苏地磁台站Z分量整点值资料,研究了江苏地区Z分量整点值的相关性及在江苏地区地震预报中的作用,给出了该法在江苏地区的异常判据指标,并应用该指标提取了1990~1997年的三个异常,其中两个异常有地震对应。 相似文献
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不同加热方式下催化氧化甲苯的性能研究 总被引:1,自引:0,他引:1
研究考察了微波单模腔、多模腔与传统电炉三种不同加热方式下甲苯的催化氧化性能,分析不同加热方式下进出口气体温度和固定床反应温度的变化,并对实验前后的Cu-Mn-Ce/TiO2-分子筛催化剂进行了扫描电镜、X射线衍射和比表面积等表征测试.研究表明,相同工艺条件下电炉加热、微波多模腔与单模腔加热对甲苯的去除效率分别为77%、83%和94%,对应的床层反应温度为265℃、215℃和145℃,微波加热的选择性、"热点效应"和偶极极化作用提高了甲苯的降解效率并降低其氧化温度和工艺处理能耗,微波单模腔内高的能量密度显著提高了甲苯的氧化效率并降低反应温度.催化剂表征发现,微波加热对催化剂结构与活性组分的分布几乎没有影响,而电炉加热则导致催化剂表面烧结与活性组分团聚,微波加热下催化剂更大的比表面积有利于甲苯的吸附与氧化降解. 相似文献
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贵州省煤中挥发性和半挥发性微量元素分布规律的初步研究 总被引:25,自引:0,他引:25
研究了贵州省四大煤田不同层位、不同煤种中Hg,As,Se,Pb,Cd,Tl,Zn,Sb等挥发性和半挥发性微量元素的分布规律。贵州省原煤中Hg,As,Se,Pb,Cd,Sb等元素的含量高于地壳克拉克值;Tl,Zn等的含量低于地壳克拉克值;另外,除了Pb,Zn外,贵州省原煤中Hg,As,Se,Cd的含量远远高于东北和内蒙古东部地区。微量元素聚类分析结果表明,Hg,As,Sb可能主要分布于煤的黄铁矿中;Zn和Se可能主要赋存于闪锌矿中;Cd可能部分存在于硫化物中,部分存在于硅酸盐矿物相中;Pb可能主要存在于硅酸盐矿物相中;而Tl在煤中的赋存形式较复杂。 相似文献