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采用Nafion修饰电极,以微分计时电位溶出法分析测定废水中对—氨基苯酚(PAP)。在选定的条件下,PAP的测定范围在1.0μ~0.5mmol/l之间;最低检测浓度为0.1μmol/l;标准偏差为1.6%:方法的回收率为92.5%~96.5%。 相似文献
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Climatic changes can be separated into two parts: natural changes -and human activity influenced on climatic changes. The observed data could not only show the effects caused by human activity. Several simulated results as simulated by the GCMs induced by the greenhouse effects in China .have been analysed. It is shown that an obvious warming of about 3-6℃ in winter and 2-5℃ in summer in China as simulated by the GCMs induced by doubling CO2 have been found. There are getting drier or wetter regions in China due to doubled CO2 as simulated by most of models. Comparing the simulated results with the observed data in China, some simulated results are able to be believed. The GCMs should be improved, especially in the regional areas. 相似文献
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凋落叶作为森林凋落物的主要组成部分,其溶出的大量有机质也是森林土壤可溶性有机质(DOM)的主要来源之一。研究森林凋落叶溶出DOM对PAHs增溶作用的影响有利于合理预测及评价森林土壤中PAHs的环境行为和生态风险。本研究采集了南亚热带常绿阔叶人工林的4种常见树种--尾叶桉(Eucalyptus urophylla)、木荷(Schima superba)、大叶相思(Acacia auriculiformis)和湿地松(Pinus elliottii)的新近凋落叶为试验材料,研究其DOM含量、组成与性质,对比分析了不同凋落叶DOM对菲的増溶作用及其与DOM性质的相关关系。结果表明,4种凋落叶的可溶性有机碳(DOC)质量分数在C 11.61~36.25 mg·g-1之间,其中尾叶桉的含量最大,湿地松最小。尾叶桉和木荷DOM的主要组分是可溶性糖(SS)和可溶性酚(SP),两者总C量占DOC的比例超过47%,而大叶相思和湿地松中SS和SP两者总量所占比例均低于30%。另外,4种凋落叶DOM的质量分数(以C计)与其电导率的线性关系图中有明显转折点,说明它们均具有表面活性剂的性质。凋落叶DOM在临界胶束浓度(CMC)之上对菲具有不同程度的増溶作用,其与菲的结合系数(logKDOC)的大小顺序为尾叶桉(3.05 L·kg-1)>木荷(3.02 L·kg-1)>大叶相思(2.79 L·kg-1)>湿地松(2.54 L·kg-1),这表明尾叶桉和木荷DOM的增溶作用明显高于大叶相思和湿地松DOM。经分析表明,logKDOC与各DOM在254、280 nm处的特征紫外吸光度值(SUV-A254、SUV-A280)及其SS、SP的相对含量均呈显著正相关(p<0.01),与A240/A420、A254/A400比值呈显著负相关(p<0.01),说明DOM的芳香化程度越高,分子量越大, SS与SP所占比例越高,其对菲的増溶效果越明显。 相似文献
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River damming provides a dominant human impact on river environments worldwide, and while local impacts of reservoir flooding
are immediate, subsequent ecological impacts downstream can be extensive. In this article, we assess seven research strategies
for analyzing the impacts of dams and river flow regulation on riparian ecosystems. These include spatial comparisons of (1)
upstream versus downstream reaches, (2) progressive downstream patterns, or (3) the dammed river versus an adjacent free-flowing
or differently regulated river(s). Temporal comparisons consider (4) pre- versus post-dam, or (5) sequential post-dam conditions.
However, spatial comparisons are complicated by the fact that dams are not randomly located, and temporal comparisons are
commonly limited by sparse historic information. As a result, comparative approaches are often correlative and vulnerable
to confounding factors. To complement these analyses, (6) flow or sediment modifications can be implemented to test causal
associations. Finally, (7) process-based modeling represents a predictive approach incorporating hydrogeomorphic processes
and their biological consequences. In a case study of Hells Canyon, the upstream versus downstream comparison is confounded
by a dramatic geomorphic transition. Comparison of the multiple reaches below the dams should be useful, and the comparison
of Snake River with the adjacent free-flowing Salmon River may provide the strongest spatial comparison. A pre- versus post-dam
comparison would provide the most direct study approach, but pre-dam information is limited to historic reports and archival
photographs. We conclude that multiple study approaches are essential to provide confident interpretations of ecological impacts
downstream from dams, and propose a comprehensive study for Hells Canyon that integrates multiple research strategies. 相似文献
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Volunteer monitoring of natural resources is promoted for its ability to increase public awareness, to provide valuable knowledge, and to encourage policy change that promotes ecosystem health. We used the case of volunteer macroinvertebrate monitoring (VMM) in streams to investigate whether the quality of data collected is correlated with data use and organizers' perception of whether they have achieved these outcomes. We examined the relation between site and group characteristics, data quality, data use, and perceived outcomes (education, social capital, and policy change). We found that group size and the degree to which citizen groups perform tasks on their own (rather than aided by professionals) positively correlated with the quality of data collected. Group size and number of years monitoring positively influenced whether a group used their data. While one might expect that groups committed to collecting good-quality data would be more likely to use it, there was no relation between data quality and data use, and no relation between data quality and perceived outcomes. More data use was, however, correlated with a group's feeling of connection to a network of engaged citizens and professionals. While VMM may hold promise for bringing citizens and scientists together to work on joint conservation agendas, our data illustrate that data quality does not correlate with a volunteer group's desire to use their data to promote regulatory change. Therefore, we encourage scientists and citizens alike to recognize this potential disconnect and strive to be explicit about the role of data in conservation efforts. 相似文献
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Stream fish bioassessment methods assume that fish assemblages observed in sample sites reflect responses to local stressors, but fish assemblages are influenced by local factors as well as regional dispersal to and from connected streams. We hypothesized that fish movement to and from refugia and source populations in connected rivers (i.e., riverine dispersal) would weaken or decouple relations between fish community metrics and local environmental conditions. We compared fish-environment relations between streams that flow into large rivers (mainstem tributaries) and streams that lack riverine confluences (headwater tributaries) at multiple spatial grains using data from the USEPA's Environmental Monitoring and Assessment Program in the mid-Atlantic highlands, USA (n = 157 sites). Headwater and mainstem tributaries were not different in local environmental conditions, but showed important differences in fish metric responses to environmental quality gradients. Stream sites flowing into mainstem channels within 10 fluvial km showed consistently weaker relations to local environmental conditions than stream sites that lacked such mainstem connections. Moreover, these patterns diminished at longer distances from riverine confluences, consistent with the hypothesis of riverine dispersal. Our results suggest that (1) the precision of fish bioassessment metrics may be improved by calibrating scoring criteria based on the spatial position of sites within stream networks and (2) the spatial grain of fish bioassessment studies may be manipulated to suit objectives by including or excluding fishes exhibiting riverine dispersal. 相似文献
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