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1.
Sulphate, Nitrogen and Base Cation Budgets at 21 Forested Catchments in Canada, the United States and Europe 总被引:1,自引:0,他引:1
Watmough SA Aherne J Alewell C Arp P Bailey S Clair T Dillon P Duchesne L Eimers C Fernandez I Foster N Larssen T Miller E Mitchell M Page S 《Environmental monitoring and assessment》2005,109(1-3):1-36
To assess the concern over declining base cation levels in forest soils caused by acid deposition, input-output budgets (1990s
average) for sulphate (SO4), inorganic nitrogen (NO3-N; NH4-N), calcium (Ca), magnesium (Mg) and potassium (K) were synthesised for 21 forested catchments from 17 regions in Canada,
the United States and Europe. Trend analysis was conducted on monthly ion concentrations in deposition and runoff when more
than 9 years of data were available (14 regions, 17 sites). Annual average SO4 deposition during the 1990s ranged between 7.3 and 28.4 kg ha−1 per year, and inorganic nitrogen (N) deposition was between 2.8 and 13.8 kg ha−1 per year, of which 41–67% was nitrate (NO3-N). Over the period of record, SO4 concentration in deposition decreased in 13/14 (13 out of 14 total) regions and SO4 in runoff decreased at 14/17 catchments. In contrast, NO3-N concentrations in deposition decreased in only 1/14 regions, while NH4-N concentration patterns varied; increasing at 3/14 regions and decreasing at 2/14 regions. Nitrate concentrations in runoff
decreased at 4/17 catchments and increased at only 1 site, whereas runoff levels of NH4-N increased at 5/17 catchments. Decreasing trends in deposition were also recorded for Ca, Mg, and K at many of the catchments
and on an equivalent basis, accounted for up to 131% (median 22%) of the decrease in acid anion deposition. Base cation concentrations
in streams generally declined over time, with significant decreases in Ca, Mg and K occurring at 8, 9 and 7 of 17 sites respectively,
which accounted for up to 133% (median 48%) of the decrease in acid anion concentration. Sulphate export exceeded input at
18/21 catchments, likely due to dry deposition and/or internal sources. The majority of N in deposition (31–100%; median 94%)
was retained in the catchments, although there was a tendency for greater NO3-N leaching at sites receiving higher (<7 kg ha-1 per year) bulk inorganic N deposition. Mass balance calculations show that export of Ca and Mg in runoff exceeds input at
all 21 catchments, but K export only exceeds input at 16/21 sites. Estimates of base cation weathering were available for
18 sites. When included in the mass balance calculation, Ca, Mg and K exports exceeded inputs at 14, 10 and 2 sites respectively.
Annual Ca and Mg losses represent appreciable proportions of the current exchangeable soil Ca and Mg pools, although losses
at some of the sites likely occur from weathering reactions beneath the rooting zone and there is considerable uncertainty
associated with mineral weathering estimates. Critical loads for sulphur (S) and N, using a critical base cation to aluminium
ratio of 10 in soil solution, are currently exceeded at 7 of the 18 sites with base cation weathering estimates. Despite reductions
in SO4 and H+ deposition, mass balance estimates indicate that acid deposition continues to acidify soils in many regions with losses of
Ca and Mg of primary concern.
The U.S. Government's right to retain a non-exclusive, royalty free licence in and to any copyright is acknowledged.
The Canadian Crown reserves the right to retain a non-exclusive, royalty free licence in and to any copyright. 相似文献
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3.
Archambault DJ Li X Foster KR Jack TR 《Environmental monitoring and assessment》2006,115(1-3):509-530
Ethephon, which releases ethylene within plant tissues after application, was chosen to perform assessments of the relative sensitivity of crops to ethylene and to determine which stages of plant development were most sensitive. The species chosen were: barley, wheat, oats, canola and field pea, all of which are important crops in the province of Alberta, Canada. Plants were treated with ethephon at one of 7 different stages. Plants were assessed for their vegetative and reproductive growth, including height, biomass, yield and seed quality. Visual symptoms were photographed and documented to compare them with symptoms caused by ethylene applied as a gas. It was concluded that in barley, wheat and canola the late vegetative and early reproductive stages were most sensitive, at least when sensitivity was defined as reductions in yield and quality. As for field pea, ethephon had no effect on yield but did cause increased numbers of pods, which in certain conditions could lead to increased yields. Significant effects on vegetative growth were only observed in the early vegetative stages of development but with no effects on yield. The screening protocol successfully identified sensitive cultivars and growth stages for further investigation of the effects of ethylene exposure. 相似文献
4.
The goal of this study was to develop a robust method of analyzing surface water samples for S-triazine herbicides, chloroacetanilide herbicides, and their transformation products (TPs) using solid-phase extraction (SPE) followed by liquid chromatograph-mass spectrometry (LC-MS) with electrospray ionization (ESI) by in-source collision-induced dissociation (ISCID) capability of an orthogonal electrospray ionization probe on a single quadrupole LC-MS system. The method developed here met the goals of the study and yielded estimated method detection limits (EMDLs) averaging 0.3 ± 0.1 ng L(-1) for S-triazines and their TPs and 0.7 ± 0.4 ng L(-1) for chloroacetanilides and TPs. Spiked filtered river water yielded SPE recoveries ranging from 94.2 % ± 4.8 % for S-triazines and TPs after eliminating three compounds with less that 65 % recovery from analysis and 95.9 % ± 19 % for chloroacetanilides and their TPs. The method was field-tested with filtered water samples collected from four sites over a four-month period. Detectible values of S-triazines and TPs ranged from 0.3 to 1540 ng L(-1) with a mean of 79.3 and a median of 19.4 ng L(-1). Detectible values for chloroacetanilides and TPs ranged from 0.31 to 3780 ng L(-1) with a mean of 252 and a median of 25.6 ng L(-1). An additional goal was to determine if the method was useful for microbial degradation studies using native bacterial communities. The bacteria transformed atrazine (2-chloro-4-ethylamino-6-isopropylamino-S-triazine) solely into 2-hydroxy atrazine (2-hydroxy-4-ethylamino-6-isopropylamino-S-triazine) with concentrations of 78.4, 63.3 and 32.5 ng L(-1) after 12 days of incubation compared with 6.3 and 7.1 ng L(-1) for control dark and control sunlight respectively. 相似文献
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7.
K. James. DeCook Kennith E. Foster Martin M. Karpiscak 《Journal of the American Water Resources Association》1988,24(6):1295-1301
ABSTRACT: An index of residential water efficiency - a “W-Index” - can serve as a measure of effectiveness of water conservation features in the home. The index provides a calculated numerical value for each dwelling unit, derived from the number and kind of water-saving features present, including indoor and outdoor water savers and water harvesting or recycling systems. A W-Index worksheet, devised for on-site evaluation of single-family residences in the Tucson, Arizona, region shows that a nonconserving residence with all the water-using features would use 151,000 gallons per year or 148 gallons per capita per day (gpcpd), while the fully conserving model would use 35,300 gallons per year or 35 gpcpd and with water harvesting and graywater recycling systems would have a maximum W-Index of W-160. A Tucson water conservation demonstration home, Casa del Agua, received a rating of W-139, and field tests of about 30 homes in new Tucson subdivisions show values ranging from W-75 to W-100, indicating the incorporation of some water conservation in current new models. By adjustment of some climatic or water-use parameters, the W-Index format can be applied to various types of dwelling units or to other urban areas. The W-Index can be used by individual homeowners or builders to evaluate water efficiency of residential units, or by water providers or water management agencies as a device for promoting and achieving water conservation goals. 相似文献
8.
E T. Foster T. C. Chen J. P. Newton E. O. Isu 《Journal of the American Water Resources Association》1972,8(5):863-870
ABSTRACT. Theoretical and practical results are summarized for a study to determine optimal water resource allocation in a proposed water conservancy district. The area of this district, which covers several river basins, contains a large number of existing and proposed facilities such as reservoirs and diversions. The operation of all of these facilities was to be determined along with the sizing of the proposed facilities in order to optimize given objective functions. Related efforts in optimal river basin utilization were surveyed, and linear programming was selected as an expedient optimization technique. The problem is formulated by identifying time stages which together constitute a repetitive cycle such as a year. With these stages, it is possible to associate operational and capacity variables with network components, which are branches and nodes. Objective functions are assembled for the component variables. Constraint equations are written in terms of the variables to reflect network nodal continuity, capacity restrictions, and adjudications such as water rights. A numerical example is considered in which the existing and proposed facilities are aggregated to produce a small, tractable number of facilities. This paper examines the example results and suggests future improvements for models of this type. 相似文献
9.
The soluble fraction (105,000 x g, 30 min) of chicken liver homogenates contained an enzyme(s), probably a dehydrochlorinase(s), which metabolized lindane in vitro. The reaction was glutathione dependent and took place anaerobically. The enzyme(s) also metabolized the alpha- and delta-isomers but not the beta-isomer. About 66% of the in vitro metabolites were soluble in petroleum ether. From the ether-soluble fraction, o-, p- amd m-dichlorobenzene, 1,2,3- and 1,2,4-trichlorobenzene, gamma-2,3,4,5,6-pentachlorocyclohex-1-ene (gamma-PCCH), 2,3- and 2,4-dichlorophenol and 2,4,6-trichlorophenol were identified by comparison of mass spectra and gas chromatographic data with those of reference compounds. Seven additional metabolites were tentatively identified from their mass spectra data. These metabolites were: chlorobenzene, 2 isomers of trichlorocyclohexene, dichlorocyclohexadienetriol, chlorophenol, trichlorocyclohexenol and trichlorocyclohexanediol. The petroleum ether-extracted aqueous phase contained a number of unidentified conjugated metabolites. It was concluded that the metabolic pathway for lindane in the chicken is quite similar to that in the pheasant. 相似文献
10.
History and Importance of Land Use and Protection in the North Quabbin Region of Massachusetts (USA)
Evaluating the consequences and future of land protection requires broad temporal and spatial perspectives of ecological and cultural factors. We assessed the development of a system of protected areas comprising 37% of central Massachusetts in terms of changing rates and means of land protection. We compared protected areas to the surrounding matrix in terms of physical, biological, and historical features and used these results to raise issues concerning future planning. The rate, purpose, and means of land protection in the North Quabbin Region (168,312 ha) have been dynamic as a result of changes in cultural values and transformation of the landscape from predominantly agriculture to forest. Protected lands are managed by 25 federal and state agencies, private groups, and municipal departments and commissions and are physically and biologically typical of the regional landscape which results from (1) participation of diverse organizations with varied agendas; (2) predominance of large government acquisitions driven by landscape-scale criteria; and (3) absence of coordination among groups. The large area, relative homogeneity and largely undeveloped status of the North Quabbin Region suggest conservation goals distinct from those in the fragmented and extensively developed neighboring areas of the Connecticut River Valley and Cape Cod and Islands Region. Large tracts of forests, wetlands, and lakes in the North Quabbin Region provide (1) habitat for species requiring extensive, intact areas; (2) the opportunity to maintain broad-scale ecological processes; (3) connections to regional conservation areas; and (4) recreation. To realize the area's potential, a comprehensive plan must be based on a broad-scale perspective and historical understanding of the landscape. 相似文献