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Sanctorum H Elskens M Leermakers M Gao Y Charriau A Billon G Goscinny S De Cooman W Baeyens W 《Chemosphere》2011,85(2):203-209
PAHs, PCDD/Fs and non-ortho PCBs have been assessed in Yser and Upper-Scheldt river sediments. Higher contamination levels were observed in the Upper-Scheldt sediments: maximum concentrations for the 16 US-EPA PAHs, PCDD/Fs and non-ortho PCBs respectively amount to 8.9 mg kg−1, 12 ng TEQ kg−1 and 5.1 ng TEQ kg−1. Diagnostic PAH ratios in sediments and atmospheric samples suggest that the PAH compounds are from pyrolytic origin, more specifically combustion processes. The huge consumption of coal in cokes-ovens and smelters and its use for house-heating in Northern France, although decreasing during the last decades, are in support of that suggestion. PCDD/F fingerprints in sediments and deposition material indicate that OCDD is the dominant congener. In addition use of pentachlorophenol (PCP) in the past led to a minor contribution of PCDD/Fs in our sediment samples. Non-ortho PCBs form a substantial fraction of the total TEQ concentrations observed in the sediments. Since the 1980s and 1990s a substantial reduction of the PCDD/F sediment concentrations is observed, but this is not the case for the PAHs. 相似文献
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Le Billon P 《Disasters》2005,29(1):1-25
This paper examines advocacy initiatives by humanitarian and human rights organisations to address problems of governance in resource-rich and conflict-affected countries, focussing on the case of Angola. Humanitarian principles preclude the use of indiscriminate conditionality and point towards a cautious approach to advocacy aimed at assisting vulnerable populations. Furthermore, the relatively insignificant amount of aid supplied to resource-rich local authorities means that individual agencies have precious little leverage, especially when commercial interests rather than humanitarian or 'good governance' principles influence the priorities of bilateral donors. A context of resource wealth calls for: high levels of coordination and cooperation between human rights groups, aid agencies and donors; balanced use of conditionality, based on the drawing, by donors, of a clear distinction between emergency and development-oriented assistance; and a sustained effort to highlight the responsibilities of local authorities, foreign governments and businesses in meeting humanitarian and development objectives. 相似文献
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Dejaeger Karlien Criquet Justine Vanoppen Marjolein Vignal Cécile Billon Gabriel Cornelissen Emile R. 《Environmental Chemistry Letters》2022,20(6):3861-3882
Environmental Chemistry Letters - During disinfection of drinking water, natural organic matter reacts with chlorine to produce harmful disinfection by-products. The... 相似文献
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O. Connan D. Boust G. Billon L. Solier M. Rozet S. Bouderbala 《Journal of environmental radioactivity》2009,100(10):905-913
A sequential extraction protocol has been used to determine the solid-phase partition of 210Po and 210Pb in anoxic marine sediment from the roads of Cherbourg (France) in the central English Channel. Measurements were also obtained in pore waters, in which 210Po activities range between 1 and 20 mBq L−1 and 210Pb activities between 2.4 and 3.8 mBq L−1, with highest activities in the topmost layer. These activities are higher than in seawater, suggesting that sediment act as a source of both 210Po and 210Pb for overlying water. The 210Po profile in the pore waters is apparently correlated with those obtained for Fe, Mn and SO42−, suggesting an influence of early diagenetic processes on the 210Po solid-liquid distribution. In the sediment, 210Po is predominantly bound to organic matter or chromium reducible sulphides, and residuals (clay minerals and refractory oxides). Our results indicate that 210Po is not significantly bound to AVS, i.e. acid volatile sulphides: bioturbation could play a role by the early redistribution of 210Po bound to acid volatile sulphides in the sediment. 210Po, 210Pb and Pb exhibit differences in terms of distribution, probably due to a different mode of penetration in the sediment. This work provides information on solid and liquid distribution of 210Po and 210Pb in marine sediment. These data are very scarce in the litterature. 相似文献
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Lourino-Cabana B Billon G Magnier A Prygiel E Baeyens W Prygiel J Mikkelsen O Ouddane B 《Journal of environmental monitoring : JEM》2011,13(8):2124-2133
The monitoring of dissolved zinc in the De?le river was undertaken at three different periods of the years 2008 and 2009. Electrolabile concentrations of Zn were estimated every 2 hours for several weeks by using an ATMS (Automatic Trace metal Monitoring System) based on voltammetric measurements using a solid Ag-Hg rotating disc working electrode. Complementary measurements were carried out with DGT (Diffusive Gradient in Thin films) pistons deployed directly in the river for 24 hours. Water samples filtrated at 0.45 μm were also analysed by HR-ICP-MS to estimate the total dissolved concentrations of zinc and other trace metals. High frequency monitoring of zinc over several weeks in the De?le river indicated that the concentration could change significantly over short time periods. Resuspension of polluted sediment and biological activities are two main factors that control the behaviour of zinc in the De?le river. Furthermore, in May 2009, daily cycles of the electrolabile zinc fraction have been observed at relatively constant total dissolved concentration. It is assumed that this particular behaviour of zinc is based on an exchange between colloids and/or nonelectrolabile forms and free cation and inorganic complexes at a daily time scale. 相似文献
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Vdović N Billon G Gabelle C Potdevin JL 《Environmental pollution (Barking, Essex : 1987)》2006,141(2):359-369
The anthropogenic impact on the environment in the last century has proven to be very negative due to the fast development of industry. A typical example is the De?le River in northern France, one of the most polluted sites in this region. The concentrations of Pb, Cd, Zn and Cu in river sediments are 300, 800, 50 and 15 times higher, respectively, than the background values. The present study was undertaken to evaluate the capacity of already polluted sediments to capture metals released from industrial wastes (slag). As it were, in spite of the high metal pollution level, sediments have still shown the ability to adsorb metals released from slag under the conditions provided. Their efficiency in "cleaning up" some of the metals (e.g. Pb) seems to be additionally enhanced in anoxic conditions. This study provided some additional information on the importance of sediments as a pollutant sink. 相似文献
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