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1.
Natija Barhoumi Nihal Oturan Salah Ammar Abdellatif Gadri Mehmet A. Oturan Enric Brillas 《Environmental Chemistry Letters》2017,15(4):689-693
There is actually increasing concern about the accumulation of antibiotics, such as tetracycline, in soil and water bodies. There is therefore a need for efficient methods to degrade antibiotics and thus clean waters. Here we tested the degradation of tetracycline using the heterogeneous electro-Fenton-pyrite method and compared the results with the conventional electro-Fenton method. The reaction was performed with a boron-doped diamond or Pt anode and carbon-felt cathode allowing electrogeneration of H2O2 from O2 reduction. Results show an increasing tetracycline mineralization using the following methods: anodic oxidation with electrogenerated H2O2, electro-Fenton and then electro-Fenton-pyrite using boron-doped diamond. Ion-exclusion HPLC revealed the complete removal of malic malonic, succinic, acetic, oxalic and oxamic acids. Nitrogen present in tetracycline was mainly mineralized in NH4 +. The higher efficiency of electro-Fenton-pyrite is explained by self-regulation of soluble Fe2+ and pH to 3.0 from pyrite catalyst favoring larger ·OH generation from Fenton’s reaction. 相似文献
2.
Yakkou Lamia Houida Sofia Bilen Serdar Kaya Leyla Okyay Raouane Mohammed Amghar Souad Harti Abdellatif El 《Environmental science and pollution research international》2023,30(5):11719-11739
Environmental Science and Pollution Research - This study evaluated the impact of Aporrectodea molleri's coelomic fluid-associated bacteria (CFB) on Zea mays L. growth and soil biochemical... 相似文献
3.
Abdellatif Ouahsine Hassan Smaoui Khouane Meftah Philippe Sergent François Sabatier 《Environmental Fluid Mechanics》2013,13(2):169-187
We present a numerical model based on the hydro-morphodynamical coupling to study coastal sandbar migration. In order to improve both nonlinear and dispersive wave processes in relatively shallow water, we developed a finite element model based on the Legendre polynomials and on the Extended Boussinesq model. This model reproduces the propagation of wave trains with a high degree of accuracy on a greater range of depths than the standard Boussinesq models. We also implemented the Total Variation Diminishing schemes to improve the quality of the computed hydrodynamic fields, especially in areas where sharp flow gradients occurred. The coupled morpho-hydrodynamical model is then used to simulate the migration of real sandbars observed at Rousty beach (Mediterranean French coast). For verification the model results are compared with field measurements obtained from a small-scale field campaign carried out over two years at Rousty beach, and the results of this comparison are thoroughly discussed and analyzed. 相似文献
4.
Aziz Khalid Aziz Faissal Mamouni Rachid Aziz Layla Anfar Zakaria Azrrar Ahmed Kjidaa Bouthayna Saffaj Nabil Laknifli Abdellatif 《Environmental science and pollution research international》2022,29(57):86020-86035
Environmental Science and Pollution Research - In this paper, Cellana tramoserica (CT) shells were modified by copper and used as an adsorbent to remove thiabendazole (TBZ) from aqueous media. The... 相似文献
5.
A proper estimation of the skin shear stress τ s is necessary for a proper evaluation of sediment flux at the sediment–fluid interface. Several empirical formulas of the skin shear stress have been proposed in the literature for rippled bed as function of the factor form η/λ (η and λ are respectively the height and wavelength of the bedform). These formulas express that in the presence of bedform, τ s is a partition of the total shear stress τ b . In contrast, when the bottom is flat, τ s is exactly equal to τ b . Based on in situ measurements, Li (J Geophys Res 99:791–799, 1994) has proposed a new formula of τ s depending on u */η (u * is the friction velocity, ${u_{*}=\sqrt{\tau_{b}/\rho}}$ ), but not as a function of η/λ. This formulation appears physically more realistic, but does not cover the flat bottom range. The purpose of this short note is therefore the extension of the Li’s expression to this type of bottom. 相似文献
6.
The low biodegradability of polyphenolic compounds typically found in olive processing indicated that biological treatment is not always successful in the treatment of olive oil mill wastewater in term of COD removal. In this study the results of investigations on the applicability of Fenton‘s reagent in the treatment of this effluent were discussed. The efficiency of this method was determined. 86% of removal COD was obtained using 5 mol H2O2 and 0.4 mol Fe^2 per liter of crude OMW. The main parameters that govem the complex reactive system, i.e., time, pH, [H2O2] and [Fe(ll)] were studied. 相似文献
7.
El-Ghenymy A Arias C Cabot PL Centellas F Garrido JA Rodríguez RM Brillas E 《Chemosphere》2012,87(10):1126-1133
8.
Abdellatif El-Ghenymy Rosa María Rodríguez Enric Brillas Nihal Oturan Mehmet A. Oturan 《Environmental science and pollution research international》2014,21(14):8368-8378
The degradation of 230 mL of a 0.6-mM sulfanilamide solution in 0.05 M Na2SO4 of pH 3.0 has been studied by electro-Fenton process. The electrolytic cell contained either a Pt or boron-doped diamond (BDD) anode and a carbon-felt cathode. Under these conditions, organics are oxidized by hydroxyl radicals formed at the anode surface from water oxidation and in the bulk from Fenton’s reaction between initially added (and then electrochemically regenerated) Fe2+ and cathodically generated H2O2. From the decay of sulfanilamide concentration determined by reversed-phase liquid chromatography, an optimum Fe2+ concentration of 0.20 mM in both cells was found. The drug disappeared more rapidly using BDD than Pt, and, in both cases, it was more quickly removed with raising applied current. Almost total mineralization was achieved using the BDD/carbon-felt cell, whereas the alternative use of Pt anode led to a slightly lower mineralization degree. In both cells, the degradation rate was accelerated at higher current but with the concomitant fall of mineralization current efficiency due to the greater increase in rate of the parasitic reactions of hydroxyl radicals. Reversed-phase liquid chromatography allowed the identification of catechol, resorcinol, hydroquinone, p-benzoquinone, and 1,2,4-trihydroxybenzene as aromatic intermediates, whereas ion exclusion chromatography revealed the formation of malic, maleic, fumaric, acetic, oxalic, formic, and oxamic acids. NH4 +, NO3 ?, and SO4 2? ions were released during the electro-Fenton process. A plausible reaction sequence for sulfanilamide mineralization involving all detected intermediates has been proposed. The toxicity of the solution was assessed from the Vibrio fischeri bacteria luminescence inhibition. Although it acquired its maximum value at short electrolysis time, the solution was completely detoxified at the end of the electro-Fenton treatment, regardless of the anode used. 相似文献
9.
Rahmani Abdellatif Zerrouki Djamal Tabchouche Ahmed Djafer Lahcène 《Environmental science and pollution research international》2022,29(58):87509-87518
Environmental Science and Pollution Research - Oilfield-produced wastewater (OPW) provided by the local oil industry was used as a medium (without any pre-treatment) for the outdoor cultivation of... 相似文献
10.
Ahmed E. Awadallah Ateyya A. Aboul-Enein Abdellatif H. Mahmoud Sayed S. Abd El Rehim Ahmed K. El-Ziaty Ahmed K. Aboul-Gheit 《International Journal of Green Energy》2018,15(10):568-576
Zirconia-magnesia supported cobalt catalysts with various Zr/Mg atomic ratios were prepared and evaluated for non-oxidative catalytic decomposition of methane to produce COx-free hydrogen and carbon nanotube. The catalytic performance of the catalysts was performed in a continuous fixed bed flow reactor at 700°C under atmospheric pressure. The fresh and spent catalysts were characterized by XRD, TPR, BET, TEM, and Raman spectroscopy. The results showed that the change in Zr/Mg ratio of the mixed oxide support has a significant effect on the catalytic performance of the active Co metal. The catalyst 30%Co/Zr0.8Mg0.2 showed the highest activity and stability within the used series of catalysts with hydrogen yield reached up to 79%. Both Co/Mg1.0 and Co/Zr1.0 showed poor stability due to strong Co-Mg interaction and aggregation of Co species on Zr support, respectively. All catalysts produced mainly MWCNTs with different diameters depending on the Zr/Mg ratio. The outer diameter increased with increasing Zr content in the catalyst due to the enlargement of the particle size of cobalt as a result of aggregation. 相似文献