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热激活过硫酸盐降解卡马西平和奥卡西平复合污染的研究 总被引:4,自引:3,他引:1
研究了利用热激活过硫酸钠降解卡马西平和奥卡西平复合污染的规律.通过HPLC分析发现,在30~ 50℃时,卡马西平和奥卡西平的降解率随着温度的升高而升高,50℃时,反应90 min后卡马西平降解率为65.5%,30 min内几乎能完全降解奥卡西平;提高过硫酸钠浓度有利于卡马西平和奥卡西平的降解,当过硫酸钠浓度为12.0 mmo1.L-1时,可分别在90 min和20 min内几乎完全降解卡马西平和奥卡西平;升高pH能提高卡马西平和奥卡西平的降解率,当pH为9.0时,可分别在75 min和15 min内将卡马西平和奥卡西平几乎完全降解.经淬灭实验和电子顺磁共振波谱仪检测表明,热激活过硫酸钠降解卡马西平和奥卡西平体系中起主要作用的自由基是·OH.结果表明,该法操作简单,pH适用范围广,可以在短时间内高效降解卡马西平和奥卡西平,实际应用前景良好,并可为实际废水中卡马西平、奥卡西平或其他有机污染物的降解提供参考. 相似文献
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Huang Shaojian Dai Chunhao Zhou Yaoyu Peng Hui Yi Kexin Qin Pufeng Luo Si Zhang Xiaoshan 《Environmental science and pollution research international》2018,25(17):16548-16566
Environmental Science and Pollution Research - Plant leaves play a key role in the accumulation of PAHs, as they are able to capture PAHs from the air. In this paper, the mechanism, including... 相似文献
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Xiang Yujia Zhou Yuzhou Yao Bin Sun Yuqing Khan Eakalak Li Wei Zeng Guihua Yang Jian Zhou Yaoyu 《Environmental science and pollution research international》2023,30(4):8916-8927
Environmental Science and Pollution Research - Highly efficient and cost-effective adsorbents for antibiotic removal are the key to mitigate pollution by industrial wastewaters. Pyrolyzing low-cost... 相似文献
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利用液相色谱/质谱联用仪(HPLC-ESI-MS)分析了石油降解菌Pseudomonas aeruginosa W3以甘露醇为碳源所产鼠李糖脂生物表面活性剂的组成.结果表明,所产鼠李糖脂共检出6种主要的鼠李糖脂同系物,均由1~2个鼠李糖分子和1~2个含β羟基的碳链长度为8~12的饱和或不饱和脂肪酸分子构成,其主要组分的m/z为649.6和621.5,对应的结构是RhaRhaC10C10和RhaRhaC8C10,分别占总检出物质量的57%和15.5%.该鼠李糖脂混合物中双鼠李糖脂的含量达到90%,是目前报道的双鼠李糖脂含量较高的菌株之一.该糖脂类生物表面活性剂可将水的表面张力从71.4mN.m-1降到30.5mN.m-1,临界胶束浓度为48mg·L-1,在高温、高盐度及高pH等极端环境下,仍能保持较高的表面活性和乳化能力,在生物修复中具有潜在应用价值. 相似文献
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Mingyue Li Jiachao Zhang Xiao Yang Yaoyu Zhou Lihua Zhang Yuan Yang Lin Luo Qingyun Yan 《环境科学学报(英文版)》2021,33(4):263-272
Heavy metal pollution affects soil ecological function. Biochar and compost can effectively remediate heavy metals and increase soil nutrients. The effects and mechanisms of biochar and compost amendments on soil nitrogen cycle function in heavy-metal contaminated soils are not fully understood. This study examined how biochar, compost, and their integrated use affected ammonia-oxidizing microorganisms in heavy metal polluted soil. Quantitative PCR was used to determine the abundance of ammonia-oxidizing archaea (AOA) and bacteria (AOB). Ammonia monooxygenase (AMO) activity was evaluated by the enzyme-linked immunosorbent assay. Results showed that compost rather than biochar improved nitrogen conversion in soil. Biochar, compost, or their integrated application significantly reduced the effective Zn and Cd speciation. Adding compost obviously increased As and Cu effective speciation, bacterial 16S rRNA abundance, and AMO activity. AOB, stimulated by compost addition, was significantly more abundant than AOA throughout remediation. Correlation analysis showed that AOB abundance positively correlated with NO3?-N (r = 0.830, P < 0.01), and that AMO activity had significant correlation with EC (r = -0.908, P < 0.01) and water-soluble carbon (r = -0.868, P < 0.01). Those seem to be the most vital factors affecting AOB community and their function in heavy metal-polluted soil remediated by biochar and compost. 相似文献
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Lai Yoke Lee Jiang Yong Hu Say Leong Ong How Yong Ng Shih Wei Wong Yaoyu Feng Xiaolan Tan 《Water environment research》2008,80(8):725-731
The application of immunofluorescent labeling using quantum dots for detection of inactivated Cryptosporidium parvum oocysts in spiked water samples (reservoir water, treated wastewater effluent, permeate of a membrane bioreactor, and tap water) provided more consistent results compared with the organic fluorophores label. The varying degree of particles present in the different water samples (with turbidity ranging from 0.2 to 6.1 NTU) in nonconcentrated water samples had insignificant interference on the labeled counts (2-sample t-tests, p > 0.236) using the quantum dot label, while the quantum dot label provided an advantage of approximately 50% lower interference in concentrated water samples compared with the organic fluorophores label. 相似文献