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分别采用磷酸、硼酸、尿素掺杂改性活性碳纤维毡(ACF)(记为PACF、BACF和NACF),研究了改性前后ACF电极的表观结构及电化学性能。结果表明,PACF的孔隙率和比表面积增大,O—P等含氧基团增多,出现更多活性位点,电催化活性增强。以PACF为阴极,采用电化学法处理含活性红X-3B的模拟印染废水。在废水pH=3.0、Na2SO4投加量为50 mmol/L、Fe2+投加量为0.60 mmol/L、电流密度为20 mA/cm2的条件下,反应180 min后,废水脱色率达100%,UV254和COD去除率分别为97.13%和99.02%。重复使用5次后,PACF的性能仍好于ACF。 相似文献
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Jinjing Tang Jinsong Guo Fang Fang Youpeng Chen Lijing Lei Lin Yang 《环境科学学报(英文版)》2013,25(12):2403-2409
Excess nitrogenous compounds are detrimental to natural water systems and to human health. To completely realize autohy- drogenotrophic nitrogen removal, a novel 3-dimensional biofilm-electrode reactor was designed. Titanium was electroplated with ruthenium and used as the anode. Activated carbon fiber felt was used as the cathode. The reactor was separated into two chambers by a permeable membrane. The cathode chamber was filled with granular graphite and glass beads. The cathode and cathode chamber were inhabited with domesticated biofilm. In the absence of organic substances, a nitrogen removal efficiency of up to 91% was achieved at DO levels of 3.42 ± 0.37 mg/L when the applied current density was only 0.02 mA/cm^2. The oxidation of ammonium in biofilmelectrode reactors was also investigated. It was found that ammonium could be oxidized not only on the anode but also on particle electrodes in the cathode chamber of the biofilm-electrode reactor. Oxidation rates of ammonium and nitrogen removal efficiency were found to be affected by the electric current loading on the biofilm-electrode reactor. The kinetic model of ammonium at different electric currents was analyzed by a first-order reaction kinetics equation. The regression analysis implied that when the current density was less than 0.02 mA/cm^2, ammonium removal was positively correlated to the current density. However, when the current density was more than 0.02 mA/cm^2, the electric current became a limiting factor for the oxidation rate of ammonium and nitrogen removal efficiency. 相似文献
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